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The innovation and practice of shale oil development system engineering management based on dialecticalrelationships: A case study of Gulong shale oil in Daqing oilfield

《工程管理前沿（英文）》 doi: 10.1007/s42524-024-3072-4

摘要： The development of shale oil is of considerable strategic importance, particularly concerning national security implications. Effective management is vital to maximize both efficiency and socio-economic benefits. This process necessitates addressing four critical relationships: balancing local and global factors, reconciling universality with particularity, integrating inheritance with innovation, and resolving primary and secondary contradictions. These relationships pose several management challenges that must be overcome to develop a robust management model for shale oil extraction. This paper uses the Gulong shale oil in the Daqing oilfield as a case study to examine the implications and specific manifestations of these relationships. To address the limitations of traditional management models, which often overly emphasize local factors, particularity, innovation, and secondary contradictions, we have developed the “Integrated Dialectical Four-Domain Coupling Management Model.” This model incorporates systems engineering theory into management strategies. Key strategies include the global deployment of experimental zone construction, systematic geological and engineering integration, combining historical practices with innovative approaches, phase analysis, and contradiction coordination. These strategies have significantly advanced the development of Gulong shale oil, demonstrating positive on-site results. The innovative management processes detailed in this paper provide valuable insights applicable to similar reservoirs and other large-scale engineering management projects.

关键词： management mode innovation systematic management dialectical relationships shale oil

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Biodegradable, superhydrophobic walnut wood membrane for the separation of oil/water mixtures

《化学科学与工程前沿（英文）》 2022年第16卷第9期页码 1377-1386 doi: 10.1007/s11705-022-2157-z

摘要： The preparation of environmentally friendly oil/water separation materials remains a great challenge. Freeze-drying of wood after lignin removal yields wood aerogels, which can be used as substrates to prepare fluorine-free environmentally friendly superhydrophobic materials, However, they are more suitable for absorption rather than filtration applications due to their poor strength. A study using cross-sections of pristine wood chips as substrates retains the original strength of wood, but the use of the cross-sectional of wood pieces limits their thickness, strength, and size. In this paper, a degradable fluorine-free superhydrophobic film (max. water contact angle of approximately 164.2°) with self-cleaning and abrasion resistance characteristics was prepared by a one-step method using pristine and activated walnut longitudinal section films as the substrate, with tetraethyl orthosilicate as a precursor and dodecyltriethoxysilane as a modifier. The tensile strength results show that superhydrophobic films with pristine or activated wood substrates maintained the strength of pristine wood and were 2.2 times stronger than the wood aerogel substrate. In addition, after cross-laminating the two samples, the films had the ability to separate oil and water by continuous filtration with high efficiency (98.5%) and flux (approximately 1.3 × 10³ L∙m^‒2∙h^‒1). The method has potential for the large-scale fabrication of degradable superhydrophobic filtration separation membranes.

关键词： wood nanotechnology superhydrophobic biodegradable surface modification oil/water separation

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Co-hydrotreating light cycle oil-canola oil blends

Huali WANG, Hena FAROOQI, Jinwen CHEN

《化学科学与工程前沿（英文）》 2015年第9卷第1期页码 64-76 doi: 10.1007/s11705-015-1504-8

摘要： Canola oil and light cycle oil (LCO) blends were co-hydrotreated over a commercial hydrotreating catalyst (NiMo/Al O ) to produce diesel fuel with a green diesel component. High hydrodeoxygenation, hydrodesulphurization and hydrodenitrogenation catalytic activities were achieved for all three feedstocks tested in the temperature range of 350–380 °C with a hydrogen pressure of 7 MPa and a gas/oil ratio of 800 nL/L. The hydrocracking conversion of the 360 °C+ materials in the feedstocks increased by 5% and 15% when 5 and 7.5 wt-% canola oil was added to the LCO, respectively. Compared to the pure LCO, the cetane index of the diesel product formed from hydrotreating the two canola oil-LCO blends increased by 2.5 and 4, respectively. Due to the higher hydrogen requirement to crack and deoxygenate the triglycerides contained in the canola oil, a higher hydrogen consumption was needed to hydrotreat the canola oil-LCO blends.

