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Adsorption and partition of benzo(a)pyrene on sediments with different particle sizes from the Yellow

XIA Xinghui, HU Lijuan, MENG Lihong

《环境科学与工程前沿(英文)》 2007年 第1卷 第2期   页码 172-178 doi: 10.1007/s11783-007-0030-4

摘要: Experiments have been carried out to study the sorption of Benzo(a)pyrene(Bap) on sediment particles from the Yellow River using a batch equilibration technique. Effects of particle size on the adsorption and partition of Bap were investigated with the particle content of 3 g/L. Several significant results were obtained from the study. (1) Isotherms of Bap could be fitted with the dual adsorption-partition model under different particle sizes, and the measured value of the adsorption and partition was in agreement with the theoretical value of the dual adsorption-partition model. (2) When the particle diameter was "e 0.025 mm, the adsorption was predominant in the sorption of Bap, which accounted for 68.7% 82.4% of the sorption. For the particles with the size of 0.007 mm "e < 0.025 mm, the adsorption was predominant when the equilibrium concentration of Bap was 0 8.87 μg/L in the water phase; and the partition was predominant when the equilibrium concentration of Bap was higher than 8.87 μg/L in the water phase. When the particle diameter was <0.007 mm, the partition was predominant. (3) On the point of particle size, the contribution of adsorption to sorption followed the order: "e0.025 mm > 0.007 mm "d<0.025 mm > <0.007 mm . (4) The partition coefficients of Bap in solids with different particle sizes were linearly correlated with the organic content, and the K of Bap was about 1.26 x 10 (L/kg).

Prediction of bed load sediments using different artificial neural network models

Reza ASHEGHI, Seyed Abbas HOSSEINI

《结构与土木工程前沿(英文)》 2020年 第14卷 第2期   页码 374-386 doi: 10.1007/s11709-019-0600-0

摘要: Modeling and prediction of bed loads is an important but difficult issue in river engineering. The introduced empirical equations due to restricted applicability even in similar conditions provide different accuracies with each other and measured data. In this paper, three different artificial neural networks (ANNs) including multilayer percepterons, radial based function (RBF), and generalized feed forward neural network using five dominant parameters of bed load transport formulas for the Main Fork Red River in Idaho-USA were developed. The optimum models were found through 102 data sets of flow discharge, flow velocity, water surface slopes, flow depth, and mean grain size. The deficiency of empirical equations for this river by conducted comparison between measured and predicted values was approved where the ANN models presented more consistence and closer estimation to observed data. The coefficient of determination between measured and predicted values for empirical equations varied from 0.10 to 0.21 against the 0.93 to 0.98 in ANN models. The accuracy performance of all models was evaluated and interpreted using different statistical error criteria, analytical graphs and confusion matrixes. Although the ANN models predicted compatible outputs but the RBF with 79% correct classification rate corresponding to 0.191 network error was outperform than others.

关键词: bed load prediction     artificial neural network     modeling     empirical equations    

Sorption of tetracycline to sediments and soils: assessing the roles of pH, the presence of cadmium andproperties of sediments and soils

Guixiang ZHANG, Xitao LIU, Ke SUN, Ye ZHAO, Chunye LIN

《环境科学与工程前沿(英文)》 2010年 第4卷 第4期   页码 421-429 doi: 10.1007/s11783-010-0265-3

摘要: Batch sorption experiments were conducted to evaluate the sorption behavior of tetracycline (TC, H L) on sediments and soils in the presence and absence of cadmium (Cd), as affected by pH and properties of sediments and soils. The results indicated stronger nonlinearity and higher capacity of TC sorption on sediments than on soils. Sorption of TC also strongly depended on environmental factors and sediment/soil properties. Lower pH facilitated TC sorption through a cation exchange mechanism, which also took place at pH values above 5.5, where TC existed as a zwitterion (H L ) or anions (HL and L ). When pH was above 7, however, ligand-promoted dissolution of TC might occur due to TC weakening the Al-O bond of aluminum oxide and the Fe-O bond of iron oxide. Natural organic matter (NOM) plays a more important role in TC sorption than cation exchange capacity (CEC) and clay contents. The presence of Cd (II) increased TC sorption on both sediments and soils, which resulted from the decrease of equilibrium solution pH caused by Cd exchange with H ions of sediment/soil surfaces. The increase of TC sorption was also related to the formation of TC-Cd complexes, where Cd acted as a bridge between the sediment/soil and TC.

