期刊首页 优先出版 当期阅读 过刊浏览 作者中心 关于期刊 English

《中国工程科学》 >> 2022年 第24卷 第6期 doi: 10.15302/J-SSCAE-2022.06.015

气候协同的区域空气质量精细化调控战略研究

1. 北京大学环境科学与工程学院,环境模拟与污染控制国家重点联合实验室,北京100871;

2. 中国气象科学研究院,灾害天气国家重点实验室和大气化学重点开放实验室,北京100081;

3. 清华大学地球系统科学系,北京100084;

4. 江苏省大气环境监测与污染控制高技术研究重点实验室,江苏省大气环境与装备技术协同创新中心,南京信息工程大学环境科学与工程学院,南京  210044;

5. 清华大学环境学院,环境模拟与污染控制国家重点联合实验室,北京100084;

6. 中国环境科学研究院,北京100012;

7. 生态环境部环境规划院,北京100012

资助项目 :中国工程院咨询项目“气候协同的区域空气质量精细化调控战略研究”(2021-XZ-09) 收稿日期: 2022-04-18 修回日期: 2022-09-15

下一篇 上一篇

摘要

开展气候协同的区域空气质量精细化调控研究,对推进我国空气质量持续改善、构建未来气候背景下多污染物协同减排路径、实现绿色可持续发展具有重大战略意义。本文分析了区域大气污染演变规律、多污染物相互作用机制、污染防治策略与控制技术成效,完成了多视角剖析与多技术相互印证的集成研究,阐明了多污染物非线性响应关系,并梳理形成了区域精细化调控技术体系;在探讨气候变化与大气污染相互影响的基础上,提炼了空气质量精细化调控技术路线,提出了中长期空气质量改善策略和路线图。研究建议,针对当前的大气复合污染特征,PM2.5与O3协同控制的核心在于大气氧化性调控,需要持续强化一次污染物减排,同时因时因地并结合气候气象条件开展VOCs和NOx协同的精细化减排;发挥“双碳”政策的推动作用,通过四大结构调整和低碳转型,实现多类型污染物的协同深度减排,达到PM2.5与O3浓度的同步下降。

图片

图1

图2

图3

参考文献

[ 1 ] Zhang X Y, Zhong J T, Wang J Z, et al. The interdecadal worsening of weather conditions affecting aerosol pollution in the Beijing area in relation to climate warming [J]. Atmospheric Chemistry and Physics, 2018, 18(8): 5991‒5999.

[ 2 ] 中华人民共和国生态环境部‍ . 2015中国环境状况公报 [EBOL]‍. 2016-06-01 [ 2022-09-14 ]. https:www‍.mee‍.gov‍.cnhjzlsthjzkzghjzkgb201606P020160602333160471955‍.pdf .

[ 3 ] 中华人民共和国生态环境部‍‍. 2020中国生态环境状况公 报 [EBO L]‍. 2021-05- 26 [2022-09-14 ]. https:www‍.mee‍.gov‍.cnhjzlsthjzkzghjzkgb202105P020210526572756184785‍.pd f.

[ 4 ] Li Z J, Sun Y L, Wang Q Q, al et‍. Nitrate and secondary organic aerosol dominated particle light extinction in Beijing due to clean air action [J]‍. Atmospheric Environment, 2022, 269: 118833‍.

[ 5 ] Lu X, Zhang L, Wang X L, al et‍. Rapid increases in warm-season surface ozone and resulting health Impact in China since 2013 [J]‍. Environmental Science & Technology Letters, 2020, 7(4): 240‒247‍.

[ 6 ] Chu B W, Ma Q, Liu J, al et‍. Air pollutant correlations in China: Secondary air pollutant responses to NOx and SO2 control [J]‍. Environmental Science & Technology Letters, 2020, 7(10): 695‒700‍.

[ 7 ] 裘彦挺 , 吴志军 , 尚冬杰 , 等‍ . 我国城市大气PM 2‍.5 与O 3 浓度相关性的时空特征分析 [J]‍. 科学通报 , 2022 , 67 : 1 ‒ 10 ‍.

[ 8 ] Lu K D, Guo S, Tan Z F, al et‍. Exploring atmospheric free-radical chemistry in China: The self-cleansing capacity and the formation of secondary air pollution [J]‍. National Science Review, 2019, 6(3): 579‒594‍.

[ 9 ] Lu K D, Funchs H, Hofzumahaus A, al et‍. Fast photochemistry in wintertime haze: Consequences for pollution mitigation strategies [J]‍. Environmental Science & Technology, 2019, 53(18): 10676‒10684‍.

