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Decomposition analysis applied to energy and emissions: A literature review

《工程管理前沿（英文）》   页码 625-639 doi: 10.1007/s42524-023-0270-4

摘要： Decomposition analysis has been widely used to assess the determinants of energy and CO2 emissions in academic research and policy studies. Both the methodology and application of decomposition analysis have been largely improved in the past decades. After more than 50 years’ developments, decomposition studies have become increasingly sophisticated and diversified, and tend to converge internally and integrate with other analytical approaches externally. A good understanding of the literature and state of the art is critical to identify knowledge gaps and formulate future research agenda. To this end, this study presents a literature survey for decomposition analysis applied to energy and emission issues, with a focus on the period of 2016–2021. A review for three individual decomposition techniques is first conducted, followed by a synthesis of emerging trends and features for the decomposition analysis literature as a whole. The findings are expected to direct future research in decomposition analysis.

关键词： index decomposition analysis     structural decomposition analysis     production decomposition analysis     energy     CO2 emissions    

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Catalytic decomposition of low level ozone with gold nanoparticles supported on activated carbon

Pengyi ZHANG , Bo ZHANG , Rui SHI ,

《环境科学与工程前沿（英文）》 2009年 第3卷 第3期   页码 281-288 doi: 10.1007/s11783-009-0032-5

摘要： Highly dispersed gold nanoparticles were supported on coal-based activated carbon (AC) by a sol immobilization method and were used to investigate their catalytic activity for low-level ozone decomposition at ambient temperature. Nitrogen adsorption-desorption, scanning electron microscope (SEM), and X-ray photoelectron spectroscopy (XPS) were used to characterize the catalysts before and after ozone decomposition. The results showed that the supported gold nanoparticles prepared with microwave heating were much smaller and more uniformly dispersed on the activated carbon than those prepared with traditional conduction heating, exhibiting higher catalytic activity for ozone decomposition. The pH values of gold precursor solution significantly influenced the catalytic activity of supported gold for ozone decomposition, and the best pH value was 8. In the case of space velocity of 120000h, inlet ozone concentration of 50mg/m, and relative humidity of 45%, the Au/AC catalyst maintained the ozone removal ratio at 90.7% after 2500min. After being used for ozone decomposition, the surface carbon of the catalyst was partly oxidized and the oxygen content increased accordingly, while its specific surface area and pore volume only decreased a little. Ozone was mainly catalytically decomposed by the gold nanoparticles supported on the activated carbon.

关键词： ozone decomposition     activated carbon     gold nanoparticles     catalysis     sodium citrate     microwave    

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Product decomposition strategy for optimization of supply chain planning

Braulio BRUNAUD, Maria Paz OCHOA, Ignacio E. GROSSMANN

《工程管理前沿（英文）》 2018年 第5卷 第4期   页码 466-478 doi: 10.15302/J-FEM-2018059

摘要：

Optimization of large-scale supply chain planning models requires the application of decomposition strategies to reduce the computational expense. Two major options are to use either spatial or temporal Lagrangean decomposition. In this paper, to further reduce the computational expense a novel decomposition scheme by products is presented. The decomposition is based on a reformulation of knapsack constraints in the problem. The new approach allows for simultaneous decomposition by products and by time periods, enabling the generation of a large number of subproblems, that can be solved by using parallel computing. The case study shows that the proposed product decomposition exhibits similar performance as the temporal decomposition, and that selecting different orders of products and aggregating the linking constraints can improve the efficiency of the algorithm.

关键词： supply chain planning     Lagrangean decomposition     mixed-integer programming    

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Variational mode decomposition based modal parameter identification in civil engineering

Mingjie ZHANG, Fuyou XU

《结构与土木工程前沿（英文）》 2019年 第13卷 第5期   页码 1082-1094 doi: 10.1007/s11709-019-0537-3

摘要： An out-put only modal parameter identification method based on variational mode decomposition (VMD) is developed for civil structure identifications. The recently developed VMD technique is utilized to decompose the free decay response (FDR) of a structure into to modal responses. A novel procedure is developed to calculate the instantaneous modal frequencies and instantaneous modal damping ratios. The proposed identification method can straightforwardly extract the mode shape vectors using the modal responses extracted from the FDRs at all available sensors on the structure. A series of numerical and experimental case studies are conducted to demonstrate the efficiency and highlight the superiority of the proposed method in modal parameter identification using both free vibration and ambient vibration data. The results of the present method are compared with those of the empirical mode decomposition-based method, and the superiorities of the present method are verified. The proposed method is proved to be efficient and accurate in modal parameter identification for both linear and nonlinear civil structures, including structures with closely spaced modes, sudden modal parameter variation, and amplitude-dependent modal parameters, etc.

