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Multi-objective optimization of molten carbonate fuel cell system for reducing CO

Ramin ROSHANDEL,Majid ASTANEH,Farzin GOLZAR

《能源前沿（英文）》 2015年第9卷第1期页码 106-114 doi: 10.1007/s11708-014-0341-7

摘要： The aim of this paper is to investigate the implementation of a molten carbonate fuel cell (MCFC) as a CO separator. By applying multi-objective optimization (MOO) using the genetic algorithm, the optimal values of operating load and the corresponding values of objective functions are obtained. Objective functions are minimization of the cost of electricity (COE) and minimization of CO emission rate. CO tax that is accounted as the pollution-related cost, transforming the environmental objective to the cost function. The results show that the MCFC stack which is fed by the syngas and gas turbine exhaust, not only reduces CO emission rate, but also produces electricity and reduces environmental cost of the system.

关键词： molten carbonate fuel cell (MCFC) multi-objective optimization (MOO) Pareto curve genetic algorithm CO₂ separation

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Comparative analysis of ceramic-carbonate nanocomposite fuel cells using composite GDC/NLC electrolyte

Muhammad I. Asghar, Sakari Lepikko, Janne Patakangas, Janne Halme, Peter D. Lund

《化学科学与工程前沿（英文）》 2018年第12卷第1期页码 162-173 doi: 10.1007/s11705-017-1642-2

摘要： A comparative analysis of perovskite structured cathode materials, La Sr MnO (LSM), La Sr CoO (LSC), La Sr FeO (LSF) and La Sr Co Fe O (LSCF), was performed for a ceramic-carbonate nanocomposite fuel cell using composite electrolyte consisting of Gd Ce O (GDC) and a eutectic mixture of Na CO and Li CO . The compatibility of these nanocomposite electrode powder materials was investigated under air, CO and air/CO atmospheres at 550 °C. Microscopy measurements together with energy dispersive X-ray spectroscopy (EDS) elementary analysis revealed few spots with higher counts of manganese relative to lanthanum and strontium under pure CO atmosphere. Furthermore, electrochemical impedance (EIS) analysis showed that LSC had the lowest resistance to oxygen reduction reaction (ORR) (14.12 Ω·cm ) followed by LSF (15.23 Ω·cm ), LSCF (19.38 Ω·cm ) and LSM (>300 Ω·cm ). In addition, low frequency EIS measurements (down to 50 µHz) revealed two additional semi-circles at frequencies around 1 Hz. These semicircles can yield additional information about electrochemical reactions in the device. Finally, a fuel cell was fabricated using GDC/NLC nanocomposite electrolyte and its composite with NiO and LSCF as anode and cathode, respectively. The cell produced an excellent power density of 1.06 W/cm at 550 °C under fuel cell conditions.

关键词： electrode fuel cell low-temperature nanocomposite perovskite

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Phenomena identification and ranking table exercise for thorium based molten salt reactor-solid fuel

Xiaojing LIU, Qi WANG, Zhaozhong HE, Kun CHEN, Xu CHENG

《能源前沿（英文）》 2019年第13卷第4期页码 707-714 doi: 10.1007/s11708-019-0616-0

摘要： Thorium based molten salt reactor-solid fuel (TMSR-SF) design is an innovative reactor concept that uses high-temperature tristructural-isotropic (TRISO) fuel with a low-pressure liquid salt coolant. In anticipation of getting licensed applications for TMSR-SF in the future, it is necessary to fully understand the significant features and phenomena of TMSR-SF design, as well as its transient behavior during accidents. In this paper, the safety-relevant phenomena, importance, and knowledge base were assessed for the selected events and the transient of TMSR-SF during station blackout scenario is simulated based on RELAP/SCDAPSIM Mod 4.0. The phenomena having significant impact but with limited knowledge of their history are core coolant bypass flows, outlet plenum flow distribution, and intermediate heat exchanger (IHX) over/under cooling transients. Some thermal hydraulic parameters during the station blackout scenario are also discussed.

