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Cu/Cr co-stabilization mechanisms in a simulated AlO-FeO-CrO-CuO waste system

《环境科学与工程前沿（英文）》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1408-4

摘要：

• Cu and Cr can be mostly incorporated into CuFexAlyCr2−x−yO4 with a spinel structure.

关键词： Spinel structure     Copper     Chromium     Co-stabilization     Thermal treatment    

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Microwave enhanced stabilization of copper in artificially contaminated soil

Hua ZHANG, Zhiliang ZHU, Noboru YOSHIKAWA

《环境科学与工程前沿（英文）》 2011年 第5卷 第2期   页码 205-211 doi: 10.1007/s11783-010-0290-2

摘要： Microwave processing was used to stabilize copper ions in soil samples. Its effects on the stabilization efficiency were studied as a function of additive, microwave power, process time, and reaction atmosphere. The stabilization efficiency of the microwave process was evaluated based on the results of the toxicity characteristic leaching procedure (TCLP) test. The results showed that the optimal experimental condition contained a 700 W microwave power, 20 min process time and 3 iron wires as the additive, and that the highest stabilization efficiency level was more than 70%. In addition, the different reaction atmospheres showed no apparent effect on the stabilization efficiency of copper in the artificially contaminated soil. According to the result of the Tessier sequential extraction, the partial species of copper in the contaminated soil was deduced to transform from unstable species to stable states after the microwave process.

关键词： microwave     copper     stabilization    

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Cement-based solidification/stabilization of contaminated soils by nitrobenzene

Jianguo LIU, Xiaoqin NIE, Xianwei ZENG, Zhaoji SU

《环境科学与工程前沿（英文）》 2012年 第6卷 第3期   页码 437-443 doi: 10.1007/s11783-012-0406-y

摘要： The cement-based solidification/stabilization (S/S) of nitrobenzene (NB) contaminated soils, with cement and lime as binders, sodium silicate solution and powder activated carbon (PAC) as additives, was optimized through an orthogonal experiment, and S/S efficiency was estimated by both leaching test and volatilization measurement. The leaching test results showed that the factors affecting S/S efficiency were NB concentration, cement-to-lime ratio and binder-to-soils ratio, in sequence. With increasing curing time, the leaching concentration of NB between different levels of the same factor in the orthogonal experiment decreased, and less than 9% NB leached out from the 28 d cured samples. The volatilization measurement results indicated that 0.5‰ of NB was volatilized during the mixing and curing processes for the samples without PAC in the 28 d cycle, whereas adding 2 wt% and 5 wt% PAC, with respect to the weight of contaminated soils, could reduce NB volatilization to half of its original values either during the mixing or curing process. The optimizing formula, that is, contaminated soils (dry weight):cement:lime= 100:25:25, with 5 wt% additional sodium silicate and 2 wt% additional PAC, was applied to the engineering application of NB contaminated soils. Both the leaching test results of the product and the ambient air quality monitoring results met related regulations during the treating process.

关键词： solidification/stabilization     nitrobenzene     contaminated soils     powder activated carbon    

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Analysis and stabilization control of a voltage source controlled wind farm under weak grid conditions

《能源前沿（英文）》 2022年 第16卷 第6期   页码 943-955 doi: 10.1007/s11708-021-0793-5

摘要： This paper investigates and discusses the interaction stability issues of a wind farm with weak grid connections, where the wind turbines (WTs) are controlled by a new type of converter control strategy referred to as the voltage source (VS) control. The primary intention of the VS control method is to achieve the high-quality inertial response capability of a single WT. However, when it is applied to multiple WTs within a wind farm, its weak-grid performance regarding the stability remains concealed and needs to be clarified. To this end, a frequency domain model of the wind farm under the VS control is first developed. Based on this model and the application of a stability margin quantification index, not only the interactions between the wind farm and the weak grid but also those among WTs will be systematically assessed in this paper. A crucial finding is that the inertial response of VS control has negative impacts on the stability margin of the system, and the dominant instability mode is more related to the interactions among the WTs rather than the typical grid-wind farm interaction. Based on this knowledge, a stabilization control strategy is then proposed, aiming for stability improvements of VS control while fulfilling the demand of inertial responses. Finally, all the results are verified by time-domain simulations in power systems computer aided design/electromagnetic transients including DC(PSCAD/EMTDC).

