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Bioinspired and biomimetic membranes for water purification and chemical separation: A review

《环境科学与工程前沿（英文）》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1412-8

摘要：

•The history of biological and artificial water channels is reviewed.

关键词： Aquaporins     Artificial water channels     Biomimetic membranes     Chemical separation and water purification    

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A hybrid fuel cell for water purification and simultaneously electricity generation

《环境科学与工程前沿（英文）》 2023年 第17卷 第1期 doi: 10.1007/s11783-023-1611-6

摘要：

● A novel hybrid fuel cell (F-HFC) was fabricated.

关键词： Flow-through field     Hybrid fuel cell     Polyoxometalates     Water purification     Electricity generation    

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Hybrid energy harvesting systems for self-powered sustainable water purification by harnessing ambient

《环境科学与工程前沿（英文）》 2023年 第17卷 第10期 doi: 10.1007/s11783-023-1718-9

摘要：

● Energy harvesters harness multiple energies for self-powered water purification.

关键词： Piezocatalysis     Solar energy     Waste heat     Decentralized water treatment     Point-of-use     Nanogenerator    

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and nitrogen co-doped porous carbon derived from sodium alginate enhanced capacitive deionization for waterpurification

《化学科学与工程前沿（英文）》 2023年 第17卷 第12期   页码 2014-2024 doi: 10.1007/s11705-023-2346-4

摘要： Capacitive deionization can alleviate water shortage and water environmental pollution, but performances are greatly determined by the electrochemical and desalination properties of its electrode materials. In this work, B and N co-doped porous carbon with micro-mesoporous structures is derived from sodium alginate by a carbonization, activation, and hydrothermal doping process, which exhibits large specific surface area (2587 m2·g‒1) and high specific capacitance (190.7 F·g‒1) for adsorption of salt ions and heavy metal ions. Furthermore, the materials provide a desalination capacity of 26.9 mg·g−1 at 1.2 V in 500 mg·L‒1 NaCl solution as well as a high removal capacity (239.6 mg·g‒1) and adsorption rate (7.99 mg·g‒1·min‒1) for Pb2+ with an excellent cycle stability. This work can pave the way to design low-cost porous carbon with high-performances for removal of salt ions and heavy metal ions.

关键词： capacitance deionization     porous carbon     B/N co-doping     heavy metal ions     water purification    

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Jellyfish-inspired alginate composite hydrogel filter prepared by macro-micro double bionic strategy for efficient waterpurification

《环境科学与工程前沿（英文）》 2024年 第18卷 第4期 doi: 10.1007/s11783-024-1811-8

摘要：

● A novel hydrogel (2%-SKP-Ca2+) was developed by macro-micro dual biomimetic strategy.

关键词： Triple crosslinking method     Alginate     Umbrella-shaped     Jellyfish     Water purification    

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Selection and characterization of eight freshwater green algae strains for synchronous water purification

Jingjing ZHAN,Qiao ZHANG,Momei QIN,Yu HONG

《环境科学与工程前沿（英文）》 2016年 第10卷 第3期   页码 548-558 doi: 10.1007/s11783-016-0831-4

摘要： The objective of this study is to select and characterize the candidate for synchronous water purification and lipid production from eight freshwater microalgae strains ( sp. HQ, , , , , , , sp. LX1). The strains sp. HQ, . , and . showed superiority in biomass accumulation, while the top biomass producers did not correspond to the top lipid producers. achieved higher lipid content (66.1%), and sp. HQ and ranked down in sequence, with lipid content above 30%. Considering nutrient removal ability (total nitrogen (TN): 52.97%; total phosphorus (TP): 84.81%), the newly isolated microalga sp. HQ was the possible candidate for water purification coupled with lipid production. To further investigate the lipid producing and nutrient removal mechanism of candidate microalga, the ultra structural changes especially the lipid droplets under different water qualities (different TN and TP concentrations) were characterized. The results elucidate the nutrient-deficiency (TN: 3.0 mg·L ; TP: 0.3 mg·L ) condition was in favor of forming lipid bodies in sp. HQ at the sub-cellular level, while the biomass production was inhibited due to the decrease in chloroplast number which could further suppress the nutrient removal effect. Finally, a two-phase cultivation process (a nutrient replete phase to produce biomass followed by a nutrient deplete phase to enhance lipid content) was conducted in a photo-bioreactor for sp. HQ to serve for algae-based synchronous biodiesel production and wastewater purification.

