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Removal of dyes from wastewater by growing fungal pellets in a semi-continuous mode

Tao Lu, Qilei Zhang, Shanjing Yao

《化学科学与工程前沿（英文）》 2017年第11卷第3期页码 338-345 doi: 10.1007/s11705-017-1644-0

摘要： To increase the efficiency of dye removal from wastewater using mycelial pellets, a bubble column reactor with a simple structure was designed and efficiently used to remove dyes from solution containing dyes. The mycelial pellets were prepared by marine fungus ZJUBE-1. Eight dyes were tested as dye targets for the adsorption capacity of mycelial pellets and good removal results were obtained. Eriochrome black T was selected as a model dye for characterizing the adsorption processes in detail. The measurement results of Zeta potential and FT-IR analysis indicate that the electrostatic attraction may play a key role in the biosorption process. The bubble column reactor was utilized to study the batch dye-removal efficiency of mycelial pellets. A re-culture process between every two batches, which was under non-sterile condition, successfully enhanced the utilization of mycelium biomass. The dye removal rate is 96.4% after 12 h in the first batch and then decreases slowly in the following batches. This semi-continuous mode, which consists of commutative processes of dye-removal and re-culture, has some outstanding advantages, such as low power consumption, easy operation, high dye removal rate, and efficient biomass utilization.

关键词： dye mycelial pellets marine fungus bubble column reactor semi-continuous biosorption

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Bending and rotational behaviour of semi-continuous composite beams

WANG Jingfeng, LI Guoqiang

《结构与土木工程前沿（英文）》 2008年第2卷第2期页码 116-122 doi: 10.1007/s11709-008-0015-9

摘要： Stresses and deflections were measured in various semi-continuous composite beams. The bending and rotational capacities of the composite connections were measured in terms of beam curvatures and deflections by using two full-scale semi-rigid composite frames with monotonic loadings. The effect of semi-rigid connections on the performance of composite beams with various loadings was compared with predictions and codes. The tests show that the semi-continuous composite beams are more economic and effective than the simple or continuous composite beams. The semi-rigid connections affect the bending capacities and beam deflections, so the connection behavior should be considered in the design of composite beams. Yielding analysis of the steel beam bottom flange has some influence on the deflection calculation of composite beams.

关键词： rotational effective deflection calculation semi-continuous composite full-scale semi-rigid

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Biosorption of Cu(II) to extracellular polymeric substances (EPS) from

Xiangliang PAN, Jing LIU, Wenjuan SONG, Daoyong ZHANG

《环境科学与工程前沿（英文）》 2012年第6卷第4期页码 493-497 doi: 10.1007/s11783-012-0416-9

摘要： Biosorption of extracellular polymeric substances (EPS) from sp. (cyanobacterium) with Cu(II) was investigated using fluorescence spectroscopy. Three fluorescence peaks were found in the excitation-emission matrix (EEM) fluorescence spectra of EPS. Fluorescence of peak A (Ex/Em= 275/452 nm) and peak C (Ex/Em= 350/452 nm) were originated from humic-like substances and fluorescence of peak B (Ex/Em= 275/338 nm) was attributed to protein-like substances. Fluorescence of peaks A, B, and C could be quenched by Cu(II). The effective quenching constants (lg K ) were 2.8–5.84 for peak A, 6.4–9.24 for peak B, and 3.48–6.68 for peak C, respectively. The values of lg K showed a decreasing trend with increasing temperature, indicating that the quenching processes were static in nature. The binding constants (lg K ) followed the order of peak A>peak B>peak C, implying that the humic-like substances in EPS have greater Cu(II) binding capacity than the protein-like substances. The binding site number, , in EPS-Cu(II) complexes for peaks A, B, and C was less than 1. This suggests the negative cooperativity between multiple binding sites and the presence of more than one Cu binding site.

关键词： biosorption conditional binding constant extracellular polymeric substances (EPS) fluorescence quenching

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The biosorption of Cr(VI) ions by dried biomass obtained from a chromium-resistant bacterium