关键词： modal parameter identification     variational mode decomposition     civil structure     nonlinear system     closely spaced modes    

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Mechanism of methanol decomposition on the Pd/WC(0001) surface unveiled by first-principles calculations

Jinhua Zhang, Yuanbin She

《化学科学与工程前沿（英文）》 2020年 第14卷 第6期   页码 1052-1064 doi: 10.1007/s11705-019-1908-y

摘要： In this study, the decomposition of methanol into the CO and H species on the Pd/tungsten carbide (WC)(0001) surface is systematically investigated using periodic density functional theory (DFT) calculations. The possible reaction pathways and intermediates are determined. The results reveal that saturated molecules, i.e., methanol and formaldehyde, adsorb weakly on the Pd/WC(0001) surface. Both CO and H prefer three-fold sites, with adsorption energies of ‒1.51 and ‒2.67 eV, respectively. On the other hand, CH O stably binds at three-fold and bridge sites, with an adsorption energy of ‒2.58 eV. However, most of the other intermediates tend to adsorb to the surface with the carbon and oxygen atoms in their sp and hydroxyl-like configurations, respectively. Hence, the C atom of CH OH preferentially attaches to the top sites, CHOH and CH O adsorb at the bridge sites, while COH and CHO occupy the three-fold sites. The DFT calculations indicate that the rupture of the initial C–H bond promotes the decomposition of CH OH and CH OH, whereas in the case of CHOH, O–H bond scission is favored over the C–H bond rupture. Thus, the most probable methanol decomposition pathway on the Pd/WC(0001) surface is CH OH → CH OH → -CHOH → CHO → CO. The present study demonstrates that the synergistic effect of WC (as carrier) and Pd (as catalyst) alters the CH OH decomposition pathway and reduces the noble metal utilization.

关键词： density functional theory     methanol     direct methanol fuel cells     WC(0001)-supported Pd monolayer     decomposition mechanism    

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Dielectric barrier micro-plasma reactor with segmented outer electrode for decomposition of pure CO

Baowei Wang, Xiaoxi Wang, Bo Zhang

《化学科学与工程前沿（英文）》 2021年 第15卷 第3期   页码 687-697 doi: 10.1007/s11705-020-1974-1

摘要： Four coaxial cylinder dielectric barrier discharge micro-plasma reactors were designed for the non-catalytic decomposition of pure CO into CO and O at low temperature and ambient pressure. The influence of segmented outer electrodes on the electrical characteristics and the reaction performance was investigated. Experimental results indicated that the introduction of segmented outer electrodes can significantly promote the decomposition of CO . Encouragingly, the highest conversion of 13.1% was obtained at an applied voltage of 18 kV, which was a substantial increase of 39.4% compared to the traditional device. Compared with other types of dielectric barrier discharge plasma reactors, the proposed segmented outer electrode micro-plasma reactor can give a higher CO conversion and acceptable energy efficiency. The increase in conversion can be attributed mainly to the enhanced corona discharge caused by the fringe effect at electrode edges, the increase in energy density and the increase in the number of micro-discharges. In addition, detailed electrical characterization was performed to reveal some trends in the electrical behavior of proposed reactors.

关键词： CO2 decomposition     dielectric barrier discharge     segmented outer electrodes     electrical analysis     reactor design    

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Thermal decomposition mechanism of ammonium sulfate catalyzed by ferric oxide

Xingfu SONG, Jingcai ZHAO, Yunzhao LI, Ze SUN, Jianguo YU

《化学科学与工程前沿（英文）》 2013年 第7卷 第2期   页码 210-217 doi: 10.1007/s11705-013-1320-y

摘要： The decomposition mechanism of ammonium sulfate catalyzed by ferric oxide was investigated in this paper. The decomposition kinetics parameters were determined via a global optimization of the Kissinger iterative method using the non-isothermal thermogravimetric analysis data. The products and intermediates were synchronously characterized by X-ray diffraction and mass spectrometry. The obtained results indicate that the decomposition process of ammonium sulfate catalyzed by ferric oxide can be divided into four stages of which the activation energies are 123.64, 126.58, 178.77 and 216.99 kJ·mol respectively. The decomposition mechanisms at the first and the fourth stage both belong to Mample power theorem, the second stage belongs to Avrami-Erofeev equation and the third belongs to contracting sphere (volume) equation. The corresponding pre-exponential factors ( ) are calculated simultaneously.