关键词： freshwater microalgae     biomass production     lipid accumulation     nutrient removal    

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The energy-free purification of trace thallium(I)-contaminated potable water using a high-selective filter

《化学科学与工程前沿（英文）》 2024年 第18卷 第2期 doi: 10.1007/s11705-023-2379-8

摘要： Thallium is a highly toxic metal, and trace amount of thallium(I) (Tl+) in potable water could cause a severe water crisis, which arouses the exploitation of highly-effective technology for purification of Tl+ contaminated water. This report proposes the multi-layered Prussian blue (PB)-decorated composite membranes (PBx@PDA/PEI-FP) based on the aminated filter papers for Tl+ uptake. Extensively characterization by Fourier transform infrared spectrometer-attenuated total reflectance, scanning electron microscope, thermogravimetric analysis, X-ray photoelectron spectroscopy and X-ray diffraction were performed to confirm the in situ growth of cubic PB crystals on filter paper membrane surfaces via the aminated layers, and the successful fabrication of multi-layered PB overcoats via the increasing of aminated layers. The effect of PB layers on Tl+ removal by PBx@PDA/PEI-FP from simulated drinking water was evaluated as well as the influence of different experimental conditions. A trade-off between PB decoration layer number and PB distribution sizes is existed in Tl+ uptake by PBx@PDA/PEI-FP. The double-layered PB2@PDA/PEI-FP membrane showed the maximum sorption capacity, but its Tl+ uptake performance was weakened by the acid, coexisting ions (K+ and Na+) and powerful operation pressure, during filtrating a large volume of low-concentrated Tl+-containing water. However, the negative effect of coexisting ions on the Tl+ uptake could be effectively eliminated in weak alkaline water, and the Tl+ removal was increased up to 100% without any pressure driving for PB2@PDA/PEI-FP membrane. Most importantly, PB2@PDA/PEI-FP displayed the high-efficiency and high-selectivity in purifying the Tl+-spiked Pearl River water, in which the residual Tl+ in filtrate was less than 2 μg·L–1 to meet the drinking water standard of United States Environmental Protection Agency. This work provides a feasible avenue to safeguard the drinking water in remote and underdeveloped area via the energy-free operation.

关键词： membrane adsorption     Prussian blue     energy-free filtration     potable water     trace thallium(I)    

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New approaches to water purification for resource-constrained settings: Production of activated biochar

Mohit Nahata, Chang Y. Seo, Pradeep Krishnakumar, Johannes Schwank

《化学科学与工程前沿（英文）》 2018年 第12卷 第1期   页码 194-208 doi: 10.1007/s11705-017-1647-x

摘要： A significant portion of the world’s population does not have access to safe drinking water. This problem is most acute in remote, resource-constrained rural settings in developing countries. Water filtration using activated carbon is one of the important steps in treating contaminated water. Lignocellulosic biomass is generally available in abundance in such locations, such as the African rain forests. Our work is focused on developing a simple method to synthesize activated biochar from locally available materials. The preparation of activated biochar with diammonium hydrogenphosphate (DAP) as the activating agent is explored under N flow and air. The study, carried out with cellulose as a model biomass, provides some insight into the interaction between DAP and biomass, as well as the char forming mechanism. Various characterization techniques such as N physisorption, X-ray photoelectron spectroscopy, scanning electron microscopy, transmission electron microscopy and Raman spectroscopy are utilized to compare the properties between biochar formed under nitrogen and partial oxidative conditions. At a temperature of 450 °C, the loading of DAP over cellulose is systematically varied, and its effect on activation is examined. The activated biochar samples are predominantly microporous in the range of concentrations studied. The interaction of DAP with cellulose is investigated and the nature of bonding of the heteroatoms to the carbonaceous matrix is elucidated. The results indicate that the quality of biochar prepared under partial oxidation condition is comparable to that of biochar prepared under nitrogen, leading to the possibility of an activated biochar production scheme on a small scale in resource-constrained settings.

关键词： cellulose     DAP     activation     heteroatom     microporous    

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饮用水安全问题及净水技术发展

李圭白

《中国工程科学》 2012年 第14卷 第7期   页码 20-23

摘要：

回顾了城市饮用水净水技术发展的历史足迹，即20世纪初的第一代工艺——常规工艺和20世纪70年代的第二代工艺——深度处理工艺，并提出了第三代工艺——以超滤为核心技术的组合工艺；提出了城市水源突发污染的技术对策——针对污染物投加多种药剂；介绍了30年来由哈尔滨工业大学引领开发的新的饮用水净化技术——高锰酸钾及其复合剂净水技术。

关键词： 城市用水的安全性     第三代净水工艺     超滤     水源突发污染及其对策     高锰酸钾及其复合剂    

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Cross-stacked super-aligned carbon nanotube/activated carbon composite electrodes for efficient waterpurification via capacitive deionization enhanced ultrafiltration