关键词： phenomena identification and ranking table (PIRT) thorium based molten salt reactor-solid fuel (TMSR-SF) safety analysis RELAP/SCDAPSIM

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Analysis of molten metal spreading and solidification behaviors utilizing moving particle full-implicit

《能源前沿（英文）》 2021年第15卷第4期页码 959-973 doi: 10.1007/s11708-021-0753-0

摘要： To retrieve the fuel debris in Fukushima Daiichi Nuclear Power Plants (1F), it is essential to infer the fuel debris distribution. In particular, the molten metal spreading behavior is one of the vital phenomena in nuclear severe accidents because it determines the initial condition for further accident scenarios such as molten core concrete interaction (MCCI). In this study, the fundamental molten metal spreading experiments were performed with different outlet diameters and sample amounts to investigate the effect of the outlet for spreading-solidification behavior. In the numerical analysis, the moving particle full-implicit method (MPFI), which is one of the particle methods, was applied to simulate the spreading experiments. In the MPFI framework, the melting-solidification model including heat transfer, radiation heat loss, phase change, and solid fraction-dependent viscosity was developed and implemented. In addition, the difference in the spreading and solidification behavior due to the outlet diameters was reproduced in the calculation. The simulation results reveal the detailed solidification procedure during the molten metal spreading. It is found that the viscosity change and the solid fraction change during the spreading are key factors for the free surface condition and solidified materials. Overall, it is suggested that the MPFI method has the potential to simulate the actual nuclear melt-down phenomena in the future.

关键词： molten metal spreading solidification particle method severe accident fuel debris decommissioning

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Dynamic characteristics of molten droplets and hot particles falling in liquid pool

Liangxing LI, Weimin MA, Huixiong LI, Tingkuan CHEN,

《能源前沿（英文）》 2010年第4卷第2期页码 246-251 doi: 10.1007/s11708-009-0077-y

摘要： The dynamic characteristics of molten droplets and hot particles at the very beginning of their fall into coolant pools are presented. The falling course of a single droplet or a single hot particle was recorded by a high-speed camera and a curve of velocity . time was obtained. Emphasis was placed on the effects of the droplet’s size and temperature, the coolant’s temperature and properties, and the droplet’s physical properties on the moving behavior. The results for the all cases showed that the velocity of a falling droplet/particle decreased rapidly but rebounded shortly, at the beginning of droplet/particle falling in the coolant. Following such a V-shaped evolution in velocity, the droplet/particle slows down gradually to a comparatively steady velocity. An increase in either coolant temperature or droplet temperature results in a larger velocity variation in the “J-region”, but a smaller deceleration when it moves out of the “J-region”. The elevated volatility of a coolant leads to a steeper deceleration in the “J-region” and beyond. The bigger size of a particle leads to a greater velocity variation in the “J-region” and terminal velocity. A high melting point and thermal conductivity as well as lower heat capacity contribute to dramatic variation in the “J-region” and low terminal velocity.

关键词： dynamic characteristics molten droplets high-temperature particles fuel and coolant interactions

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Failure mode investigation of fuel cell for vehicle application

Zhongjun HOU, Renfang WANG, Keyong WANG, Weiyu SHI, Danming XING, Hongchun JIANG

《能源前沿（英文）》 2017年第11卷第3期页码 318-325 doi: 10.1007/s11708-017-0488-0

摘要： The durability of proton exchange membrane fuel cells (PEMFCs) has been posing a key technical challenge to commercial spread of fuel cell vehicles (FCVs). To improve the durability, it is necessary to optimize the fuel cell system (FCS) design against failure modes. The fuel cell durability research method at FCS scale was exhibited, and the failure modes of fuel cell were experimentally investigated in this paper. It is found that the fuel cell dry operation, start/stop cycle and gas diffusion layer (GDL) flooding are typical failure modes of fuel cells. After the modifications against the failure modes, the durability of FCSs is improved to over 3000 h step by step.