关键词： hydrotreating co-hydrotreating co-processing canola oil light cycle oil (LCO)

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Microwave-assisted pyrolysis of plastics for aviation oil production: energy and economic analyses

《化学科学与工程前沿（英文）》 2024年第18卷第7期页码 81-81 doi: 10.1007/s11705-024-2436-y

摘要： Microwave-assisted pyrolysis is an effective method for recycling plastic wastes into oils that can be used for aviation fuels. In this study, energy and economic analyses of aviation oil production from microwave-assisted pyrolysis of polystyrene were performed. The total energy efficiency, recovered energy efficiency, unitary cost, unitary energy economic cost, relative cost difference, and energy economic factor were detailed. And the effects of microwave power, pyrolysis temperature, microwave absorbent loading, and microwave absorbent type on these parameters were covered. It was found that pyrolysis temperature has the most significant effect on the unitary cost and unitary energy economic cost of aviation oil, and-microwave absorbent type has a significant influence on energy economic factor during the whole microwave-assisted pyrolysis process. The optimum reaction conditions at the tonnage system for pyrolysis of 1 t polystyrene were microwave power of 650 W, pyrolysis temperature of 460 °C, and silicon carbide (microwave absorbent) at a loading of 2 t (twice than feedstock loading). At these optimal conditions, the total energy efficiency, recovered energy efficiency, unitary cost, unitary energy economic cost, relative cost difference, and energy economic factor were 62.78%, 96.51%, 3.21 × 10⁴ yuan·t^–1, 779 yuan·GJ^–1, 1.49, and 71.02%, respectively.

关键词： energy analysis economic analysis microwave-assisted pyrolysis polystyrene aviation oil

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Cultivars and oil extraction techniques affect Cd/Pb contents and health risks in oil of rapeseed grown

《环境科学与工程前沿（英文）》 2023年第17卷第7期 doi: 10.1007/s11783-023-1687-z

摘要：

● Organic solvent extracted fewer Cd/Pb in rapeseed oil than physical pressing.

关键词： Rapeseed oil Oil extraction technologies Human health risk assessment Cd/Pb-contaminated farmland Substitute planting

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创新石油与战略思考

康玉柱

《中国工程科学》 2012年第14卷第3期页码 37-40

摘要：

中国油气勘探开发的历史，就是开拓创新的历史。这段历史取得了辉煌的成就，实现了陆相和海相油气勘探两大跨越。自主创新了八大油气地质理论和八大技术系列，发现500多个油气田，2010年产油达2.1×108 t油当量，天然气950×108 m3。从近期研究和实践认为，中国油气资源十分丰富，勘探潜力巨大，勘探领域广泛，并提出了油气资源开发的战略。

关键词：油气田油气资源油气资源潜力油气勘探战略

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Influence of different oil feed rate on bituminous coal ignition in a full-scale tiny-oil ignition burner

Chunlong LIU, Qunyi ZHU, Zhengqi LI, Qiudong ZONG, Xiang ZHANG, Zhichao CHEN

《能源前沿（英文）》 2013年第7卷第3期页码 406-412 doi: 10.1007/s11708-013-0266-6

摘要： To reduce oil consumption during firing-up and partial-load operation, a tiny-oil ignition burner has been recommended. Through reacting-flow experiments performed on a full-scale experimental setup, the influence of different oil flow rates on bituminous coal combustion as well as flow rates without coal feed was analyzed. The ignition burner is identical to that normally used in an 800 MWe utility boiler. Under operating conditions with flow rates of 50, 100, and 150 kg/h, gas temperature distributions were measured in the burner. At the equivalent measuring points at the exits of the first and second combustion chambers, these distributions remained almost unchanged under a constant coal feed rate of 4 t/h. However on the burner centerline, distributions increased slightly with increasing flow rate. Different gas concentrations were measured at the center of the burner exit. For instance, the O concentration at the burner exit varied from 0.01% to 0.31% whereas CO concentrations were more than 10000 ppm. At the same coal feed rate of 4 t/h, burner resistances are 480, 600, and 740 Pa for oil flow rates of 50, 100, and 150 kg/h, respectively.

关键词： ignition coal burner boiler oil flow rate

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世界油气上游国际合作的形势和机会

童晓光

《中国工程科学》 2011年第13卷第4期页码 15-19

摘要：

指出中国利用国外油气的必要性，重点分析了伊拉克、伊朗、巴西、加拿大、委内瑞拉和北美油气上游合作的机会及世界油气国际合作的合同变化趋势，提出了当前扩大油气上游国际合作的主要方向。

关键词：油气上游国际合作伊拉克深水油气勘探重油和油砂非常规天然气

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Mesoporous zeolites as efficient catalysts for oil refining and natural gas conversion

