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《工程(英文)》 >> 2018年 第4卷 第3期 doi: 10.1016/j.eng.2018.05.017

天然气水合物浆液流变学研究综述

a Center for Hydrate Research, Chemical and Biological Engineering, Colorado School of Mines, Golden, CO 80401, USA
b Faculty of Chemical and Natural Resources Engineering, Universiti Malaysia Pahang, Pekan 26600, Malaysia
c Department of Chemistry, Colorado School of Mines, Golden, CO 80401, USA

收稿日期: 2017-12-13 修回日期: 2018-01-21 录用日期: 2018-05-16 发布日期: 2018-05-24

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摘要

天然气水合物是固体包裹化合物,由三维的氢键网络组成,可以用来捕获气体小分子,比如甲烷和二氧化碳。了解溶液中天然气水合物晶体的流变性能对于许多能源方面的应用至关重要,包括天然气在海底和陆地上的运输,以及气体分离、脱盐或封存等方面的技术应用。人们已经对水合物浆体流变学进行了多次实验和模型模拟;然而,理论与实验之间的联系并不明确。本文讲述了对高、低压流变仪的研究以及在高压流动环境下,一系列不同的过冷度(ΔTsub = TequilTexp)和流体条件的水合物浆体黏度测量技术的现状(包括水和油的连续系统)。本文介绍了天然气水合物泥浆相对黏度的理论模型,还讨论了实验和理论之间的联系。

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