Paul Fabrice NGUEMA,Zejiao LUO,Jingjing LIAN

《化学科学与工程前沿（英文）》 2014年第8卷第4期页码 454-464 doi: 10.1007/s11705-014-1456-4

摘要： The biosorption potential of many different kinds of biomaterials has been widely studied. However, there is little data on the biosorption mechanism of Cr(VI) by dried biomass. So the bio-removal of Cr(VI) ions from aqueous solutions was investigated using dried biomass from a chromium-resistant bacterium. The bacterium was isolated from dewatered sludge samples that were obtained from a sewage treatment plant. Equilibrium and kinetic experiments were performed at different metal concentrations, pH values, and biosorbents dosages. The biomass was characterized using scanning electron microscopy and energy-dispersive X-ray spectroscopy. The functional groups in the biomass which may play a role in the biosorption process were identified by Fourier transform infrared spectroscopy. The biosorption process was found to be highly pH dependent and the optimum pH for the adsorption of Cr(VI) was 2.0±0.3 at 30±2 °C. The experimental data fit well with Langmuir and Freundlich models as well as a pseudo-second order kinetic model. The mechanism for the biosorption was also studied by fitting the kinetic data with an intra-particle diffusion model and a Boyd plot. External mass transfer was found to be the rate-determining step for the adsorption process. Biosorption could be an alternative mechanism besides bio-oxidation and bio-reduction for the bioremediation of heavy metals.

关键词： Cr(VI) biomass Bacillus cereus Pf-1 biosorption capacity biosorbents

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Biosorption of mercury and lead by aqueous

Pratibha SANJENBAM, Kumar SAURAV, Krishnan KANNABIRAN

《化学科学与工程前沿（英文）》 2012年第6卷第2期页码 198-202 doi: 10.1007/s11705-012-1285-2

摘要： Toxic heavy metals are increasingly accumulating in the environment worldwide and are considered to be life threatening contaminants. The biosorption of mercury and lead by marine actinomycetes isolated from marine sediment collected from the Bay of Bengal coast of Puducherry, India, was evaluated. The maximum tolerance concentration (MTC) of sp. was determined by a well diffusion method and a broth dilution method. The effects of the initial metal ion concentration, the pH and the biomass dosage on the biosorption of mercury and lead ions were investigated. The MTC of the isolate to metals was 200 mg·L for mercury and 1800 mg·L for lead. At neutral pH, the isolate had a maximum biosorption of metal ions of 200 mg·L and 150 mg·L for mercury and lead respectively. Fourier transform infrared (FTIR) absorption spectra showed the chemical interactions between the functional groups in the biomass such as hydroxyl (-OH), amine (-NH ), carboxyl (-COOH) and the metal ions. The isolate was further characterized by molecular taxonomy and identified as a member of the genus Based on the phenotypic and phylogenetic analysis, the strain was classified as a new species of the genus and designated as VITSVK9 sp. (HM137310). A blast search of the 16S rDNA sequence of the strain showed the most similarity (95%) with sp. A515 Ydz-FQ (EU384279). Based on the results, it can be concluded that this marine could be used as a biosorbent for the removal of heavy metal ions from aqueous environments.

关键词： mercury lead biosorption maximum tolerance concentration Streptomyces VITSVK9 sp.

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Biosorption and biotransformation of crystal violet by

Tao PAN, Suizhou REN, Jun GUO, Meiying XU, Guoping SUN

《环境科学与工程前沿（英文）》 2013年第7卷第2期页码 185-190 doi: 10.1007/s11783-012-0435-6

摘要： DN322p, an offspring of DN322, has the capacity to adsorb and decolorize triphenylmethane dyes in wastewater simultaneously. As a common triphenylmethane dye, crystal violet (CV) was chosen to test the decolorization characteristics of DN322p. Within 0.5 h, the strain DN322p adsorbed a large amount of CV, producing a deep-colored cell pellet and colorless supernatant. The colors of the cell pellet and supernatant lightened over time. The supernatant and dichloromethane extract of the cell pellet both showed conspicuous CV and leuco CV (LCV) characteristic absorbance peaks at 590 nm and 260 nm, respectively, in the UV-vis spectral analysis. This finding indicated that the DN322p cells can adsorb the two dyes. A 99% (w/w) decolorization rate was achieved within 2.5 h with shaking at 30°C for 50 mg CV·L . High Performance Liquid Chromatography (HPLC) analysis of the dichloromethane extract of the supernatant and cell pellet confirmed that CV was mainly converted into its leuco form. Dead cells had a similar adsorption capacity with living cells. About 90% of CV in the dye solution (50 mg·L ) was removed by autoclaved cells with an optical delnsity at 600 nm (OD ) above 1.0.

关键词： crystal violet decolorization biosorption biotransformation Aeromonas hydrophila DN322p

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Micromixing performance of the teethed high shear mixer under semi-batch operation

《化学科学与工程前沿（英文）》 2022年第16卷第4期页码 546-559 doi: 10.1007/s11705-021-2069-3

摘要： Semi-batch operated reaction processes are necessary for some competitive reaction systems to achieve a desirable process selectivity and productivity of fine chemical products. Herein the structural and operating parameters of the teethed high shear mixers were adjusted to study the micromixing performance in the semi-batch operated system, using the Villermaux/Dushman reaction system. The results indicate that the rising of the rotor speed and the number of rotor teeth, the decrease of the width of the shear gap and the radial distance between the feed position and the inner wall of stator can enhance the micromixing level and lead to the decrease of the segregation index. Additionally, computational fluid dynamics calculations were carried out to disclose the evolution of the flow pattern and turbulent energy dissipation rate of the semi-batch operated high shear mixer. Furthermore, the correlation was established with a mean relative error of 8.05% and R² of 0.955 to fit the segregation index and the parameters studied in this work, which can provide valuable guidance on the design and optimization of the semi-batch operated high shear mixers in practical applications.

