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微生物絮凝剂 1

焦化废水净化 1

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The treatment of black-odorous water using tower bipolar electro-flocculation including the removal of

Huan He, Qinjin Yu, Chaochao Lai, Chen Zhang, Muhan Liu, Bin Huang, Hongping Pu, Xuejun Pan

《环境科学与工程前沿（英文）》 2021年 第15卷 第2期 doi: 10.1007/s11783-020-1310-5

摘要： Abstract • An innovative bubble column tower BPE was designed to treat the black-odorous water. • PO43−, S2− and turbidity were removed, and dissolved oxygen was enriched in the BPE. • An aluminum bipolar electrode gave the best oxygen enrichment and pollutant removal. • Changes of microorganisms confirmed the improvement in water quality achieved. The large amount of municipal wastewater discharged into urban rivers sometimes exceeds the rivers’ self-purification capacity leading to black-odorous polluted water. Electro-flocculation has emerged as a powerful remediation technology. Electro-flocculation in a bubble column tower with a bipolar electrode (BPE) was tested in an attempt to overcome the high resistance and weak gas-floatation observed with a monopolar electrode (MPE) in treating such water. The BPE reactor tested had a Ti/Ta2O5-IrO2 anode and a graphite cathode with an iron or aluminum bipolar electrode suspended between them. It was tested for its ability to reduce turbidity, phosphate and sulphion and to increase the concentration of dissolved oxygen. The inclusion of the bipolar electrode was found to distinctly improved the system’s conductivity. The system’s electro-flocculation and electrical floatation removed turbidity, phosphate and sulphion completely, and the dissolved oxygen level improved from 0.29 to 6.28 mg/L. An aluminum bipolar electrode performed better than an iron one. Changes in the structure of the microbial community confirmed a significant improvement in water quality.

关键词： Black-odorous water     Bipolar electrodes     Flocculation     Floatation     Oxygen enrichment     Turbidity    

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Flocculation behaviors of a novel papermaking sludge-based flocculant in practical printing and dyeing

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-021-1390-x

摘要：

•PSBF performed better than PAC and PAM in CODCr removals.

关键词： Practical wastewater treatment     Commercial coagulant/flocculant     Secondary coagulation-flocculation process     Chemical oxygen demand     Coagulation-flocculation mechanism    

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Performance evaluation on the pollution control against wet weather overflow based on on-site coagulation/flocculation

Zongqun Chen, Wei Jin, Hailong Yin, Mengqi Han, Zuxin Xu

《环境科学与工程前沿（英文）》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1400-z

摘要： Abstract • A way for overflow control based on on-site coagulation/flocculation was proposed. • Coagulant and flocculant dose were optimized based on pollutant removal performance. • Settling time of 5 min is enough in a proper transmission distance. • Fast removal of particulate pollutants could be achieved under varied flow. The pollution caused by wet weather overflow in urban drainage systems is a main factor causing blackening an odorization of urban rivers. The conventional overflow treatment based on coagulation/flocculation in terminal drainage systems requires relatively large space and long retention time demand that makes it not applicable in crowded urban drainage systems or under heavy rains. On-site coagulation/flocculation in terminal drainage pipes was proposed in this study which was aimed to transfer the coagulation/flocculation process to the inside of pipes at the terminal drainage system to save space and reduce the retention time of the coagulation/flocculation process. The optimized dose of chemicals was studied first which was 80 mg/L of coagulant and 0.8 mg/L of flocculant. Settling for only 5 min can remove most of the pollutants at 406.5 m of transmission distance. In addition, the relation of wet weather overflow rate and concentration of pollution load on the on-site coagulation/flocculation process was investigated, which indicated that high removal of pollutant was gained at a large range of flow velocity and pollutant concentration. Finally, the study confirmed electric neutralization, bridging, and net capture as the major mechanisms in this process, and further optimization was proposed. The proposed process can reduce much turbidity, chemical oxygen demand, and total phosphorous, but hardly remove soluble ammonia and organics. This work provides scientific guidance to address wet weather overflow in terminal drainage pipes.