关键词： weak grids     voltage source (VS) control     wind turbine (WT)     stabilization control     wind farm     inertial response    

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The use of fine portions from construction and demolition waste for expansive soil stabilization: A review

Mgboawaji Claude UJILE; Samuel Jonah ABBEY

《结构与土木工程前沿（英文）》 2022年 第16卷 第7期   页码 803-816 doi: 10.1007/s11709-022-0835-z

摘要： Construction and demolition waste (CDW) are the largest waste products in the world today and competes as a viable recycled additive material in place of natural aggregates. Due to the increase in compressive strength of different mix proportions of CDW, it is also considered for reuse in concrete and subbase construction. This study shows the effect of CDW in expansive soil stabilization. The chemical and mechanical properties of these materials have shown that they are capable of developing compressive strength properties for replacement of cement with significant reduction in carbon emission. The inherent compositional properties of recycled CDW compared in this review suggests that CDW have good filler properties in highly expansive soils. Mixtures of crushed brick and recycled aggregates characterised based on chemical properties of different replacement ratios suggests that CDW of good-quality aggregates reduces swell potential of expansive soils and increased mechanical strength in pavement construction.

关键词： mixed fine portions     construction and demolition waste     expansive soil     soil stabilization    

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Phosphate-induced differences in stabilization efficiency for soils contaminated with lead, zinc, and

Jie Ren, Zhuo Zhang, Mei Wang, Guanlin Guo, Ping Du, Fasheng Li

《环境科学与工程前沿（英文）》 2018年 第12卷 第2期 doi: 10.1007/s11783-018-1006-2

摘要： Phosphates can cost-effectively decrease the mobility of Pb in contaminated soils. However, Pb always coexists with other metals in soil, their competitive reactions with phosphates have not been tested. In this study, the abilities of KH PO , K HPO , and K PO to stabilize Pb, Zn, and Cd in soils contaminated with a single metal or a ternary metal for different phosphorus/metal molar ratios were investigated. Results indicated that the stabilization efficiency of KH PO , K HPO , and K PO for Pb, Zn, and Cd in single metal contaminated soil (P/M ratio 0.6) was 96.00%–98.74%, 33.76%–47.81%, and 9.50%–55.79%, respectively. Competitive stabilization occurred in the ternary system, Pb exhibited a strong competition, the stabilization efficiency of Zn and Cd reduced by 23.50%–31.64%, and 7.10%–39.26%, respectively. Pyromorphite and amorphous lead phosphate formed with excess KH PO or K HPO addition, while K PO resulted in the formation of a hydroxypyromorphite precipitate. Amorphous Zn and Cd phosphates and hydroxides were the primary products. The immobilization rate of Zn and Cd depends on pH, and increased significantly in response to the excess phosphate application. This approach provides insight into phosphate-induced differences in stabilization efficiency in soils contaminated with multiple metals, which is of theoretical and engineering significance.

关键词： Heavy metals     Metal-contaminated soil     Phosphate     Competitive stabilization    

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Indicating landfill stabilization state by using leachate property from Laogang Refuse Landfill

LOU Ziyang,CHAI Xiaoli,ZHAO Youcai,SONG Yu,ZHU Nanwen,JIA Jinping

《环境科学与工程前沿（英文）》 2014年 第8卷 第3期   页码 405-410 doi: 10.1007/s11783-013-0565-5

摘要： Variation and evolution process of leachate can be applied as a reference for landfill stabilization phase. In this work, leachates with different ages were collected from Laogang Refuse Landfill, and characterized with 14 key parameters. Simultaneously, principal component analysis (PCA) was applied to develop a synthetic parameter-F based on these 14 parameters, and a logarithm equation was simulated for the landfill stabilization process finally. It was predicted that leachates would meet Class I and Class II in standard for pollution control on the landfill site of municipal solid waste (GB 16889-1997) after 32 years and 22 years disposal under the natural attenuation in the humid and warm southern areas of China, respectively. The predication of landfill state would be more accurate and useful according to the synthetic parameter of leachate from a working landfill.