Jie ZHU, Xiangju MENG, Fengshou XIAO

《化学科学与工程前沿（英文）》 2013年第7卷第2期页码 233-248 doi: 10.1007/s11705-013-1329-2

摘要： Zeolites have been regarded as one of the most important catalysts in petrochemical industry due to their excellent catalytic performance. However, the sole micropores in zeolites severely limit their applications in oil refining and natural gas conversion. To solve the problem, mesoporous zeolites have been prepared by introducing mesopores into the zeolite crystals in recent years, and thus have the advantages of both mesostructured materials (fast diffusion and accessible for bulky molecules) and microporous zeolite crystals (strong acidity and high hydrothermal stability). In this review, after giving a brief introduction to preparation, structure, and characterization of mesoporous zeolites, we systematically summarize catalytic applications of these mesoporous zeolites as efficient catalysts in oil refining and natural gas conversion including catalytic cracking of heavy oil, alkylation, isomerization, hydrogenation, hydrodesulfurization, methane dehydroaromatization, methanol dehydration to dimethyl ether, methanol to olefins, and methanol to hydrocarbons.

关键词： mesoporous zeolite catalysis oil refining natural gas conversion

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properties of a silver particle-coated and 1-dodecanethiol-modified superhydrophobic melamine sponge for oil

《化学科学与工程前沿（英文）》 2022年第16卷第8期页码 1237-1246 doi: 10.1007/s11705-022-2140-8

摘要： A Ag particle-coated and 1-dodecanethiol-modified melamine sponge (Ag-DDT-MS) was prepared through surface roughness by coating silver particles and subsequent grafting of a hydrophobic long hydrocarbon chain. Superhydrophobic and 3D porous Ag-DDT-MS was characterized by Fourier transform infrared spectroscopy, scanning electron microscope, energy-dispersive X-ray spectroscopy, and X-ray diffraction. The water contact angle of Ag-DDT-MS reached 159.2°. Ag-DDT-MS exhibited excellent absorption capacity for high viscous oils and organic solvents, ranging from 42.8 to 105.2 g∙g⁻¹. The absorbed oils can be easily collected by the mechanical pressing process, and the oil recovery rate was satisfactory, more than 90% after 20 recycles. Ag-DDT-MS material also demonstrated good stability and excellent compression-recovery ability, keeping 88.6% of the initial height after ten compression-release cycles.

关键词： melamine sponge oil-absorbing material hydrophobic oil-water separation oil absorption capacity

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Catalytic hydrodeoxygenation of pyrolysis bio-oil to jet fuel: A review

《能源前沿（英文）》 doi: 10.1007/s11708-024-0943-7

摘要： Bio-oil from biomass pyrolysis cannot directly substitute traditional fuel due to compositional deficiencies. Catalytic hydrodeoxygenation (HDO) is the critical and efficient step to upgrade crude bio-oil to high-quality bio-jet fuel by lowering the oxygen content and increasing the heating value. However, the hydrocracking reaction tends to reduce the liquid yield and increase the gas yield, causing carbon loss and producing hydrocarbons with a short carbon-chain. To obtain high-yield bio-jet fuel, the elucidation of the conversion process of biomass catalytic HDO is important in providing guidance for metal catalyst design and optimization of reaction conditions. Considering the complexity of crude bio-oil, this review aimed to investigate the catalytic HDO pathways with model compounds that present typical bio-oil components. First, it provided a comprehensive summary of the impact of physical and electronic structures of both noble and non-noble metals that include monometallic and bimetallic supported catalysts on regulating the conversion pathways and resulting product selectivity. The subsequent first principle calculations further corroborated reaction pathways of model compounds in atom-level on different catalyst surfaces with the experiments above and illustrated the favored C–O/C=O scission orders thermodynamically and kinetically. Then, it discussed hydrogenation effects of different H-donors (such as hydrogen and methane) and catalysts deactivation for economical and industrial consideration. Based on the descriptions above and recent researches, it also elaborated on catalytic HDO of biomass and bio-oil with multi-functional catalysts. Finally, it presented the challenges and future prospective of biomass catalytic HDO.

