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Mechanisms for simultaneous ozonation of sulfamethoxazole and natural organic matters in secondary effluent

《环境科学与工程前沿(英文)》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1368-0

摘要:

• SMX was mainly degraded by hydrolysis, isoxazole oxidation and double-bond addition.

关键词: Sulfamethoxazole     Ozonation     Natural organic matters     Secondary effluent     Degradation mechanism    

Dissolved methane in anaerobic effluent: Emission or recovery?

《环境科学与工程前沿(英文)》 2022年 第16卷 第4期 doi: 10.1007/s11783-022-1537-4

摘要: Various anaerobic processes have been explored for the energy-efficient treatment of municipal wastewater. However, dissolved methane in anaerobic effluent appears to be a barrier towards the energy and carbon neutrality of wastewater treatment. Although several dissolved methane recovery methods have been developed, their engineering feasibility and economic viability have not yet been assessed in a holistic manner. In this perspective, we thus intend to offer additional insights into the cost-benefit of dissolved methane recovery against its emission.

关键词: Anaerobic treatment     Municipal wastewater     Dissolved methane     Methane recovery     Carbon emission    

Optimization of thermophilic anaerobic-aerobic treatment system for Palm Oil Mill Effluent (POME)

Yijing CHAN,Meifong CHONG,Chunglim LAW

《环境科学与工程前沿(英文)》 2015年 第9卷 第2期   页码 334-351 doi: 10.1007/s11783-014-0626-4

摘要: Optimization of an integrated anaerobic-aerobic bioreactor (IAAB) treatment system for the reduction of organic matter (Chemical Oxygen Demand (COD), Biochemical Oxygen Demand (BOD) and Total Suspended Solids (TSS) concentrations) in Palm Oil Mill Effluent (POME) to legal standards with high methane yield was performed for the first time under thermophilic condition (50°C–55°C) by using response surface methodology (RSM). The experiments were conducted based on a central composite rotatable design (CCRD) with three independent operating variables, organic loading rates in anaerobic compartment (OLR ) and mixed liquor volatile suspended solids (MLVSS) concentration in anaerobic (MLVSS ) and aerobic compartments (MLVSS ). The optimum conditions for the POME treatment were determined as OLR of 15.6 g COD·L ·d , MLVSS of 43100 mg·L , and MLVSS of 18600 mg·L , where high aerobic COD, BOD and TSS removal efficiencies of 96.3%, 97.9%, and 98.5% were achieved with treated BOD of 56 mg·L and TSS of 28 mg·L meeting the discharge standard. This optimization study successfully achieved a reduction of 42% in the BOD concentrations of the final treated effluent at a 48% higher OLR as compared to the previous works. Besides, thermophilic IAAB system scores better feasibility and higher effectiveness as compared to the optimized mesophilic system. This is due to its higher ability to handle high OLR with higher overall treatment efficiencies (more than 99.6%), methane yield (0.31 L CH ·g COD ) and purity of methane (67.5%). Hence, these advantages ascertain the applicability of thermophilic IAAB in the POME treatment or even in other high-strength wastewaters treatment.

关键词: palm oil mill effluent (POME)     anaerobic     aerobic     thermophilic     biogas     optimization    

Controlling various contaminants in wastewater effluent through membranes and engineered wetland

Sarper SARP, Sungyun LEE, Noeon PARK, Nguyen Thi HANH, Jaeweon CHO

《环境科学与工程前沿(英文)》 2009年 第3卷 第1期   页码 98-105 doi: 10.1007/s11783-009-0006-7

摘要: For effective wastewater reclamation and water recovery, the treatment of natural and effluent organic matters (NOM and EfOM), toxic anions, and micropollutants was considered in this work. Two different NOM (humic acid of the Suwannee River, and NOM of US and Youngsan River, Korea), and one EfOM from the Damyang wastewater treatment plant, Korea, were selected for investigating the removal efficiencies of tight nanofiltration (NF) and ultrafiltration (UF) membranes with different properties. Nitrate, bromate, and perchlorate were selected as target toxic anions due to their well known high toxicities. Tri-(2-chloroethyl)-phosphate (TCEP), oxybenzone, and caffeine, due to their different and p values, were selected as target micropollutants. As expected, the NF membranes provided high removal efficiencies in terms of all the tested contaminants, and the UF membrane provided fairly high removal efficiencies for anions (except for nitrate) and the relatively hydrophobic micropollutant, oxybenzon