关键词： landfill stabilization     leachate evolution     principal component analysis    

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Effects of sepiolite on stabilization remediation of heavy metal-contaminated soil and its ecological

Yuebing SUN,Dan ZHAO,Yingming XU,Lin WANG,Xuefeng LIANG,Yue SHEN

《环境科学与工程前沿（英文）》 2016年 第10卷 第1期   页码 85-92 doi: 10.1007/s11783-014-0689-2

摘要： Stabilization in the remediation of heavy metal contaminated soils has been gaining prominence because of its cost-effectiveness and rapid implementation. In this study, microbial properties such as microbial community and enzyme activities, chemical properties such as soil pH and metal fraction, and heavy metal accumulation in spinach ( ) were considered in assessing stabilization remediation effectiveness using sepiolite. Results showed that soil pH values increased with rising sepiolite concentration. Sequential extraction results indicated that the addition of sepiolite converted significant amounts of exchangeable fraction of Cd and Pb into residual form. Treatments of sepiolite were observed to reduce Cd and Pb translocation from the soil to the roots and shoots of spinach. Concentrations of Cd and Pb exhibited 12.6%–51.0% and 11.5%–46.0% reduction for the roots, respectively, and 0.9%–46.2% and 43.0%–65.8% reduction for the shoots, respectively, compared with the control group. Increase in fungi and actinomycete counts, as well as in catalase activities, indicated that soil metabolic recovery occurred after sepiolite treatments.

关键词： stabilization remediation     heavy metals     sepiolite     soil quality     spinach (Spinacia oleracea)    

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An integrated method for the rapid dewatering and solidification/stabilization of dredged contaminated

Hefu Pu, Aamir Khan Mastoi, Xunlong Chen, Dingbao Song, Jinwei Qiu, Peng Yang

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1359-1

摘要： Abstract • An integrated method, called PHDVPSS, was proposed for treating DCS. • The PHDVPSS method showed superior performance compared to conventional method. • Using the method, water content (%) of DCS decreased from 300 to<150 in 3 days. • The 56-day UCS from this method is 12‒17 times higher than conventional method. • Relative to PC, GGBS-MgO binder yielded greater reduction in the leachability. To more efficiently treat the dredged contaminated sediment (DCS) with a high water content, this study proposes an integrated method (called PHDVPSS) that uses the solidifying/stabilizing (S/S) agents and prefabricated horizontal drain (PHD) assisted by vacuum pressure (VP). Using this method, dewatering and solidification/stabilization can be carried out simultaneously such that the treatment time can be significantly shortened and the treatment efficacy can be significantly improved. A series of model tests was conducted to investigate the effectiveness of the proposed method. Experimental results indicated that the proposed PHDVPSS method showed superior performance compared to the conventional S/S method that uses Portland cement (PC) directly without prior dewatering. The 56-day unconfined compressive strength of DCS treated by the proposed method with GGBS-MgO as the binder is 12‒17 times higher than that by the conventional S/S method. DCS treated by the PHDVPSS method exhibited continuous decrease in leaching concentration of Zn with increasing curing age. The reduction of Zn leachability is more obvious when using GGBS-MgO as the binder than when using PC, because GGBS-MgO increased the residual fraction and decreased the acid soluble fraction of Zn. The microstructure analysis reveals the formation of hydrotalcite in GGBS-MgO binder, which resulted in higher mechanical strength and higher Zn stabilization efficiency.

关键词： Dredged contaminated sediment     Dewatering     Solidification/stabilization     Vacuum preloading     Prefabricated horizontal drain     Heavy metal    

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Stabilization treatment of contaminated soil: a field-scale application in Shanghai, China

Changbo ZHANG, Qishi LUO, Chunnu GENG, Zhongyuan LI

《环境科学与工程前沿（英文）》 2010年 第4卷 第4期   页码 395-404 doi: 10.1007/s11783-010-0271-5

摘要： Stabilization is one of the best demonstrated available technologies for treating toxic pollutants in soils and has been used worldwide but is rarely used for treatment of contaminated sites in China despite many bench-scale studies. Here, a field-scale application of stabilization treatment in Shanghai, China was summarized to demonstrate the whole engineering process and the key technical issues regarding stabilization of contaminated soil. A site contaminated with arsenic (As) and polycyclic aromatic hydrocarbons (PAHs), formerly used as a lighting plant in Shanghai, was chosen as the demonstration site. Stabilizing measures were taken to treat the contaminated soil to reuse the site for residential purposes. The whole engineering remediation process consisted of phase I environmental site assessment (ESA) and phase II ESA, quantitative human health risk assessment, remediation alternatives evaluation, bench-scale testing, remedial design, engineering implementation, and post-remediation assessment. A third party conducted evaluation monitoring indicated desirable results were achieved via the stabilization treatment. In addition, some technical obstacles related to soil stabilization treatment were discussed, including soil quality evaluation, stabilization effectiveness validation, and soil reuse assessment.