[10] Li J T, An X, Cui M M, al et‍. Simulation study on regional atmospheric oxidation capacity and precursor sensitivity [J]‍. Atmospheric Environment, 2021, 263: 1‒12‍.

[11] Peng X, Wang T, Wang W H, al et‍. Photodissociation of particulate nitrate as a source of daytime tropospheric Cl2 [J]‍. Nature Communications, 2022, 13(1): 939‍.

[12] Cheng Y F, Zheng G J, Wei C, al et‍. Reactive nitrogen chemistry in aerosol water as a source of sulfate during haze events in China [J]‍. Science Advances, 2016, 2(12): 1‒12‍.

[13] Wang W G, Liu M Y, Wang T T, al et‍. Sulfate formation is dominated by manganese-catalyzed oxidation of SO2 on aerosol surfaces during haze events [J]‍. Nature Communications, 2021, 12(1): 1993‍.

[14] Zhang X Y, Xu X D, Ding Y H, al et‍. The impact of meteorological changes from 2013 to 2017 on PM2‍.5 mass reduction in key regions in China [J]‍. Science China-Earth Sciences, 2019, 62(12): 1885‒1902‍.

[15] 张小曳 , 徐祥德 , 丁一汇 , 等‍ . 2013—2017年气象条件变化对中国重点地区PM 2‍.5 质量浓度下降的影响 [J]‍. 中国科学: 地球科学 , 2020 , 50 4 : 483 ‒ 500 ‍.

[16] Wang L L, Liu J K, Gao Z Q, al et‍. Vertical observations of the atmospheric boundary layer structure over Beijing urban area during air pollution episodes [J]‍. Atmospheric Chemistry and Physics, 2019, 19(10): 6949‒6967‍.

[17] Wang Z L, Wang C, Yang S, al et‍. Evaluation of surface solar radiation trends over China since the 1960s in the CMIP6 models and potential impact of aerosol emissions [J]‍. Atmospheric Research, 2019, 268: 1‒12‍.

[18] Wang Z L, Lin L, Xu Y Y, al et‍. Incorrect Asian aerosols affecting the attribution and projection of regional climate change in CMIP6 models [J]‍. npj Climate and Atmospheric Science, 2021, 4(1): 2‍.

[19] Lin L, Wang Z L, Xu Y Y, al et‍. Sensitivity of precipitation extremes to radiative forcing of greenhouse gases and aerosols [J]‍. Geophysics Research Letters, 2016, 43(18): 9860‒9868‍.

[20] Lin L, Wang Z L, Xu Y Y, al et‍. Larger sensitivities of precipitation extremes in response to aerosol than greenhouse gas forcing in CMIP5 models [J]‍. Journal of Geophysical Research: Atmosphere, 2018, 123(15): 8062‒8073‍.

[21] Wang Z L, Lin L, Yang M L, al et‍. The effect of future reduction in aerosol emissions on climate extremes in China [J]‍. Climate Dynamics, 2016, 47(9-10): 2885‒2899‍.

[22] Zhang Q, Zheng Y X, Tong D, al et‍. Drivers of improved PM2‍.5 air quality in China from 2013 to 2017 [J]‍. Proceedings of the National Academy of Sciences of the United States of America, 2019, 116(49): 24463‒24469‍.

[23] Ding D, Xing J, Wang S X, al et‍. Optimization of a NOx and VOC cooperative control strategy based on clean air benefits [J]‍. Environmental Science & Technology, 2022, 56(2): 739‒749‍.

[24] Ding D, Xing J, Wang S X, al et‍. Optimization of a NOx and VOC cooperative control strategy based on clean air benefits [J]‍. Environmental Science & Technology, 2021, 56(2): 739‒749‍.

[25] Tong D, Cheng J, Liu Y, al et‍. Dynamic projection of anthropogenic emissions in China: Methodology and 2015—2050 emission pathways under a range of socio-economic, climate policy, and pollution control scenarios [J]‍. Atmospheric Chemistry and Physics, 2020, 20(9): 5729‒5757‍.

[26] Cheng J, Tong D, Liu Y, al et‍. Air quality and health benefits of China´s current and upcoming clean air policies [J]‍. Faraday Discussions, 2021, 226: 584‒606‍.

[27] Cheng J, Tong D, Zhang Q, al et‍. Pathways of China´s PM2‍.5 air quality 2015—2060 in the context of carbon neutrality [J]‍. National Science Review, 2021, 8(12): 1‒11‍.

[28] Shi X R, Zheng Y X, Lei Y, al et‍. Air quality benefits of achieving carbon neutrality in China [J]‍. Science of the Total Environment, 2021, 795: 148784‍.

相关研究