关键词: wastewater reclamation     natural organic matter (NOM)     effluent organic matter (EfOM)     membranes     wetlands    

Characterization of the dissolved organic matter in sewage effluent of sequence batch reactor: the impact

Jin GUO, Feng SHENG, Jianhua GUO, Xiong YANG, Mintao MA, Yongzhen PENG

《环境科学与工程前沿(英文)》 2012年 第6卷 第2期   页码 280-287 doi: 10.1007/s11783-011-0336-0

摘要: Dissolved organic matter (DOM) transformation in sequence batch reactor (SBR) fed with carbon sources of different biodegradability was investigated. During the biologic degradation process, the low molecular weight (MW) fraction (<1 kDa) gradually decreased, while the refractory compounds with higher aromaticity were aggregated. Size exclusion chromatography (SEC) and fluorescence of excitation emission matrices (EEM) demonstrated that more biopolymers (polysaccharides or proteins) and humic-like substances were presented in the extracellular polymeric substance (EPS) extracted from the SBR fed with sodium acetate or glucose, while the EPS from SBR fed with slowly biodegradable dissolved organic carbon (DOC) substrate-starch had relatively less biopolymers. Comparing the EfOM in sewage effluent of three SBRs, the effluent from SBR fed with starch is more aromatic. Organic carbon with MW>1 kDa as well as the hydrophobic fraction in DOM gradually increased with the carbon sources changing from sodium acetate to glucose and starch. The DOC fractionation and the EEM all demonstrated that EfOM from the effluent of the SBR fed with starch contained more fulvic acid-like substances comparing with the SBR fed with sodium acetate and glucose.

关键词: effluent organic matter (EfOM)     extracellular polymeric substance (EPS)     molecular weight distribution (MWD)     hydrophobic     hydrophilic     excitation emission matrices (EEM)    

Recovering humic substances from the dewatering effluent of thermally treated sludge and its performance

Yuning YANG,Huan LI

《环境科学与工程前沿(英文)》 2016年 第10卷 第3期   页码 578-584 doi: 10.1007/s11783-015-0827-5

摘要: The biologic treatment of the dewatering effluent from thermally treated sludge is difficult due to the high concentration of refractory humic substances. On the other hand, humic substances are an important source of organic fertilizer. In this study, a novel process using ferric coagulant was developed to recover humic substances from dewatering effluent for use as an organic fertilizer. When ferric coagulant was applied to raw dewatering effluent, up to 70% of humic substances were enmeshed by hydrolyzed ferric ions at an optimum pH of 4.5. The proper mass ratio of iron ions to humic substances was 0.6. In the recovered material, humic substances accounted for 24.2% of the total dry solids, and the amount of phosphorus (equivalent phosphorus pentoxide) was 6.2%. Heavy metals and other components all met the legal requirements for organic fertilizer. When the recovered material was applied to soybeans, the germination and growth of the seeds was significantly improved.

关键词: sewage sludge     humic substances     recovery     phosphorus     fertilizer    

Simultaneous enhanced ammonia and nitrate removal from secondary effluent in constructed wetlands using

《环境科学与工程前沿(英文)》 2023年 第18卷 第4期 doi: 10.1007/s11783-024-1807-4

摘要:

● MnO2/PCL composite material (MPCM) enhances ammonia and nitrate removal in CWs.