关键词： stabilization     contaminated soil     field-scale demonstration     technical obstacles    

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Stabilization of hexavalent chromium with pretreatment and high temperature sintering in highly contaminated

Haiyan Mou, Wenchao Liu, Lili Zhao, Wenqing Chen, Tianqi Ao

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1353-7

摘要： Abstract • Separate reduction and sintering cannot be effective for Cr stabilization. • Combined treatment of reduction and sintering is effective for Cr stabilization. • Almost all the Cr in the reduced soil is residual form after sintering at 1000°C. This study explored the effectiveness and mechanisms of high temperature sintering following pre-reduction with ferric sulfate (FeSO4), sodium sulfide (Na2S), or citric acid (C6H8O7) in stabilizing hexavalent chromium (Cr(VI)) in highly contaminated soil. The soil samples had an initial total Cr leaching of 1768.83 mg/L, and Cr(VI) leaching of 1745.13 mg/L. When FeSO4 or C6H8O7 reduction was followed by sintering at 1000°C, the Cr leaching was reduced enough to meet the Safety Landfill Standards regarding general industrial solid waste. This combined treatment greatly improved the stabilization efficiency of chromium because the reduction of Cr(VI) into Cr(III) decreased the mobility of chromium and made it more easily encapsulated in minerals during sintering. SEM, XRD, TG-DSC, and speciation analysis indicated that when the sintering temperature reached 1000°C, almost all the chromium in soils that had the pre-reduction treatment was transformed into the residual form. At 1000°C, the soil melted and promoted the mineralization of Cr and the formation of new Cr-containing compounds, which significantly decreased subsequent leaching of chromium from the soil. However, without reduction treatment, chromium continued to leach from the soil even after being sintered at 1000°C, possibly because the soil did not fully fuse and because Cr(VI) does not bind with soil as easily as Cr(III).

关键词： Chromium     Heavy contaminated soil     Reduction     Sintering     Stabilization     Speciation    

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Stabilization-based soil remediation should consider long-term challenges

Zhengtao Shen, Zhen Li, Daniel S. Alessi

《环境科学与工程前沿（英文）》 2018年 第12卷 第2期 doi: 10.1007/s11783-018-1028-9

摘要： Soil remediation is of increasing importance globally, especially in developing countries. Among available remediation options, stabilization, which aims to immobilize contaminants within soil, has considerable advantages, including that it is cost-effective, versatile, sustainable, rapid, and often results in less secondary pollution. However, there are emerging challenges regarding the long-term performance of the technology, which may be affected by a range of environmental factors. These challenges stem from a research gap regarding the development of accurate, quantitative laboratory simulations of long-term conditions, whereby laboratory accelerated aging methods could be normalized to real field conditions. Therefore, field trials coupled with long-term monitoring are critical to further verify conditions under which stabilization is effective. Sustainability is also an important factor affecting the long-term stability of site remediation. It is hence important to consider these challenges to develop an optimized application of stabilization technology in soil remediation.

关键词： Stabilization     Soil remediation     Long-term     Trace metals    

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Leaching characteristics of heavy metals during cement stabilization of fly ash from municipal solid

LIANG Shunwen, JIANG Jianguo, ZHANG Yan, XU Xin

《环境科学与工程前沿（英文）》 2008年 第2卷 第3期   页码 358-363 doi: 10.1007/s11783-008-0060-6

摘要： The leaching characteristics of heavy metals in products of cement stabilization of fly ash from a municipal solid waste incinerator were investigated in this paper. The stabilization of heavy metals such as Cd, Pb, Cu, and Zn in fly ash from such incinerators was examined through the national standard method in China based on the following factors: additive quantity of cement and NaS, curing time, and pH of leaching liquor. The results showed that as more additives were used, less heavy metals were leached except for Pb, which is sensitive to pH of the leachate, and the worse effect was observed for Cd. The mass ratio of cement to fly ash = 10% is the most appropriate parameter according to the national standard method. When the hydration of cement was basically finished, stabilization of heavy metals did not vary after curing for 1 d. The mixtures of cement and fly ash had excellent adaptability to environmental pH. The pH of leachate was maintained at 7 when pH of leaching liquor varied from 3 to 11.

关键词： heavy     national standard     environmental     leachate     liquor    

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The stabilization effect of Al2O3 on unconventional Pb/SiO2 catalyst

《化学科学与工程前沿（英文）》 2023年 第17卷 第10期   页码 1423-1429 doi: 10.1007/s11705-023-2315-y

摘要： Similar to Sn, Pb located at the same group (IVA) in the periodic table of elements, can also catalyze propane dehydrogenation to propene, while a fast deactivation can be observed. To enhance the stability, the traditional carrier Al2O3 with a small amount, was introduced into Pb/SiO2 catalyst in this study. It has been proved that Al2O3 can inhibit the reduction of PbO, and weaken the agglomeration and loss of Pb species due to its enhanced interaction with Pb species. As a result, 3Al15Pb/SiO2 catalyst exhibits a much higher stability up to more than 150 h. In addition, a simple schematic diagram of the change of surface species on the catalyst surface after Al2O3 addition was also proposed.