关键词: sorption     tetracycline (TC)     pH     cadmium (Cd)     antibiotic    

Assessment on contaminations in sediments of an intake and the inflow canals in Taihu Lake, China

Xiaolong WANG,Shiming DING,Qi ZHANG,Weiping HU

《环境科学与工程前沿(英文)》 2015年 第9卷 第4期   页码 665-674 doi: 10.1007/s11783-014-0701-x

摘要: As the second largest freshwater lake in China, Taihu Lake provides water supply to approximately 32 million inhabitants around the lake. However, dramatically increased pollution has threatened the safety of drinking water supply in recent years. In the present study, we investigated the contaminations of nutrients and heavy metals in the sediments of an intake and inflow canals in Gonghu Bay, Taihu Lake. Moreover, we also examined the impact of human activities on spatial distribution characteristics of contaminations. Our results showed that the intake presented relatively lower concentrations of phosphorus and nitrogen compared with inflow canals. However, the concentrations of Cr, Ni, Cu, Zn and Pb in the sediments of the intake exceeded the lowest effect level (LEL) values, indicating a potential risk to drinking water resource. In addition, the concentrations of Ni in the sediments of Tianji Canal and Jinshu Canal exceeded the severe effect level (SEL) value. More importantly, the concentrations of Cu in the sediments of Tianji Canal exceeded three times of the SEL value. Multivariate statistical analysis confirmed that the domestic sewage primarily contributed to the nutrient accumulation, and the leakage of electronic trash dominated the enrichment of metals in the sediments. Taken together, more effort should be made to ensure the security of water resources in Taihu Lake, especially for the treatment of domestic sewage and industrial wastewater.

关键词: drinking water resource     nutrients     heavy metals     sediments     Taihu Lake    

The temporal changes of the concentration level of typical toxic organics in the river sediments around

Qiang Li, Xiong Xu, Yaoyao Fang, Ruiyang Xiao, Donghong Wang, Wenjue Zhong

《环境科学与工程前沿(英文)》 2018年 第12卷 第6期 doi: 10.1007/s11783-018-1054-7

摘要:

The current situation of typical organics in the sediments around Beijing was unclear.

56 kinds of typical toxic organics were detected in this article.

Historical data was compared with the data in this study.

The change of different organics in the sediments around Beijing was concluded.

关键词: Organic compounds     Endocrine disrupters     Sediments     Concentration     Temporal changes    

Recent advances in pharmaceuticals and personal care products in the surface water and sediments in China

Wentao Zhao, Ying Guo, Shuguang Lu, Pingping Yan, Qian Sui

《环境科学与工程前沿(英文)》 2016年 第10卷 第6期 doi: 10.1007/s11783-016-0868-4

摘要: Recent publications on PPCPs in surface water environment in China were reviewed. Antibiotics received more attention than other PPCPs in surface water environment. Uneven attention has been focused across different study areas in China. Sulfamethoxazole showed the most significant environmental risk in surface water. Higher risks were posed by PPCPs in sediments than in surface water. Pharmaceuticals and personal care products (PPCPs) have been regarded as an emerging problem in the surface water environment in the past few decades. In China, although related studies were initiated several years ago, an increasing number of studies on this topic have been conducted in recent years. These studies have expanded knowledge of their occurrence, behavior and associated risk in the surface water environment in China. This review compiles the most recent literature related to the studies of PPCPs in the surface water environment in China. It includes PPCP occurrence in surface water and sediments, their geographical distribution, and outcomes of the associated risk assessment. It shows that antibiotics have received much more attention in both surface water and sediments than other PPCPs. Compared to other countries; most antibiotics in the collected sediments in China showed higher contamination levels. Many more study areas have been covered in recent years; however, attention has been given to only specific areas. Environmental risk assessment based on risk quotients indicated that sulfamethoxazole presents the most significant environmental risk to relevant aquatic organisms; followed by ofloxacin, ciprofloxacin, enrofloxacin, 17α-ethynylestradiol, ibuprofen and diclofenac. Despite limited research on the environmental risk assessment of PPCPs in sediments, higher risks posed by PPCPs in the sediments rather than surface water were identified highlighting the need for further risk assessment of PPCPs in sediment samples.