关键词: Constructed wetland     Nitrogen removal     Manganese redox     Polycaprolactone     Nitrous oxide    

Unintended nutrient imbalance induced by wastewater effluent inputs to receiving water and its ecological

《环境科学与工程前沿(英文)》 2022年 第16卷 第11期 doi: 10.1007/s11783-022-1584-x

摘要: Eutrophication is the most widespread water quality issue globally. To date, most efforts to control eutrophication have focused on reductions of external nutrient inputs, yet importance of nutrient stoichiometry and subsequent shift in plankton composition in aquatic ecosystem has been largely neglected. To address eutrophication, improved sanitation is one of the United Nations Sustainable Development Goals, spurring the constructions of wastewater treatment facilities that have improved water quality in many lakes and rivers. However, control measures are often targeted at and effective in removing a single nutrient from sewage and thus are less effective in removing the others, resulting in the changes of nutrient stoichiometry. In general, more effective phosphorus removal relative to nitrogen has occurred in wastewater treatment leading to substantial increases in N/P ratios in effluent relative to the influent. Unfortunately, high N/P ratios in receiving waters can impose negative influences on ecosystems. Thus, long-term strategies for domestic wastewater management should not merely focus on the total reduction of nutrient discharge but also consider their stoichiometric balances in receiving waters.

关键词: Nutrient stoichiometry     Wastewater treatment     Ecosystem functioning     Water quality management    

Effect of effluent organic matter on ozonation of bezafibrate

Huan HE,Qian SUI,Shuguang LU,Wentao ZHAO,Zhaofu QIU,Gang YU

《环境科学与工程前沿(英文)》 2015年 第9卷 第6期   页码 962-969 doi: 10.1007/s11783-015-0772-3

摘要: The influence of three effluent organic matter (EfOM) model compounds, humic acid (HA), bovine serum albumin (BSA), and sodium alginate (AGS), on the ozonation of bezafibrate (BF), a typical pharmaceutical and personal care product (PPCP), was investigated. The results show that ozonation efficiently removed BF from aqueous solution with removal efficiencies>95% within 8 min for all conditions. The reaction rate of BF decreased with increasing model compounds concentrations and the influence was more pronounced for HA and BSA, while less pronounced for AGS. Although BF concentration was significantly reduced, the degree of mineralization achieved was only approximately 11%. The addition of HA and BSA improved the mineralization of the solution, while the influence of AGS was minor. The acute toxicity of BF solution during ozonation was determined using the Luminescent bacteria test, and the toxicity exhibited an initial increase and a successive reduction. An overall decreased acute toxicity was observed with an increase of HA. The presence of BSA increased the formation rate of toxicity intermediates and resulted in inhibition peak forward.

关键词: ozonation     bezafibrate     acute toxicity     humic acid     bovine serum albumin     sodium alginate    

Removal efficiencies of natural and synthetic progesterones in hospital wastewater treated by different disinfection processes

《环境科学与工程前沿(英文)》 2022年 第16卷 第10期 doi: 10.1007/s11783-022-1558-z

摘要:

● The concentrations of 61 progesterones in HWW, PFTE, SBTE were evaluated.

关键词: Progesterones     Hospital wastewater     Primary filtration treatment effluent     Secondary biological treatment effluent     Disinfection process    

Identifying human-induced influence on microbial community: A comparative study in the effluent-receiving

Yuhan Zheng, Zhiguo Su, Tianjiao Dai, Feifei Li, Bei Huang, Qinglin Mu, Chuanping Feng, Donghui Wen

