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2022 1

2007 2

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Study on the NOx release rule along the boiler during pulverized coal combustion

JIN Jing, ZHANG Zhongxiao, LI Ruiyang

《能源前沿（英文）》 2007年 第1卷 第1期   页码 91-95 doi: 10.1007/s11708-007-0009-7

摘要： Numerical simulation and experimental study on NO release along the boiler during pulverized coal combustion have been conducted. With the increase of temperature the NO emission increased and the peak value of NO release moved forward. But when the temperature increased to a certain degree, NO emission began to reduce. NO emission increased with the increase of nitrogen content of coal. The peak value of NO release moved backwards with the increase of coal rank. NO emission increased obviously with the increase of stoichiometric ratio. There existed a critical average diameter of the pulverized coal (). If "d, NO emission reduced with the decrease of pulverized coal size. If >, NO emission reduced with the increase of the pulverized coal size. The results showed that the simulation results are in agreement with the experimental results for concentration distribution of NO along the axis of the furnace.
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Selective catalytic reduction of NOx from exhaust of lean-burn engine over Ag-Al2O3/cordierite catalyst

LI Junhua, KANG Shoufang, FU Lixin, HAO Jiming

《环境科学与工程前沿（英文）》 2007年 第1卷 第2期   页码 143-146 doi: 10.1007/s11783-007-0025-1

摘要： A highly effective Ag-AlO catalyst was prepared using the sol-gel method, and characterized by surface area using nitrogen adsorption, scanning electron microscopy (SEM), and transmission electron microscopy (TEM) techniques. The catalyst performance was tested on a real lean-burn gasoline engine. Only unburned hydrocarbons and carbon monoxide in the exhaust were directly used as reductant (without any external reductant), the maximum NO conversion could only reach 40% at 450?C. When an external reductant, ethanol was added, the average NO conversion was greater than 60%. At exhaust gas temperature range of 350 500?C, the maximum NO conversion reached about 90%. CO and HC could be efficiently oxidized with Pt-AO oxidation catalyst placed at the end of SCR converter. However, NO conversion drastically decreased because of the oxidation of some intermediates to NO again. The possible reaction mechanism was proposed as two typical processes, nitration, and reduction in HC-SCR over Ag-AlO.

关键词： lean-burn gasoline     external reductant     nitrogen adsorption     conversion     catalyst performance    

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NOx removal by non-thermal plasma reduction: experimental and theoretical investigations

《化学科学与工程前沿（英文）》 2022年 第16卷 第10期   页码 1476-1484 doi: 10.1007/s11705-022-2165-z

摘要： Green and efficient NOx removal at low temperature is still desired. NOx removal via non-thermal plasma (NTP) reduction is one of such technique. This work presents the experimental and theoretical study on the NOx removal via NTP reduction (NTPRD) in dielectric barrier discharge reactor (DBD). The effect of O2 molar fraction on NOx species in the outlet of DBD, and effects of NH3/NO molar ratio and discharge power of DBD on NOx removal efficiency are investigated. Results indicate that anaerobic condition and higher discharge power is beneficial to direct removal of NOx, and the NOx removal efficiency can be up to 98.5% under the optimal operating conditions. It is also found that adding NH3 is favorable for the reduction of NOx to N2 at lower discharge power. In addition, the NOx removal mechanism and energy consumption analysis for the NTPRD process are also studied. It is found that the reduced active species ( N∗, N−, N+, N2∗, NH2+, etc.) generated in the NTPRD process play important roles for the reduction of NOx to N2. Our work paves a novel pathway for NOx removal from anaerobic gas in industrial application.

关键词： ${\rm{NO}}_x $ removal     NTP reduction     mechanism     energy consumption    

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标题 作者 时间 类型 操作

Study on the NOx release rule along the boiler during pulverized coal combustion

JIN Jing, ZHANG Zhongxiao, LI Ruiyang

期刊论文

Selective catalytic reduction of NOx from exhaust of lean-burn engine over Ag-Al2O3/cordierite catalyst

LI Junhua, KANG Shoufang, FU Lixin, HAO Jiming

期刊论文

NOx removal by non-thermal plasma reduction: experimental and theoretical investigations

期刊论文