关键词： Wet weather overflow     On-site coagulation/flocculation     Fast removal of particulate pollutants    

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Optimization and modeling of coagulation-flocculation to remove algae and organic matter from surface

Ziming Zhao, Wenjun Sun, Madhumita B. Ray, Ajay K Ray, Tianyin Huang, Jiabin Chen

《环境科学与工程前沿（英文）》 2019年 第13卷 第5期 doi: 10.1007/s11783-019-1159-7

摘要： Charge neutralization and sweep flocculation were the major mechanisms. Effect of process parameters was investigated. Optimal coagulation conditions were studied by response surface methodology. ANN models presented more robust and accurate prediction than RSM. Seasonal algal blooms of Lake Yangcheng highlight the necessity to develop an effective and optimal water treatment process to enhance the removal of algae and dissolved organic matter (DOM). In the present study, the coagulation performance for the removal of algae, turbidity, dissolved organic carbon (DOC) and ultraviolet absorbance at 254 nm (UV254) was investigated systematically by central composite design (CCD) using response surface methodology (RSM). The regression models were developed to illustrate the relationships between coagulation performance and experimental variables. Analysis of variance (ANOVA) was performed to test the significance of the response surface models. It can be concluded that the major mechanisms of coagulation to remove algae and DOM were charge neutralization and sweep flocculation at a pH range of 4.66–6.34. The optimal coagulation conditions with coagulant dosage of 7.57 mg Al/L, pH of 5.42 and initial algal cell density of 3.83 × 106 cell/mL led to removal of 96.76%, 97.64%, 40.23% and 30.12% in term of cell density, turbidity, DOC and UV254 absorbance, respectively, which were in good agreement with the validation experimental results. A comparison between the modeling results derived through both ANOVA and artificial neural networks (ANN) based on experimental data showed a high correlation coefficient, which indicated that the models were significant and fitted well with experimental results. The results proposed a valuable reference for the treatment of algae-laden surface water in practical application by the optimal coagulation-flocculation process.

关键词： Algae     Coagulation-flocculation     Response surface methodology     Artificial neural networks    

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微生物絮凝剂的絮凝条件及焦化废水净化研究

魏晓金,李静,何绪文

《中国工程科学》 2009年 第11卷 第2期   页码 88-91

摘要：

从活性污泥中筛选出一株能产高效絮凝剂的芽孢杆菌，对该菌产生的微生物絮凝剂进行了絮凝条 件及废水絮凝实验研究。结果表明，微生物絮凝剂最佳絮凝条件为：原水pH值7.0以上；助凝剂CaCl2 （1％ 浓度）适宜投加量为 5.0 ％ ；发酵液的适宜投加量为0.2％ ；发酵液较好的离心条件为n ＝ 4000转/min， t ＝ 30 min。在最佳絮凝条件下，该菌产生的微生物絮凝剂对多种废水净化效果明显。

关键词： 微生物絮凝剂     絮凝条件     焦化废水净化    

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Suspended solid abatement in a conical fluidized bed flocculator