关键词： proton exchange membrane fuel cell (PEMFC) fuel cell system (FCS) durability failure mode fuel cell vehicle (FCV) carbon corrosion water management

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A comprehensive assessment on the durability of gas diffusion electrode materials in PEM fuel cell stack

Arunkumar JAYAKUMAR

《能源前沿（英文）》 2019年第13卷第2期页码 325-338 doi: 10.1007/s11708-019-0618-y

摘要： Polymer electrolyte membrane (PEM) fuel cell is the most promising among the various types of fuel cells. Though it has found its applications in numerous fields, the cost and durability are key barriers impeding the commercialization of PEM fuel cell stack. The crucial and expensive component involved in it is the gas diffusion electrode (GDE) and its degradation, which limits the performance and life of the fuel cell stack. A critical analysis and comprehensive understanding of the structural and functional properties of various materials involved in the GDE can help us to address the related durability and cost issues. This paper reviews the key GDE components, and in specific, the root causes influencing the durability. It also envisages the role of novel materials and provides a critical recommendation to improve the GDE durability.

关键词： PEM fuel cell gas diffusion electrode(GDE) gas diffusion layer(GDL) membrane electrode assembly durability fuel cell catalyst

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A hybrid fuel cell for water purification and simultaneously electricity generation

《环境科学与工程前沿（英文）》 2023年第17卷第1期 doi: 10.1007/s11783-023-1611-6

摘要：

● A novel hybrid fuel cell (F-HFC) was fabricated.

关键词： Flow-through field Hybrid fuel cell Polyoxometalates Water purification Electricity generation

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TiO supported IrO for anode reversal tolerance in proton exchange membrane fuel cell

《能源前沿（英文）》 2022年第16卷第5期页码 852-861 doi: 10.1007/s11708-021-0811-7

摘要： Fuel starvation can occur and cause damage to the cell when proton exchange membrane fuel cells operate under complex working conditions. In this case, carbon corrosion occurs. Oxygen evolution reaction (OER) catalysts can alleviate carbon corrosion by introducing water electrolysis at a lower potential at the anode in fuel shortage. The mixture of hydrogen oxidation reaction (HOR) and unsupported OER catalyst not only reduces the electrolysis efficiency, but also influences the initial performance of the fuel cell. Herein, Ti₄O₇ supported IrO_x is synthesized by utilizing the surfactant-assistant method and serves as reversal tolerant components in the anode. When the cell reverse time is less than 100 min, the cell voltage of the MEA added with IrO_x/Ti₄O₇ has almost no attenuation. Besides, the MEA has a longer reversal time (530 min) than IrO_x (75 min), showing an excellent reversal tolerance. The results of electron microscopy spectroscopy show that IrO_x particles have a good dispersity on the surface of Ti₄O₇ and IrO_x/Ti₄O₇ particles are uniformly dispersed on the anode catalytic layer. After the stability test, the Ti₄O₇ support has little decay, demonstrating a high electrochemical stability. IrO_x/Ti₄O₇ with a high dispersity has a great potential to the application on the reversal tolerance anode of the fuel cell.

关键词： proton exchange membrane fuel cell (PEMFC) fuel starvation cell reverse reversal tolerance anode oxygen evolution reaction

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Significant potential of Solid Oxide Fuel Cell systems for distributed power generation and carbon neutrality

《能源前沿（英文）》 2022年第16卷第6期页码 879-882 doi: 10.1007/s11708-022-0850-8

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Numerical investigation of the chemical and electrochemical characteristics of planar solid oxide fuelcell with direct internal reforming