关键词： Pb/SiO2     Al2O3     propane dehydrogenation     propene     stability    

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Impact of wind power generating system integration on frequency stabilization in multi-area power system

Y. K. BHATESHVAR,H. D. MATHUR,H. SIGUERDIDJANE

《能源前沿（英文）》 2015年 第9卷 第1期   页码 7-21 doi: 10.1007/s11708-014-0338-2

摘要： Among the available options for renewable energy integration in existing power system, wind power is being considered as one of the suited options for future electrical power generation. The major constraint of wind power generating system (WPGS) is that it does not provide inertial support because of power electronic converters between the grid and the WPGS to facilitate frequency stabilization. The proposed control strategy suggests a substantial contribution to system inertia in terms of short-term active power support in a two area restructured power system. The control scheme uses fuzzy logic based design and takes frequency deviation as input to provide quick active power support, which balances the drop in frequency and tie-line power during transient conditions. This paper presents a comprehensive study of the wind power impact with increasing wind power penetration on frequency stabilization in restructured power system scenario. Variation of load conditions are also analyzed in simulation studies for the same power system model with the proposed control scheme. Simulation results advocates the justification of control scheme over other schemes.

关键词： two area power system     automatic generation control     wind power generating system (WPGS)     deregulated environment     fuzzy logic controller (FLC)    

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标题 作者 时间 类型 操作

Cu/Cr co-stabilization mechanisms in a simulated AlO-FeO-CrO-CuO waste system

期刊论文

Microwave enhanced stabilization of copper in artificially contaminated soil

Hua ZHANG, Zhiliang ZHU, Noboru YOSHIKAWA

期刊论文

Cement-based solidification/stabilization of contaminated soils by nitrobenzene

Jianguo LIU, Xiaoqin NIE, Xianwei ZENG, Zhaoji SU

期刊论文

Analysis and stabilization control of a voltage source controlled wind farm under weak grid conditions

期刊论文

The use of fine portions from construction and demolition waste for expansive soil stabilization: A review

Mgboawaji Claude UJILE; Samuel Jonah ABBEY

期刊论文

Phosphate-induced differences in stabilization efficiency for soils contaminated with lead, zinc, and

Jie Ren, Zhuo Zhang, Mei Wang, Guanlin Guo, Ping Du, Fasheng Li

期刊论文

Indicating landfill stabilization state by using leachate property from Laogang Refuse Landfill

LOU Ziyang,CHAI Xiaoli,ZHAO Youcai,SONG Yu,ZHU Nanwen,JIA Jinping

期刊论文

Effects of sepiolite on stabilization remediation of heavy metal-contaminated soil and its ecological

Yuebing SUN,Dan ZHAO,Yingming XU,Lin WANG,Xuefeng LIANG,Yue SHEN

期刊论文

An integrated method for the rapid dewatering and solidification/stabilization of dredged contaminated

Hefu Pu, Aamir Khan Mastoi, Xunlong Chen, Dingbao Song, Jinwei Qiu, Peng Yang

期刊论文

Stabilization treatment of contaminated soil: a field-scale application in Shanghai, China

Changbo ZHANG, Qishi LUO, Chunnu GENG, Zhongyuan LI

期刊论文

Stabilization of hexavalent chromium with pretreatment and high temperature sintering in highly contaminated

Haiyan Mou, Wenchao Liu, Lili Zhao, Wenqing Chen, Tianqi Ao

期刊论文

Stabilization-based soil remediation should consider long-term challenges

Zhengtao Shen, Zhen Li, Daniel S. Alessi

期刊论文

Leaching characteristics of heavy metals during cement stabilization of fly ash from municipal solid

LIANG Shunwen, JIANG Jianguo, ZHANG Yan, XU Xin

期刊论文

The stabilization effect of Al2O3 on unconventional Pb/SiO2 catalyst

期刊论文

Impact of wind power generating system integration on frequency stabilization in multi-area power system

Y. K. BHATESHVAR,H. D. MATHUR,H. SIGUERDIDJANE

期刊论文