Dandan ZHOU, Shuangshi DONG, Keyu LI, Huizhong JIANG, Dandan SHANG

《环境科学与工程前沿（英文）》 2013年 第7卷 第1期   页码 127-134 doi: 10.1007/s11783-012-0415-x

摘要： With the random movement of silica gel beads in a conical fluidized bed, micro-vortices resulting from the fluidization promoted the collision and aggregation of suspended fine kaolin powders. The abatement efficiencies of the suspended fine solids under several hydrodynamic conditions were studied, and a suitable control strategy for operating the conical fluidized bed flocculators was identified. The suspended solids abatement efficiency was found to increase with increasing Camp Number and flocculation time ( ), but decreased with the increase of velocity gradient ( ) within the range studied in this research (165.1–189.6 s ). The abatement efficiencies were all more than 60% at the range of = 165–180 s and = 15–33 s at an initial kaolin solid concentration of 150 mg·L , polymer aluminum chloride dosage of 60 mg·L and sedimentation time of 20 min. However, the formation of flocs was influenced by the liquid backmixing. Excessive backmixing caused the breakup of flocs and resulted in difficulty for the fine powders to aggregate and sediment to the reactor bottom. The results of the calculated fractal dimension and measured free sedimentation velocity of flocs obtained at different runs showed similar flocs properties, and indicated an easy control strategy for sedimentation of the flocs.

关键词： conical fluidized bed     flocculation     velocity gradient    

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What have we known so far about microplastics in drinking water treatment? A timely review

《环境科学与工程前沿（英文）》 2022年 第16卷 第5期 doi: 10.1007/s11783-021-1492-5

摘要：

• 23 available research articles on MPs in drinking water treatment are reviewed.

关键词： Microplastics     Drinking water treatment     Coagulation     Flocculation     Membrane     Filtration    

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Evaluation of activated sludge properties’ changes in industrial-wastewater pre-treatment: role of residual aluminum hydrolyzed species with different polymerization degree

《环境科学与工程前沿（英文）》 2023年 第17卷 第6期 doi: 10.1007/s11783-023-1675-3

摘要：

● Medium poly Al salts dominated the PAC residual salts with a rational dosage.

关键词： Coagulation/flocculation     Hydroxyl-aluminum     Hydrolysis reaction     Reactor performance     Activated sludge property     Surface properties    

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Repeated batch fermentation with water recycling and cell separation for microbial lipid production

Yumei WANG, Wei LIU, Jie BAO

《化学科学与工程前沿（英文）》 2012年 第6卷 第4期   页码 453-460 doi: 10.1007/s11705-012-1210-8

摘要： Large waste water disposal was the major problem in microbial lipid fermentation because of low yield of lipid. In this study, the repeated batch fermentation was investigated for reducing waste water generated in the lipid fermentation of an oleaginous yeast CX1 strain. The waste fermentation broth was recycled in the next batch operation after the cells were separated using two different methods, centrifugation and flocculation. Two different sugar substrates, glucose and inulin, were applied to the proposed operation. The result showed that at least 70% of the waste water was reduced, while lipid production maintained satisfactory in the initial four cycles. Furthermore, it is suggested that CX1 cells might produce certain naturally occurring inulin hydrolyzing enzyme(s) for obtaining fructose and glucose from inulin directly. Our method provided a practical option for reducing the waste water generated from microbial lipid fermentation.

关键词： batch fermentation     microbial lipid     Trichosporon cutaneum CX1     flocculation     waste water recycle    

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A new polystyrene-latex-based and EPS-containing synthetic sludge

Ling-Ling Wang, Shan Chen, Hai-Ting Zheng, Guo-Qing Sheng, Zhi-Jun Wang, Wen-Wei Li, Han-Qing Yu

《环境科学与工程前沿（英文）》 2012年 第6卷 第1期   页码 131-139 doi: 10.1007/s11783-011-0390-7

摘要： Since the living microorganisms in activated sludge continuously change, it is difficult to conduct controlled experiments and achieve reproducible results for evaluating sludge characteristics. Synthetic sludge, as a chemical surrogate to activated sludge, could be used to investigate the sludge physicochemical properties, and it is desirable to prepare synthetic sludge with similar structure and properties to real activated sludge to explore the flocculation and settlement processes in activated sludge systems. In this work, a high-strength synthetic sludge was prepared with functional polystyrene latex particles as the framework and extracellular polymeric substances (EPS) to modify its surface. The flocculation and settling characteristics of the microspheres and the prepared synthetic sludge were tested. Compared with other three functional polystyrene latex microspheres, the synthetic sludge prepared with EPS-modified polystyrene latex microspheres showed good settling characteristics and a significantly higher strength. They could be used for studying the physicochemical properties of activated sludge.