关键词： high shear mixer semi-batch operation micromixing performance Villermaux/Dushman system segregation index

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Biosorption of Cd

Fengyu ZAN, Shouliang HUO, Beidou XI, Xiulan ZHAO

《环境科学与工程前沿（英文）》 2012年第6卷第1期页码 51-58 doi: 10.1007/s11783-011-0206-9

摘要： The biosorption of Cd and Cu onto the immobilized ( ) was investigated in this study. Adsorption kinetics, isotherms and the effect of pH were studied. The results indicated that the biosorption of Cd and Cu on the immobilized was fast at initial stage and then became slow. The maximum biosorption of heavy metal ions on immobilized were observed at pH 4 for Cd and Cu . by the pseudo-second-order model described the sorption kinetic data well according to the high correlation coefficient ( ) obtained. The biosorption isotherm was fitted well by the Langmuir model, indicating possible mono-layer biosorption of Cd and Cu on the immobilized . Moreover, the immobilized after the sorption of Cd and Cu could be regenerated and reused.

关键词： Saccharomyces cerevisiae (S. cerevisiae) biosorption heavy metals immobilization desorption

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Biosorption of Cr(VI) by carbonized

Jinfa CHEN,Ping YANG,Dagang SONG,Sha YANG,Li ZHOU,Lei HAN,Bo LAI

《环境科学与工程前沿（英文）》 2014年第8卷第6期页码 960-966 doi: 10.1007/s11783-013-0612-2

摘要： High quality and low cost carbon can be prepared from ( ) and Buckwheat straw. The biosorbent was used for Cr(VI) removal. The effect of experimental parameters, such as pH, sorbent dosage and temperature were examined and the optimal experimental condition was determined. Solution pH is found influencing the adsorption. Cr(VI) removal efficiency is found to be maximum (98%) at pH= 1. Langmuir and Freundlich adsorption isotherms were applicable to the adsorption process and their constants were evaluated. The adsorption data obtained agreed well with the Langmuir sorption isotherm model. The maximum adsorption capacities for Cr(VI) ranged from 46.23 to 55.19 mg·g for temperature between 298 K and 308 K under the condition of pH= 1.0. Thermodynamic parameters such as free energy change ( ), enthalpy ( ) and entropy ( ) indicate a spontaneous, endothermic and increased randomness nature of Cr(VI) adsorption. Studies found that the raw and buckwheat straw mixed materials with simple treatment had a high efficiency for the removal of Cr(VI) and would be a promising adsorbent.

关键词： Eupatorium adenophorum buckwheat straw adsorption Cr(VI) thermodynamics

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Ant colony optimization in continuous problem

YU Ling, LIU Kang, LI Kaishi

《机械工程前沿（英文）》 2007年第2卷第4期页码 459-462 doi: 10.1007/s11465-007-0079-6

摘要： Based on the analysis of the basic ant colony optimization and optimum problem in a continuous space, an ant colony optimization (ACO) for continuous problem is constructed and discussed. The algorithm is efficient and beneficial to the study of the ant colony optimization in a continuous space.

关键词： beneficial algorithm efficient continuous ACO

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Prediction of the theoretical and semi-empirical model of ambient temperature

Foued CHABANE,Noureddine MOUMMI,Abdelhafid BRIMA,Abdelhafid MOUMMI

《能源前沿（英文）》 2016年第10卷第3期页码 268-276 doi: 10.1007/s11708-016-0413-y

摘要： It is well known that the ambient temperature is a sensitive parameter which has a great effect on biology, technology, geology and even on human behavior. A prediction is a statement about an uncertain event. It is often, but not always, based upon experience or knowledge. Although guaranteed accurate information about the future is in many cases impossible, prediction can be useful to assist in making plans about possible developments. As a result, temperature profiles can be developed which accurately represent the expected ambient temperature exposure that this environment experiences during measurement. The ambient temperature over time is modeled based on the previous and data and using a Lagrange interpolation. To observe the comprehensive variation of ambient temperature the profile must be determined numerically. The model proposed in this paper can provide an acceptable way to measure the change in ambient temperature.