《环境科学与工程前沿(英文)》 2019年 第13卷 第6期 doi: 10.1007/s11783-019-1174-8

摘要: Microbial compositions showed high differences in two study areas. COD was the key anthropogenic indicator in the coastal wastewater disposal area. Distinctive microbes capable of degrading toxic pollutants were screened. Microbial communities in effluent-receiving areas followed “niche theory”. Microbial community structure is affected by both natural processes and human activities. In coastal area, anthropegenetic activity can usually lead to the discharge of the effluent from wastewater treatment plant (WWTP) to sea, and thus the water quality chronically turns worse and marine ecosystem becomes unhealthy. Microorganisms play key roles in pollutants degradation and ecological restoration; however, there are few studies about how the WWTP effluent disposal influences coastal microbial communities. In this study, sediment samples were collected from two WWTP effluent-receiving areas (abbreviated as JX and SY) in Hangzhou Bay. First, based on the high-throughput sequencing of 16S rRNA gene, microbial community structure was analyzed. Secondly, several statistical analyses were conducted to reveal the microbial community characteristics in response to the effluent disposal. Using PCoA, the significant difference of in microbial community structure was determined between JX and SY; using RDA, water COD and temperature, and sediment available phosphate and ammonia nitrogen were identified as the key environmental factors for the community difference; using LDA effect size analysis, the most distinctive microbes were found and their correlations with environmental factors were investigated; and according to detrended beta-nearest-taxon-index, the sediment microbial communities were found to follow “niche theory”. An interesting and important finding was that in SY that received more and toxic COD, many distinctive microbes were related to the groups that were capable of degrading toxic organic pollutants. This study provides a clear illustration of eco-environmental deterioration under the long-term human pressure from the view of microbial ecology.

关键词: Microbial community structure     Effluent-receiving area     High-throughput sequencing     Costal sediments     Wastewater treatment plant (WWTP)    

Fluoride removal from secondary effluent of the graphite industry using electrodialysis: Optimization

Xiaomeng Wang, Ning Li, Jianye Li, Junjun Feng, Zhun Ma, Yuting Xu, Yongchao Sun, Dongmei Xu, Jian Wang, Xueli Gao, Jun Gao

《环境科学与工程前沿(英文)》 2019年 第13卷 第4期 doi: 10.1007/s11783-019-1132-5

摘要:

RSM was utilized to optimize and model influential parameters on fluoride removal.

Regression models involving independent variables and main response were developed.

Interactive effects and optimum of process factors were illuminated and determined.

Fluoride removal efficiency of 99.69% was observed in optimal process conditions.

关键词: Response surface methodology     Fluoride removal     Electrodialysis     Box-Behnken design    

Effects of nitrite on phosphate uptake in anaerobic-oxic process

LI Jie, XIONG Biyong, ZHANG Shude, YANG Hong, ZHANG Jie

《环境科学与工程前沿(英文)》 2007年 第1卷 第1期   页码 39-42 doi: 10.1007/s11783-007-0007-3

摘要: An anaerobic-oxic (A/O) biological phosphorus removal reactor was operated to study the effect of nitrite on phosphate uptake. The phosphorus uptake profile was determined under different operating conditions. The results indicated that in addition to oxygen and nitrate (DPB, nitrate denitrifying phosphorus removal), to some extent, nitrite could also serve as an electron acceptor to achieve nitrite denitrifying phosphorus removal (DPB). The quantity and rate of phosphorus uptake of DPB, however, were evidently lower than that of DPB The experiment results revealed that nitrite would bring toxic action to phosphate-accumulating organisms (PAOs) when NO-N"e93.7 mg/L. The nitrite existing in the anoxic reactor made no difference to the quantity and rate of denitrifying phosphorus removal, but it could reduce the consumption of nitrate. Moreover, the data showed that the aerobic phosphate uptake of DPB was lower than that of anaerobic phosphorus-released sludge in a traditional A/O process. However, there was not much difference between these two kinds of sludge in terms of the total phosphorus uptake quantity and the effluent quality.

关键词: effluent     PAOs     experiment     phosphate-accumulating     phosphorus removal    

Electro-assisted regeneration of ion exchange resins

LIU Zhigang, WANG Ying, LI Yansheng, CHANG Hui

《环境科学与工程前沿(英文)》 2008年 第2卷 第4期   页码 410-414 doi: 10.1007/s11783-008-0069-x

摘要: Electro-assisted regeneration (EAR) for the mixed bed of strongly acidic cation and weakly basic anion exchange resins with the Al(OH) suspension in a three-compartment cell was investigated. The desalination experiments were carried out to evaluate the characteristic of the regenerated mixed resins. Experimental results showed that the efficiency of resin regeneration was strictly dependent on the voltage, regeneration time, and feed regenerant flow rate. The amount of the effluent reached 50 times the volume of the resins bed, and the conductivity was less than 1.0 ?s/cm. Compared to the conventional ER, the total effluent volume of EAR was about 1000 mL more than that of ER under the same conditions, and the outlet conductivity was significantly lower. The desalination and regeneration reaction mechanisms of the mixed resins indicated the regeneration efficiency of resin with Al(OH) as the regenerant was much higher than that with HO.