关键词： biomass pyrolysis oil bio-jet fuel catalytic hydrodeoxygenation (HDO) metal catalyst reaction pathways

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Simulate oil spill weathering with system dynamic model

Aihaiti KASIMU, Junran DONG, Yuan BIAN, Desheng WU

《工程管理前沿（英文）》 2022年第9卷第4期页码 696-696 doi: 10.1007/s42524-019-0060-1

摘要： Numerous oil spill fate and trajectory models have been recently developed to predict oil spill weathering processes. However, these models separately predicted the fate of spilled oil and the change in oil properties. A system dynamic model is thus developed based on the most significant oil weathering processes, which include spreading, evaporation, dispersion into the water bulk, emulsification, and changes in viscosity and density. We employ differential equations to describe these main oil weathering processes, which vary and have different effects on each other. Oil density and viscosity are functions of evaporation and emulsification and change over time. Oil evaporation is the most important process and removes most of the spilled oil from sea surface. Considering the main oil weathering processes, our model provides a different method of predicting the fate of oil and changes in oil properties. The Alaska North Slope is selected as a case study, and the estimated fractions of evaporation are 19% and 16% at 273 K and 283 K, respectively, within 240 h. Simulation results of oil properties and fates are also presented in this study.

关键词： oil spill weathering modeling system dynamics

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Kinetic study of hydrodesulfurization of coker gas oil in a slurry reactor

Haiding XIANG, Tiefeng WANG

《化学科学与工程前沿（英文）》 2013年第7卷第2期页码 139-144 doi: 10.1007/s11705-013-1323-8

摘要： Coker gas oil (CGO) is a poor-quality feedstock for fluidized bed catalytic cracking (FCC) or hydrocracking. The pretreatment of CGO, especially hydrotreating, can significantly improve the product quality and protect the catalyst. In this work, we studied the hydrodesulfurization (HDS) of CGO in a slurry reactor. All the experiments were carried out in an autoclave using a NiMo/Al O catalyst at reaction temperature 340°C–400°C, pressure 6–10 MPa, and stirring speed 800 r·min , with hydrogen-to-oil ratio in the range of 500–1500. The effects of the operating parameters on the desulfurization ratio were investigated and discussed. A macro reaction kinetic model was established for the HDS of CGO in the slurry reactor.

关键词： coker gas oil hydrodesulfurization slurry reactor reaction kinetic model

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Highly hydrophobic oil−water separation membrane: reutilization of waste reverse osmosis membrane

《化学科学与工程前沿（英文）》 2023年第17卷第10期页码 1606-1615 doi: 10.1007/s11705-022-2200-0

摘要： The increasing applications of seawater desalination technology have led to the wide usage of polyamide reverse osmosis membranes, resulting in a large number of wasted reverse osmosis membranes. In this work, the base nonwoven layer of the wasted reverse osmosis membrane was successfully modified into the hydrophobic membrane via surface deposition strategy including TiO₂ and 1H,1H,2H,2H-perfluorooctyltrichlorosilane (PFOTS), respectively. Various techniques were applied to characterize the obtained membranes, which were then used to separate the oil–water system. The optimally modified membrane displayed good hydrophobicity with a contact angle of 135.2° ± 0.3°, and its oil–water separation performance was as high as 97.8%. After 20 recycle tests, the oil–water separation performance remained more than 96%, which was attributed to the film adhesion of the anchored TiO₂ and PFOTS layer on the surface. This work might provide a new avenue for recycling the wasted reverse osmosis membrane used in oily wastewater purification.

关键词： oil–water separation wasted reverse osmosis membrane hydrophobic modification

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全球主要盆地油气分布规律

康玉柱

《中国工程科学》 2014年第16卷第8期页码 14-25

摘要：

全球发育的含油气盆地有上千个，根据盆地结构特征可将含油气盆地分为3 大类型：克拉通盆地、断陷盆地和前陆盆地。笔者按这3 大类型盆地论述其油气分布规律。克拉通盆地：油汽主要分布在盆地内的古隆起、古斜坡，区域性的不整合及断裂带内；断陷盆地：油气主要分布在深凹带内的构造带、陡坡带和缓坡带；前陆盆地：油气主要分布在前陆断摺带、斜坡带、逆埯带及坳陷帶。这些规律性的认识，对全球油气勘探工作具有重要的指导意义。

关键词：含油气盆地油气田油气分布规律

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标题作者时间类型操作

The innovation and practice of shale oil development system engineering management based on dialecticalrelationships: A case study of Gulong shale oil in Daqing oilfield

期刊论文

Biodegradable, superhydrophobic walnut wood membrane for the separation of oil/water mixtures

期刊论文

Co-hydrotreating light cycle oil-canola oil blends

Huali WANG, Hena FAROOQI, Jinwen CHEN

期刊论文

Microwave-assisted pyrolysis of plastics for aviation oil production: energy and economic analyses

期刊论文

Cultivars and oil extraction techniques affect Cd/Pb contents and health risks in oil of rapeseed grown

期刊论文

创新石油与战略思考

康玉柱