关键词: Surface water     Sediment     Antibiotics     Geographical distribution     Risk assessment    

Sulfur mediated heavy metal biogeochemical cycles in coastal wetlands: From sediments, rhizosphere to

《环境科学与工程前沿(英文)》 2022年 第16卷 第8期 doi: 10.1007/s11783-022-1523-x

摘要:

• In sediments, the transformation of sulfides may lead to the release of heavy metals.

关键词: Coastal wetland     Heavy metal     Sulfur     Biogeochemical cycle    

Species distribution of arsenic in sediments after an unexpected emergent discharge of high-arsenic wastewater

Ruiping LIU, Wei XU, Kun WU, Wenxin GONG, Huijuan LIU, Jiuhui QU

《环境科学与工程前沿(英文)》 2013年 第7卷 第4期   页码 568-578 doi: 10.1007/s11783-013-0514-3

摘要: The unexpected emergent discharge of high-arsenic wastewater into water environments results in significantly increased levels of arsenic in water; however, the species distribution of arsenic in sediments has never been reported before for such cases. This study focuses on an As pollution accident in the Dasha River, and uses sequential extraction procedures with deionized water, 1?mol·L MgCl at pH= 8, 1?mol·L NaH PO at pH= 5, and 1?mol·L HCl to investigate four binding phases of arsenic (i.e., water soluble, ion-exchangeable, strongly-bound, and precipitates) in sediments at different layers in different cross-sections along the river. The average ratio of arsenite (As(III)) to arsenate (As(V)) was found to decrease from 0.74:1 in river water to 0.48:1 in sediment, owing to its higher affinity toward As(V) than As(III). The content of arsenic in the sediments was relatively low and the maximum content was observed to be 36.3?mg·kg for As(III) and 97.5?mg·kg for As(V). As(III) and As(V) showed different binding phases in sediments, and the average fractions of these four species were determined to be 0.09, 0.11, 0.17, and 0.63 for As(III) and 0.03, 0.14, 0.63, and 0.20 for As(V), respectively. For all the sediment samples, the content of arsenic showed no relationship with the characteristics of the sediments such as the particle diameter, the content of organic carbon, Fe, and Mn, although a negative correlation with particle diameter was observed for the sediments in the uppermost 2-cm layer. The unexpected emergent As incident results in the high content of total arsenic in the surface sediment, which may be potential secondary source to the elevated As levels in surface water.

关键词: river sediments     arsenic     species distribution     binding phases     unexpected discharge of high-As wastewater    

Characterization of phosphorus species and modeling for its organic forms in eutrophic shallow lake sediments

Hongguang CHENG,Xiao PU,Yiting CHEN,Fanghua HAO,Liming DONG

《环境科学与工程前沿(英文)》 2014年 第8卷 第6期   页码 905-921 doi: 10.1007/s11783-014-0650-4

摘要: Variations of phosphorus (P) and its species in surface sediment of Baiyangdian Lake, a eutrophic shallow lake located in North China, were investigated through combination of field survey and numerical calculation based on cluster analysis. P fractionation was performed by a sequential extraction scheme, categorized as loosely bound P (NH Cl-P), reductant soluble P (BD-P), metallic oxide bound P (NaOH-P), calcium bound P (HCl-P) and organic P (Org-P). P concentrations exhibited regional similarities and a total of four sub-areas were identified in which the same rank was HCl-P>Org-P>BD-P ≈ NaOH-P>NH Cl-P. NH Cl-P, BD-P and Org-P were found to contribute to P enrichment in overlying water column. Specifically, labile Org-P acted as a potential pool with a greater contribution in aerobic layer compared to anaerobic layer. A hysteresis (lag= 4 months) existed when labile Org-P concentration was negatively correlated with aerobic layer thickness. In view of magnitude of identified P contributors in sub-areas, higher potential of P release was present in Fuhe River and Tang River estuary areas. On the basis of calibration and verification, the mathematical model with parameter settings applied in this study was improved to serve as a tool for limnology management and eutrophic control.