关键词： ammonium sulfate     decomposition kinetics     ferric oxide     thermogravimetric analysis    

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Effect of alkyl nitrite decomposition on catalytic performance of CO coupling reaction over supported

Zhenhua LI, Weihan WANG, Dongxue YIN, Jing LV, Xinbin MA

《化学科学与工程前沿（英文）》 2012年 第6卷 第4期   页码 410-414 doi: 10.1007/s11705-012-1213-5

摘要： The syntheses of dimethyl oxalate (DMO) and diethyl oxalate (DEO) by CO coupling reaction in gaseous phase were investigated in a fixed bed reactor over Pd-Fe/Al O catalyst. The catalytic performance was characterized by CO conversion, space-time yield (STY) and selectivity of DMO (or DEO). The results showed that over Pd-Fe/Al O catalyst, the STY of DMO was higher than that of DEO under the same reaction conditions. The optimum reaction temperatures for synthesizing DMO and DEO were 403 K and 393 K, respectively, at the molar ratio 1 ∶ 1 of alkyl nitrite to CO. The difference in synthesizing DMO and DEO on the same catalyst was attributed to the decomposition performances of methyl nitrite (MN) and ethyl nitrite (EN), as density functional theory (DFT) calculation showed that EN decomposed more easily than MN.

关键词： palladium     CO coupling     dialkyl oxalate     alkyl nitrite     decomposition    

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Photo-induced surface frustrated Lewis pairs for promoted photocatalytic decomposition of perfluorooctanoic

《环境科学与工程前沿（英文）》 2023年 第17卷 第1期 doi: 10.1007/s11783-023-1603-6

摘要：

● Terminal carboxylate group activation is PFOA degradation’s rate-limiting step.

关键词： Heterogeneous photocatalysis     Surface frustrated Lewis pairs     Perfluorooctanoic acid     Defluorination efficiency     Environmental remediation    

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Thermal decomposition of poly(ethylene terephthalate)/mesoporous molecular sieve composites

RUN Mingtao, ZHANG Dayu, WU Sizhu, WU Gang

《化学科学与工程前沿（英文）》 2007年 第1卷 第1期   页码 50-54 doi: 10.1007/s11705-007-0010-z

摘要： The nonisothermal and isothermal degradation processes of poly (ethylene terephthalate)/mesoporous molecular sieve (PET/MMS) composites synthesized by in-situ polymerization were studied by using thermogravimetric analysis in nitrogen. The nonisothermal degradation of the composite is found to be the first-order reaction. An iso-conversional procedure developed by Ozawa is used to calculate the apparent activation energy (), which is an average value of about 260 kJ/mol with the weight conversion from 0% to 30%, and is higher than that of neat PET. Isothermal degradation results are confirmed with the nonisothermal process, in which PET/MMS showed higher thermal stability than neat PET. The polymer in mesoporous channels has more stability due to the protection of the inorganic pore-wall. These results indicate that mesoporous MMS in PET/MMS composites improve the stability of the polymer.

关键词： polymerization     isothermal degradation     conversion     nonisothermal degradation     activation    

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Mass loss and nutrient dynamics during litter decomposition in response to warming and nitrogen addition