Yuzhang WANG, Shilie WENG, Yiwu WENG

《能源前沿（英文）》 2011年第5卷第2期页码 195-206 doi: 10.1007/s11708-011-0148-8

摘要： A fully three-dimensional mathematical model of a planar solid oxide fuel cell (SOFC) with complete direct internal steam reforming was constructed to investigate the chemical and electrochemical characteristics of the porous-electrode-supported (PES)-SOFC developed by the Central Research Institute of Electric Power Industry of Japan. The effective kinetic models developed over the Ni/YSZ anode takes into account the heat transfer and species diffusion limitations in this porous anode. The models were used to simulate the methane steam reforming processes at the co- and counter-flow patterns. The results show that the flow patterns of gas and air have certain effects on cell performance. The cell at the counter-flow has a higher output voltage and output power density at the same operating conditions. At the counter-flow, however, a high hotspot temperature is observed in the anode with a non-fixed position, even when the air inlet flow rate is increased. This is disadvantageous to the cell. Both cell voltage and power density decrease with increased air flow rate.

关键词： planar solid oxide fuel cell (SOFC) direct internal reforming chemical reaction methane electrochemical

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Scaling up a novel denitrifying microbial fuel cell with an oxic-anoxic two stage biocathode

Peng LIANG, Jincheng WEI, Ming LI, Xia HUANG

《环境科学与工程前沿（英文）》 2013年第7卷第6期页码 913-919 doi: 10.1007/s11783-013-0583-3

摘要： A scaled up microbial fuel cell (MFC) of a 50 L volume was set up with an oxic-anoxic two-stage biocathode and activated semicoke packed electrodes to achieve simultaneous power generation and nitrogen and organic matter removals. An average maximum power density of 43.1 W·m was obtained in batch operating mode. By adjusting the two external resistances, the denitrification in the A-MFC and power production in the O-MFC could be enhanced. In continuous mode, when the hydraulic retention times were set at 6 h, 8 h and 12 h, the removal efficiencies of COD, and total nitrogen (TN) were higher than 95%, 97%, and 84%, respectively. Meanwhile the removal loads for COD, and TN were10, 0.37 and 0.4 kg·(m ·d) , respectively.

关键词： microbial fuel cell (MFC) oxic-anoxic two stage biocathode denitrifying

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锌空燃料电池电站

朱梅,徐献芝,苏润

《中国工程科学》 2004年第6卷第12期页码 62-64

摘要：

燃料电池发电技术已经受到人们越来越多的重视。介绍了利用锌空气燃料电池技术建设电站，利用分体式电极技术制造世界上最大的单电池，该电站采用独特的分离循环技术，可以提高电站总体效率。给出建设电站的相关参数。

关键词：燃料电池锌空气燃料电池分体式电极单电池分离循环技术

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A mini-microbial fuel cell for voltage testing of exoelectrogenic bacteria

Xiaoxin CAO , Xia HUANG , Xiaoyuan ZHANG , Peng LIANG , Mingzhi FAN ,

《环境科学与工程前沿（英文）》 2009年第3卷第3期页码 307-312 doi: 10.1007/s11783-009-0028-1

摘要： Current methods for testing the electricity generation capacity of isolates are time- and labor-consuming. This paper presents a rapid voltage testing system of exoelectrogenic bacteria called Quickscreen, which is based on a microliter microbial fuel cell (MFC). and were used as the model exoelectrogenic bacteria; that cannot generate electricity was used as a negative control. It was found that the electricity generation capacity of the isolates could be determined within about five hours by using Quickscreen, and that its time was relatively rapid compared with the time needed by using larger MFCs. A parallel, stable, and low background voltage was achieved using titanium as a current collector in the blank run. The external resistance had little impact on the blank run during the initial period. The cathode with a five-hole configuration, used to hydrate the carbon cathode, gave higher cathode potentials than did that with a one-hole configuration. Steady discharge and current interrupt methods showed that the anode mostly contributed to the large internal resistance of the Quickscreen system. However, the addition of graphite felt decreased the resistance from 18kΩ to 5kΩ. This device was proved to be useful to rapidly evaluate the electricity generation capacity of different bacteria.