关键词: phosphorus fractionation     variation characteristics     modeling     sediment     Baiyangdian Lake    

Transferral of HMs pollution from road-deposited sediments to stormwater runoff during transport processes

Qian Wang, Qionghua Zhang, Mawuli Dzakpasu, Nini Chang, Xiaochang Wang

《环境科学与工程前沿(英文)》 2019年 第13卷 第1期 doi: 10.1007/s11783-019-1091-x

摘要:

Ratio of turbidity and TSS (Tur/TSS) was used to characterize PSD of stormwater particles.

Pb and Zn preferred to accumulate in finer RDS, while Cu, Cr and Ni in coarser RDS.

HMs pollution in stormwater particles increased linearly with Tur/TSS.

Dissolvability of HMs and PSD variations contribute to the differences between RDS and stormwater.

关键词: Road-deposited sediment     Stormwater runoff     Heavy metal     Particle size     Pollution variation    

Phenanthrene sorption to environmental black carbon in sediments from the Song-Liao watershed (China)

Jinghuan ZHANG, Mengchang HE, Chunye LIN, Ke SUN, Bin MEN, John L. ZHOU,

《环境科学与工程前沿(英文)》 2009年 第3卷 第4期   页码 434-442 doi: 10.1007/s11783-009-0150-0

摘要: Black carbon (BC) in ten contaminated sediments from the Song-Liao watershed, NE China, was isolated upon treatments using a combustion method at 375°C, and the isolates’ sorption isotherms for phenanthrene (Phen) were determined. All sorption isotherms were nonlinear and fitted well by the Freundlich model. A negative relation was found between Freundlich sorption nonlinearity parameter ( values) and BC/total organic carbon (TOC) content of the original sediments (=0.687, <0.01), indicating the dominance of BC in Phen sorption nonlinearity. The BC isolates from this industrialized region had values of 0.342 to 0.505 and log values of 6.02 to 6.42(μg·kg·OC)/(μg·L) for Phen. At a given , the BC had higher value than the original sediments, revealing a higher sorption capacity for BC. BC was responsible for 50.0% to 87.3% of the total sorption at =0.05 , clearly indicating the dominance of BC particles in overall sorption of Phen by sediments.

关键词: phenanthrene     sorption     black carbon     sediment     Song-Liao watershed    

Different response of bacterial community to the changes of nutrients and pollutants in sediments from

Fang Zhang, Hao Zhang, Ying Yuan, Dun Liu, Chenyu Zhu, Di Zheng, Guanghe Li, Yuquan Wei, Dan Sun

《环境科学与工程前沿(英文)》 2020年 第14卷 第2期 doi: 10.1007/s11783-019-1207-3

摘要: • Bacterial community varied spatially in sediments from the urban river network. • Key environmental factors shaping bacterial community were detected by RDA. • Bacterial co-occurrence networks changed at different levels of nutrient and metal. • Potential indicator species were selected to predict pollution risk in sediment. Microbial communities in sediment are an important indicator linking to environmental pollution in urban river systems. However, how the diversity and structure of bacterial communities in sediments from an urban river network respond to different environmental factors has not been well studied. The goal of this study was to understand the patterns of bacterial communities in sediments from a highly dense urbanized river network in the lower Yangtze River Delta by Illumina MiSeq sequencing. The correlations between bacterial communities, the environmental gradient and geographical distance were analyzed by redundancy analysis (RDA) and network methods. The diversity and richness of bacterial community in sediments increased from upstream to downstream consistently with the accumulation of nutrient in the urban river network. Bacterial community composition and structure showed obvious spatial changes, leading to two distinct groups, which were significantly related to the characteristics of nutrient and heavy metal in sediments. Humic substance, available nitrogen, available phosphorus, Zn, Cu, Hg and As were selected as the key environmental factors shaping the bacterial community in sediments based on RDA. The co-occurrence patterns of bacterial networks showed that positive interaction between bacterial communities increased but the connectivity among bacterial genera and stability of sediment ecosystem reduced under a higher content of nutrient and heavy metal in average. The sensitive and ubiquitous taxa with an overproportional response to key environmental factors were detected as indicator species, which provided a novel method for the prediction of the pollution risk of sediment in an urban river network.