Haiyan REN, Jie QIN, Baolong YAN, Alata, Baoyinhexige, Guodong HAN

《农业科学与工程前沿（英文）》 2018年 第5卷 第1期   页码 64-70 doi: 10.15302/J-FASE-2017194

摘要： Plant litter decomposition has been studied extensively in the context of both warming and increased atmospheric nitrogen deposition. However, the temporal patterns of mass loss and nutrient release in response to warming and nitrogen addition remain unclear. A 2-year decomposition experiment aimed to examine the effects of warming and nitrogen addition on decomposition rate, and nitrogen and phosphorus dynamics. The effects of warming and nitrogen addition on decomposition of litter of , a dominant species in a desert steppe of northern China, were studied. Warming and nitrogen addition significantly enhanced litter mass loss by 10% and 16%, respectively, and moreover promoted nitrogen and phosphorus release from the litter in the first year of decomposition, followed by an immobilization period. The interactive effects of warming and nitrogen addition on mass loss, nitrogen and phosphorus concentrations of litter were also found during the decomposition. This study indicates that warming and nitrogen addition increased litter mass loss through altering litter quality. These findings highlight that interactions between climate change and other global change factors could be highly important in driving decomposition responses.

关键词： climate warming     grassland     litter decomposition     nitrogen deposition     nutrient release    

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A decomposition approach to the design of a multiferroic memory bit

Ruben ACEVEDO, Cheng-Yen LIANG, Gregory P. CARMAN, Abdon E. SEPULVEDA

《机械工程前沿（英文）》 2017年 第12卷 第2期   页码 215-223 doi: 10.1007/s11465-017-0446-x

摘要：

The objective of this paper is to present a methodology for the design of a memory bit to minimize the energy required to write data at the bit level. By straining a ferromagnetic nickel nano-dot by means of a piezoelectric substrate, its magnetization vector rotates between two stable states defined as a 1 and 0 for digital memory. The memory bit geometry, actuation mechanism and voltage control law were used as design variables. The approach used was to decompose the overall design process into simpler sub-problems whose structure can be exploited for a more efficient solution. This method minimizes the number of fully dynamic coupled finite element analyses required to converge to a near optimal design, thus decreasing the computational time for the design process. An in-plane sample design problem is presented to illustrate the advantages and flexibility of the procedure.

关键词： multiferroics     nano memory     piezoelectric     optimization    

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A building unit decomposition model for energy leakage by infrared thermography image analysis

Yan SU, Fangjun HONG, Lianjie SHU

《能源前沿（英文）》 2020年 第14卷 第4期   页码 901-921 doi: 10.1007/s11708-020-0679-y

摘要： A quantitative energy leakage model was developed based on the thermography image data measured for both external and internal building surfaces. The infrared thermography images of both surfaces of doors, windows, and walls of an office building in the Hengqin Campus of University of Macao were taken at various times in a day for four seasons. The transient heat flux for sample units were obtained based on measurements of the seasonal transient local temperature differences and calculations of the effective thermal conductivity from the multiple-layer porous medium conduction model. Effects of construction unit types, orientations, and seasons were quantitatively investigated with unit transient orientation index factors. The corresponding electric energy consumption was calculated based on the air conditioning system coefficient of performance of heat pump and refrigerator cycles for different seasons. The model was validated by comparing to the electric meter records of energy consumption of the air conditioning system. The uncertainties of the predicted total building energy leakage are about 14.7%, 12.8%, 12.4%, and 15.8% for the four seasons, respectively. The differences between the predicted electric consumption and meter values are less than 13.4% and 5.4% for summer and winter, respectively. The typical daily thermal energy leakage value in winter is the highest among the four seasons. However, the daily electric energy consumption by the air conditioning system in summer and autumn is higher than that in winter. The present decomposition model for energy leakage is expected to provide a practical tool for quantitative analysis of energy leakage of buildings.

关键词： heat conductivity     heat coefficient     heat &fllig     ux     infrared thermography     thermal image    

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Weak characteristic information extraction from early fault of wind turbine generator gearbox

Xiaoli XU, Xiuli LIU

《机械工程前沿（英文）》 2017年 第12卷 第3期   页码 357-366 doi: 10.1007/s11465-017-0423-4

摘要：

Given the weak early degradation characteristic information during early fault evolution in gearbox of wind turbine generator, traditional singular value decomposition (SVD)-based denoising may result in loss of useful information. A weak characteristic information extraction based on µ-SVD and local mean decomposition (LMD) is developed to address this problem. The basic principle of the method is as follows: Determine the denoising order based on cumulative contribution rate, perform signal reconstruction, extract and subject the noisy part of signal to LMD and µ-SVD denoising, and obtain denoised signal through superposition. Experimental results show that this method can significantly weaken signal noise, effectively extract the weak characteristic information of early fault, and facilitate the early fault warning and dynamic predictive maintenance.