关键词： ambient temperature environment correlation theoretical model semi-empirical

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Cavitation in semi-open centrifugal impellers for a miniature pump

LUO Xianwu, LIU Shuhong, ZHANG Yao, XU Hongyuan

《能源前沿（英文）》 2008年第2卷第1期页码 31-35 doi: 10.1007/s11708-008-0011-8

摘要： Cavitation in miniature pumps was investigated experimentally for two semi-open centrifugal impellers. Although both impellers had the same blade cross-section, one impeller had a two-dimensional blade, while the other had a leaned blade. The flows were also analyzed using a numerical model of the three-dimensional turbulent flow in the pumps near the peak efficiency point using the -? turbulence model and the VOF cavitation model. The average cavitation performance of each impeller was satisfactorily predicted by the numerical simulations. The results show that the miniature pumps have similar cavitation performances as an ordinary-size pump, with the cavitation performance of the semi-open impeller reduced by increased axial tip clearances. Also, both the hydraulic and cavitation performance of the semi-open impeller were improved by the leaned blade. The results also show that uniform flow upstream of the impeller inlet will improve the cavitation performance of a miniature pump.

关键词： cavitation performance semi-open impeller increased two-dimensional efficiency

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连续铸钢前沿技术的工程化

干勇

《中国工程科学》 2002年第4卷第9期页码 12-18

摘要：

论述了具有我国自主知识产权的高效连铸和薄板坯连铸工程化关键技术的特点；介绍了连续铸钢领域轻压下、液压非正弦振动、电磁连铸等前沿技术的开发现状；阐述了传统连铸技术超高效率、高品质化及近终形连铸、电磁连铸开发的研发方向。

关键词：连续铸钢高效连铸薄板坯连铸轻压下电磁连铸

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Utilization of waste vanadium-bearing resources in the preparation of rare-earth vanadate catalysts for semi-hydrogenation

《化学科学与工程前沿（英文）》 2022年第16卷第12期页码 1793-1806 doi: 10.1007/s11705-022-2191-x

摘要： Recycling industrial solid waste not only saves resources but also eliminates environmental concerns of toxic threats. Herein, we proposed a new strategy for the utilization of petrochemical-derived carbon black waste, a waste vanadium-bearing resource (V > 30000 ppm (10 ⁻⁶)). Chemical leaching was employed to extract metallic vanadium from the waste and the leachate containing V was used as an alternative raw material for the fabrication of vanadate nanomaterials. Through the screening of various metal cations, it was found that the contaminated Na⁺ during the leaching process showed strong competitive coordination with the vanadium ions. However, by adding foreign Ce³⁺ and Y³⁺ cations, two rare-earth vanadates, viz., flower-like CeVO₄ and spherical YVO₄ nanomaterials, were successfully synthesized. Characterization techniques such as scanning electron microscopy, transmission electron microscopy, X-ray diffraction, energy-dispersive X-ray spectroscopy, Fourier-transform infrared, and N₂ physisorption were applied to analyze the physicochemical properties of the waste-derived nanomaterials. Importantly, we found that rare-earth vanadate catalysts exhibited good activities toward the semi-hydrogenation of α,β-unsaturated aldehydes. The conversion of cinnamaldehyde and cinnamic alcohol selectivity were even higher than those of the common CeVO₄ prepared using pure chemicals (67.2% vs. 27.7% and 88.4% vs. 53.5%). Our work provides a valuable new reference for preparing vanadate catalysts by the use of abundant vanadium-bearing waste resources.

关键词： petrochemical solid wastes vanadium recovery resource utilization nanomaterials semi-hydrogenation

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Anti-biofouling strategies for implantable biosensors of continuous glucose monitoring systems

《化学科学与工程前沿（英文）》 doi: 10.1007/s11705-023-2340-x

摘要： Continuous glucose monitoring (CGM) systems play an increasingly vital role in the glycemic control of patients with diabetes mellitus. However, the immune responses triggered by the implantation of poorly biocompatible sensors have a significant impact on the accuracy and lifetime of CGM systems. In this review, research efforts over the past few years to mitigate the immune responses by enhancing the anti-biofouling ability of sensors are summarized. This review divided these works into active immune engaging strategy and passive immune escape strategy based on their respective mechanisms. In each strategy, the various biocompatible layers on the biosensor surface, such as drug-releasing membranes, hydrogels, hydrophilic membranes, anti-biofouling membranes based on zwitterionic polymers, and bio-mimicking membranes, are described in detail. This review, therefore, provides researchers working on implantable biosensors for CGM systems with vital information, which is likely to aid in the research and development of novel CGM systems with profound anti-biofouling properties.

关键词： implantable glucose biosensor anti-biofouling continuous glucose monitoring immune responses