关键词: effluent volume     acidic     three-compartment     weakly     exchange    

Industrial water treatment and industrial marine outfalls: Achieving the right balance

Adrian W. K. Law,Chunyan Tang

《化学科学与工程前沿(英文)》 2016年 第10卷 第4期   页码 472-479 doi: 10.1007/s11705-016-1592-0

摘要: Industrial water treatment and industrial marine outfalls both function together to reduce the pollutant concentrations in the effluent and mitigate the potential impact on the environment. The former uses environmental treatment technology with energy and material cost considerations, while the latter utilizes the natural assimilation potential of the coastal water environment achievable at the outfall location. Because of their synergistic nature, marine outfalls are now commonly used for the disposal of partially treated domestic and industrial effluents in many coastal cities around the world, with many successful examples of low and acceptable risks to the environment. The objective of this paper is to review their balance from both environmental and economic considerations. We also discuss the end-of-the-pipe and mixing zone approaches for industrial effluents, and give some recommendations particularly for developing countries. Finally, we emphasize that a compulsory and vigorous monitoring program is essential regardless of how the balance is achieved.

关键词: industrial effluent treatment     industrial marine outfalls     economic and environmental considerations    

标题 作者 时间 类型 操作

Mechanisms for simultaneous ozonation of sulfamethoxazole and natural organic matters in secondary effluent

期刊论文

Dissolved methane in anaerobic effluent: Emission or recovery?

期刊论文

Optimization of thermophilic anaerobic-aerobic treatment system for Palm Oil Mill Effluent (POME)

Yijing CHAN,Meifong CHONG,Chunglim LAW

期刊论文

Controlling various contaminants in wastewater effluent through membranes and engineered wetland

Sarper SARP, Sungyun LEE, Noeon PARK, Nguyen Thi HANH, Jaeweon CHO

期刊论文

Characterization of the dissolved organic matter in sewage effluent of sequence batch reactor: the impact

Jin GUO, Feng SHENG, Jianhua GUO, Xiong YANG, Mintao MA, Yongzhen PENG

期刊论文

Recovering humic substances from the dewatering effluent of thermally treated sludge and its performance

Yuning YANG,Huan LI

期刊论文

Simultaneous enhanced ammonia and nitrate removal from secondary effluent in constructed wetlands using

期刊论文

Unintended nutrient imbalance induced by wastewater effluent inputs to receiving water and its ecological

期刊论文

Effect of effluent organic matter on ozonation of bezafibrate

Huan HE,Qian SUI,Shuguang LU,Wentao ZHAO,Zhaofu QIU,Gang YU

期刊论文

Removal efficiencies of natural and synthetic progesterones in hospital wastewater treated by different disinfection processes

期刊论文

Identifying human-induced influence on microbial community: A comparative study in the effluent-receiving

Yuhan Zheng, Zhiguo Su, Tianjiao Dai, Feifei Li, Bei Huang, Qinglin Mu, Chuanping Feng, Donghui Wen

期刊论文

Fluoride removal from secondary effluent of the graphite industry using electrodialysis: Optimization

Xiaomeng Wang, Ning Li, Jianye Li, Junjun Feng, Zhun Ma, Yuting Xu, Yongchao Sun, Dongmei Xu, Jian Wang, Xueli Gao, Jun Gao

期刊论文

Effects of nitrite on phosphate uptake in anaerobic-oxic process

LI Jie, XIONG Biyong, ZHANG Shude, YANG Hong, ZHANG Jie

期刊论文

Electro-assisted regeneration of ion exchange resins

LIU Zhigang, WANG Ying, LI Yansheng, CHANG Hui

期刊论文

Industrial water treatment and industrial marine outfalls: Achieving the right balance

Adrian W. K. Law,Chunyan Tang

期刊论文