关键词： wind turbine generator gearbox     µ-singular value decomposition     local mean decomposition     weak characteristic information extraction     early fault warning    

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Additives effects on crystallization and morphology in a novel caustic aluminate solution decomposition

Ying ZHANG, Shili ZHENG, Yifei ZHANG, Hongbin XU, Yi ZHANG

《化学科学与工程前沿（英文）》 2009年 第3卷 第1期   页码 88-92 doi: 10.1007/s11705-009-0133-5

摘要： A novel process of caustic aluminate solution decomposition by alcohol medium was developed by the Institute of Process Engineering, Chinese Academy of Sciences in order to solve the problem of low decomposition ratio in the traditional Bayer seeded hydrolysis process. In this research, effects of additives on the crystallization ratio, secondary particle size and morphology of aluminum hydroxide in the new process were studied to obtain high-quality products. On the basis of primary selection of additives, an orthogonal design L9(3 ) was used as a chemometric method to investigate the effects of additives. The studied parameters include the reaction style, quantity of additives, caustic soda concentration, as well as the combination manner. The crystallization ratios of sodium aluminate solution and crystal size of aluminum hydroxide, determined by ICP-OES, SEM and MLPSA (Malvern Laser Particle Size Analyzer), were used to evaluate the effects of the additives. The results showed that different combination manners could promote agglomeration or dispersion. An additive composed by Tween 80 and PEG 200 could promote agglomeration, while a spot of PEG species had a relatively strong dispersion effect. However, the additives had little effects on the crystallization ratios. According to the Raman spectra result, the added alcohol medium might serve as a kind of solvent.

关键词： additive     crystallization     morphology     caustic aluminate solution     aluminium hydroxide    

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标题 作者 时间 类型 操作

Decomposition analysis applied to energy and emissions: A literature review

期刊论文

Catalytic decomposition of low level ozone with gold nanoparticles supported on activated carbon

Pengyi ZHANG , Bo ZHANG , Rui SHI ,

期刊论文

Product decomposition strategy for optimization of supply chain planning

Braulio BRUNAUD, Maria Paz OCHOA, Ignacio E. GROSSMANN

期刊论文

Variational mode decomposition based modal parameter identification in civil engineering

Mingjie ZHANG, Fuyou XU

期刊论文

Mechanism of methanol decomposition on the Pd/WC(0001) surface unveiled by first-principles calculations

Jinhua Zhang, Yuanbin She

期刊论文

Dielectric barrier micro-plasma reactor with segmented outer electrode for decomposition of pure CO

Baowei Wang, Xiaoxi Wang, Bo Zhang

期刊论文

Thermal decomposition mechanism of ammonium sulfate catalyzed by ferric oxide

Xingfu SONG, Jingcai ZHAO, Yunzhao LI, Ze SUN, Jianguo YU

期刊论文

Effect of alkyl nitrite decomposition on catalytic performance of CO coupling reaction over supported

Zhenhua LI, Weihan WANG, Dongxue YIN, Jing LV, Xinbin MA

期刊论文

Photo-induced surface frustrated Lewis pairs for promoted photocatalytic decomposition of perfluorooctanoic

期刊论文

Thermal decomposition of poly(ethylene terephthalate)/mesoporous molecular sieve composites

RUN Mingtao, ZHANG Dayu, WU Sizhu, WU Gang

期刊论文

Mass loss and nutrient dynamics during litter decomposition in response to warming and nitrogen addition

Haiyan REN, Jie QIN, Baolong YAN, Alata, Baoyinhexige, Guodong HAN

期刊论文

A decomposition approach to the design of a multiferroic memory bit

Ruben ACEVEDO, Cheng-Yen LIANG, Gregory P. CARMAN, Abdon E. SEPULVEDA

期刊论文

A building unit decomposition model for energy leakage by infrared thermography image analysis

Yan SU, Fangjun HONG, Lianjie SHU

期刊论文

Weak characteristic information extraction from early fault of wind turbine generator gearbox

Xiaoli XU, Xiuli LIU

期刊论文

Additives effects on crystallization and morphology in a novel caustic aluminate solution decomposition

Ying ZHANG, Shili ZHENG, Yifei ZHANG, Hongbin XU, Yi ZHANG

期刊论文