关键词: Sediment     Urban river network     Bacterial community     Network analysis     Indicator species    

Spatial distribution of phosphorus forms in sediments with different distances to the estuary of the

Shaoyong LU, Xiangcan JIN, Fengchang WU, Jing SI, Jianning GUO,

《环境科学与工程前沿(英文)》 2010年 第4卷 第3期   页码 295-300 doi: 10.1007/s11783-010-0231-0

摘要: Effects of human activity on the distribution of phosphorus (P) forms were investigated for the sediments and porewaters in Daqinghe Estuary of Dianchi Lake, China. The concentrations of total P (TP), inorganic-P (I-P), and organic-P (Org-P), and the ratio of iron-bound P (Fe-P)/calcium-bound P (Ca-P) in the sediments decreased with the increasing distance from the sampling site to the estuary. This is probably due to the flocculant materials, e.g., ferric and aluminous salts, usually being added in the wastewater treatment processes. The concentration of ammonia in the sediment porewaters significantly decreased with the increasing distance from the sampling site to the estuary. Both concentrations of total nitrogen and nitrogen in the sediment porewaters decreased to some content with the increasing distance from the sampling site to the estuary. However, the concentrations of nitrate, dissolved total P (DTP), and TP did not have strong relationship with the distances from the sampling sites to the estuary. Pollution load and water quantity also had an important influence on the concentrations of P in sediments and its interstitial water in estuary sedimentary area.

关键词: estuary sedimentary area     phosphorus (P)     spatial distribution     human activity     the Dianchi Lake    

Analysis and assessment of heavy metal contamination in surface water and sediments: a case study from

Zhaoming WANG,Ranhao SUN,Haiping ZHANG,Liding CHEN

《环境科学与工程前沿(英文)》 2015年 第9卷 第2期   页码 240-249 doi: 10.1007/s11783-014-0646-0

摘要: Concentrations of the heavy metals Cu, Ni, Pb, Zn, Cd, and Cr were examined in surface water and sediment from the Luan River inChina,. With a decline in Cu and Ni concentration found in surface water at downstream stations. This finding suggests that water currents are a major explanatory factor in heavy metal contamination. The abundance of Cr, Pb, and Cd observed in the middle reaches of the river indicates heavy metal contamination in local areas, although there was an obvious decrease in concentrations in the water downstream of the Daheiting Reservoir. The significant rising trend in Cu, Pb, and Ni seen the sediment farther away from the river also suggests that anthropogenic activities contribute to heavy metal pollution Sediments were therefore used as environmental indicators, with sediment assessment was conducted using the geo-accumulation index ( ) and the potential ecological risk index ( ). The values revealed that Cd (3.13) and Cr (2.39) had accumulated significantly in the Luan River. The values for most (89%) of the sampling stations were higher than 300, suggesting that sediment from the Luan River poses a severe ecological risk, with the potential ecological risks downstream higher than that in the upper and middle streams. Good correlations among Pb/Ni, Pb/Cd, Cu/Pb, and Cu/Cd in the water and Cr/Ni in the sediment were observed. Cluster analysis suggested that Cd may have various origins, being derived from anthropogenic sources.