关键词： activated sludge     extracellular polymeric substances (EPS)     flocculation     polystyrene latex particles     synthetic sludge    

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Detection of geosmin and 2-methylisoborneol by liquid-liquid extraction-gas chromatograph mass spectrum (LLE-GCMS) and solid phase extraction-gas chromatograph mass spectrum (SPE-GCMS)

MA Xiaoyan, CHEN Beibei, LI Qingsong, ZHANG Qiaoli, GU Guofen

《环境科学与工程前沿（英文）》 2007年 第1卷 第3期   页码 286-291 doi: 10.1007/s11783-007-0048-7

摘要： Two sample preparation methods were introduced and compared in this paper to establish a simple, quick and exact analysis of geosmin and 2-methylisoborneol. LC-18 column was employed in solid phase extraction (SPE), 1.0 mL of hexane was adopted in liquid-liquid extraction (LLE), and the extracts were analyzed by gas chromatograph mass spectrum (GCMS) in selected ion mode. Mean recoveries of SPE were low for 2-methylisoborneol (2-MIB) and geosmin (GSM) with values below 50%. For LLE, the recoveries were satisfyingly above 50% for 2-MIB and 80% for GSM. Detection limits of the LLE method were as low as 1.0 ng/L for GSM and 5.0 ng/L for 2-MIB. A year-long investigation on odor chemicals of drinking water in Shanghai demonstrated that in the summer, there was a serious odor problem induced by a high concentration of 2-MIB. The highest concentration of 152.82 ng/L appeared in July in raw water, while GSM flocculation was minimal with concentrations below odor threshold.

关键词： summer     flocculation     simple     Shanghai     spectrum    

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标题 作者 时间 类型 操作

The treatment of black-odorous water using tower bipolar electro-flocculation including the removal of

Huan He, Qinjin Yu, Chaochao Lai, Chen Zhang, Muhan Liu, Bin Huang, Hongping Pu, Xuejun Pan

期刊论文

Flocculation behaviors of a novel papermaking sludge-based flocculant in practical printing and dyeing

期刊论文

Performance evaluation on the pollution control against wet weather overflow based on on-site coagulation/flocculation

Zongqun Chen, Wei Jin, Hailong Yin, Mengqi Han, Zuxin Xu

期刊论文

Optimization and modeling of coagulation-flocculation to remove algae and organic matter from surface

Ziming Zhao, Wenjun Sun, Madhumita B. Ray, Ajay K Ray, Tianyin Huang, Jiabin Chen

期刊论文

微生物絮凝剂的絮凝条件及焦化废水净化研究

魏晓金,李静,何绪文

期刊论文

Suspended solid abatement in a conical fluidized bed flocculator

Dandan ZHOU, Shuangshi DONG, Keyu LI, Huizhong JIANG, Dandan SHANG

期刊论文

What have we known so far about microplastics in drinking water treatment? A timely review

期刊论文

Evaluation of activated sludge properties’ changes in industrial-wastewater pre-treatment: role of residual aluminum hydrolyzed species with different polymerization degree

期刊论文

Repeated batch fermentation with water recycling and cell separation for microbial lipid production

Yumei WANG, Wei LIU, Jie BAO

期刊论文

A new polystyrene-latex-based and EPS-containing synthetic sludge

Ling-Ling Wang, Shan Chen, Hai-Ting Zheng, Guo-Qing Sheng, Zhi-Jun Wang, Wen-Wei Li, Han-Qing Yu

期刊论文

Detection of geosmin and 2-methylisoborneol by liquid-liquid extraction-gas chromatograph mass spectrum (LLE-GCMS) and solid phase extraction-gas chromatograph mass spectrum (SPE-GCMS)

MA Xiaoyan, CHEN Beibei, LI Qingsong, ZHANG Qiaoli, GU Guofen

期刊论文