关键词： microbial fuel cell exoelectrogenic bacteria rapid screening

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Abating transport GHG emissions by hydrogen fuel cell vehicles: Chances for the developing world

Han HAO, Zhexuan MU, Zongwei LIU, Fuquan ZHAO

《能源前沿（英文）》 2018年第12卷第3期页码 466-480 doi: 10.1007/s11708-018-0561-3

摘要：

Fuel cell vehicles, as the most promising clean vehicle technology for the future, represent the major chances for the developing world to avoid high-carbon lock-in in the transportation sector. In this paper, by taking China as an example, the unique advantages for China to deploy fuel cell vehicles are reviewed. Subsequently, this paper analyzes the greenhouse gas (GHG) emissions from 19 fuel cell vehicle utilization pathways by using the life cycle assessment approach. The results show that with the current grid mix in China, hydrogen from water electrolysis has the highest GHG emissions, at 3.10 kgCO₂/km, while by-product hydrogen from the chlor-alkali industry has the lowest level, at 0.08 kgCO₂/km. Regarding hydrogen storage and transportation, a combination of gas-hydrogen road transportation and single compression in the refueling station has the lowest GHG emissions. Regarding vehicle operation, GHG emissions from indirect methanol fuel cell are proved to be lower than those from direct hydrogen fuel cells. It is recommended that although fuel cell vehicles are promising for the developing world in reducing GHG emissions, the vehicle technology and hydrogen production issues should be well addressed to ensure the life-cycle low-carbon performance.

关键词： hydrogen fuel cell vehicle life cycle assessment energy consumption greenhouse gas (GHG) emissions China

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标题作者时间类型操作

Multi-objective optimization of molten carbonate fuel cell system for reducing CO

Ramin ROSHANDEL,Majid ASTANEH,Farzin GOLZAR

期刊论文

Comparative analysis of ceramic-carbonate nanocomposite fuel cells using composite GDC/NLC electrolyte

Muhammad I. Asghar, Sakari Lepikko, Janne Patakangas, Janne Halme, Peter D. Lund

期刊论文

Phenomena identification and ranking table exercise for thorium based molten salt reactor-solid fuel

Xiaojing LIU, Qi WANG, Zhaozhong HE, Kun CHEN, Xu CHENG

期刊论文

Analysis of molten metal spreading and solidification behaviors utilizing moving particle full-implicit

期刊论文

Dynamic characteristics of molten droplets and hot particles falling in liquid pool

Liangxing LI, Weimin MA, Huixiong LI, Tingkuan CHEN,

期刊论文

Failure mode investigation of fuel cell for vehicle application

Zhongjun HOU, Renfang WANG, Keyong WANG, Weiyu SHI, Danming XING, Hongchun JIANG

期刊论文

A comprehensive assessment on the durability of gas diffusion electrode materials in PEM fuel cell stack

Arunkumar JAYAKUMAR

期刊论文

A hybrid fuel cell for water purification and simultaneously electricity generation

期刊论文

TiO supported IrO for anode reversal tolerance in proton exchange membrane fuel cell

期刊论文

Significant potential of Solid Oxide Fuel Cell systems for distributed power generation and carbon neutrality

期刊论文

Numerical investigation of the chemical and electrochemical characteristics of planar solid oxide fuelcell with direct internal reforming

Yuzhang WANG, Shilie WENG, Yiwu WENG

期刊论文

Scaling up a novel denitrifying microbial fuel cell with an oxic-anoxic two stage biocathode

Peng LIANG, Jincheng WEI, Ming LI, Xia HUANG

期刊论文

锌空燃料电池电站

朱梅,徐献芝,苏润

期刊论文

A mini-microbial fuel cell for voltage testing of exoelectrogenic bacteria

Xiaoxin CAO , Xia HUANG , Xiaoyuan ZHANG , Peng LIANG , Mingzhi FAN ,

期刊论文

Abating transport GHG emissions by hydrogen fuel cell vehicles: Chances for the developing world

Han HAO, Zhexuan MU, Zongwei LIU, Fuquan ZHAO

期刊论文

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