关键词: heavy metal     water     sediment     geo-accumulation index     Luan River    

Fundamental characteristics of gas hydrate-bearing sediments in the Shenhu area, South China Sea

Xin LYU, Qingping LI, Yang GE, Junlong ZHU, Shouwei ZHOU, Qiang FU

《能源前沿(英文)》 2021年 第15卷 第2期   页码 367-373 doi: 10.1007/s11708-020-0714-z

摘要: The basic physical properties of marine natural gas hydrate deposits are important to the understanding of seabed growth conditions, occurrence regularity, and occurrence environment of natural gas hydrates. A comprehensive analysis of the core samples of drilling pressure-holding hydrate deposits at a depth of 1310 m in the Shenhu area of the South China Sea was conducted. The experimental results indicate that the particle size in the hydrate sediment samples are mainly distributed in the range from 7.81 µm to 21.72µm, and the average particle size decreases as the depth of the burial increases. The X-ray CT analytical images and surface characteristics SEM scan images suggest that the sediment is mostly silty clay. There are a large number of bioplastics in the sediment, and the crack inside the core may be areas of hydrate formation.

关键词: natural gas hydrate     Shenhu area     reservoirs characteristics    

标题 作者 时间 类型 操作

Adsorption and partition of benzo(a)pyrene on sediments with different particle sizes from the Yellow

XIA Xinghui, HU Lijuan, MENG Lihong

期刊论文

Prediction of bed load sediments using different artificial neural network models

Reza ASHEGHI, Seyed Abbas HOSSEINI

期刊论文

Sorption of tetracycline to sediments and soils: assessing the roles of pH, the presence of cadmium andproperties of sediments and soils

Guixiang ZHANG, Xitao LIU, Ke SUN, Ye ZHAO, Chunye LIN

期刊论文

Assessment on contaminations in sediments of an intake and the inflow canals in Taihu Lake, China

Xiaolong WANG,Shiming DING,Qi ZHANG,Weiping HU

期刊论文

The temporal changes of the concentration level of typical toxic organics in the river sediments around

Qiang Li, Xiong Xu, Yaoyao Fang, Ruiyang Xiao, Donghong Wang, Wenjue Zhong

期刊论文

Recent advances in pharmaceuticals and personal care products in the surface water and sediments in China

Wentao Zhao, Ying Guo, Shuguang Lu, Pingping Yan, Qian Sui

期刊论文

Sulfur mediated heavy metal biogeochemical cycles in coastal wetlands: From sediments, rhizosphere to

期刊论文

Species distribution of arsenic in sediments after an unexpected emergent discharge of high-arsenic wastewater

Ruiping LIU, Wei XU, Kun WU, Wenxin GONG, Huijuan LIU, Jiuhui QU

期刊论文

Characterization of phosphorus species and modeling for its organic forms in eutrophic shallow lake sediments

Hongguang CHENG,Xiao PU,Yiting CHEN,Fanghua HAO,Liming DONG

期刊论文

Transferral of HMs pollution from road-deposited sediments to stormwater runoff during transport processes

Qian Wang, Qionghua Zhang, Mawuli Dzakpasu, Nini Chang, Xiaochang Wang

期刊论文

Phenanthrene sorption to environmental black carbon in sediments from the Song-Liao watershed (China)

Jinghuan ZHANG, Mengchang HE, Chunye LIN, Ke SUN, Bin MEN, John L. ZHOU,

期刊论文

Different response of bacterial community to the changes of nutrients and pollutants in sediments from

Fang Zhang, Hao Zhang, Ying Yuan, Dun Liu, Chenyu Zhu, Di Zheng, Guanghe Li, Yuquan Wei, Dan Sun

期刊论文

Spatial distribution of phosphorus forms in sediments with different distances to the estuary of the

Shaoyong LU, Xiangcan JIN, Fengchang WU, Jing SI, Jianning GUO,

期刊论文

Analysis and assessment of heavy metal contamination in surface water and sediments: a case study from

Zhaoming WANG,Ranhao SUN,Haiping ZHANG,Liding CHEN

期刊论文

Fundamental characteristics of gas hydrate-bearing sediments in the Shenhu area, South China Sea

Xin LYU, Qingping LI, Yang GE, Junlong ZHU, Shouwei ZHOU, Qiang FU

期刊论文