Min Li, Shuai Liang, Yang Wu, Meiyue Yang, Xia Huang

《环境科学与工程前沿（英文）》 2020年 第14卷 第6期 doi: 10.1007/s11783-020-1286-1

摘要： Abstract • A high-performance electrode was prepared with super-aligned carbon nanotubes. • SACNT/AC electrode achieved a ~100% increase in desalination capacity and rate. • SACNT/AC electrode achieved a ~26% increase in charge efficiency. • CUF process with SACNT/AC achieved an up to 2.43-fold fouling reduction. • SACNT/AC imparts overall improved water purification efficiency. The practical application of the capacitive deionization (CDI) enhanced ultrafiltration (CUF) technology is hampered due to low performance of electrodes. The current study demonstrated a novel super-aligned carbon nanotube (SACNT)/activated carbon (AC) composite electrode, which was prepared through coating AC on a cross-stacked SACNT film. The desalination capability and water purification performance of the prepared electrode were systematically investigated at different applied voltages (0.8–1.2 V) with a CDI system and a CUF system, respectively. In the CDI tests, as compared with the control AC electrode, the SACNT/AC electrode achieved an approximately 100% increase in both maximum salt adsorption capacity and average salt adsorption rate under all the applied voltage conditions, demonstrating a superior desalination capability. Meanwhile, a conspicuous increase by an average of ~26% in charge efficiency was also achieved at all the voltages. In the CUF tests, as compared with the control run at 0 V, the treatment runs at 0.8, 1.0, and 1.2 V achieved a 2.40-fold, 2.08-fold, and 2.43-fold reduction in membrane fouling (calculated according to the final transmembrane pressure (TMP) data at the end of every purification stage), respectively. The average TMP increasing rates at 0.8, 1.0, and 1.2 V were also roughly two times smaller than that at 0 V, indicating a dramatical reduction of membrane fouling. The SACNT/AC electrode also maintained its superior desalination capability in the CUF process, resulting in an overall improved water purification efficiency.

关键词： Carbon nanotube     Super aligned     Conductive membrane     Capacitive deionization     Ultrafiltration     Desalination    

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Reductant-assisted polydopamine-modified membranes for efficient water purification

Feng Sun, Jinren Lu, Yuhong Wang, Jie Xiong, Congjie Gao, Jia Xu

《化学科学与工程前沿（英文）》 2021年 第15卷 第1期   页码 109-117 doi: 10.1007/s11705-020-1987-9

摘要： Surface engineering with polydopamine coatings has been considered a promising surface functionalisation tool. However, it is difficult to control the self-polymerisation for polydopamine formation, which usually causes severe interparticle aggregation. In this study, polydopamine self-polymerisation was controlled by adjusting its reducing environment using a reductant (NaBH ) to fabricate mixed cellulose ester (MCE)/polydopamine membranes. An oxidising environment using NaIO was additionally tested as the control. The results showed that a thin polydopamine coating with small polydopamine particles was formed on the skeleton frameworks of the MCE membrane with NaBH , and the self-polymerisation rate was suppressed. The polydopamine coating formed in the reducing environment facilitated excellent water transport performance with a water permeance of approximately 400 L·m ·h ·bar as well as efficient organic foulant removal with a bovine serum albumin rejection of approximately 90%. In addition, the polydopamine coating with NaBH exhibited both excellent chemical stability and anti-microbial activity, demonstrating the contribution of the reducing environment to the performance of the MCE/polydopamine membranes. It shows significant potential for use in water purification.

关键词： membrane     water purification     polydopamine     reducing environment     self-polymerization control    

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micron polyhedron with Pt nanoparticle and their enhanced photocatalytic performance in N fixation and waterpurification

《化学科学与工程前沿（英文）》 2023年 第17卷 第12期   页码 1949-1961 doi: 10.1007/s11705-023-2360-6

摘要： This study aimed to prepare and apply a novel Pt/CdMoO4 composite photocatalyst for photocatalytic N2 fixation and tetracycline degradation. The Pt/CdMoO4 composite was subjected to comprehensive investigation on the morphology, structure, optical properties, and photoelectric chemical properties. The results demonstrate the dispersion of Pt nanoparticles on the CdMoO4 surface. Close contact between CdMoO4 and Pt was observed, resulting in the formation of a heterojunction structure at their contact region. Density functional theory calculation and Mott-Schottky analysis revealed that Pt possesses a higher work function value than CdMoO4, resulting in electron drift from CdMoO4 to Pt and the formation of a Schottky barrier. The presence of this barrier increases the separation efficiency of electron-hole pairs, thereby improving the performance of the Pt/CdMoO4 composite in photocatalysis. When exposed to simulated sunlight, the optimal Pt/CdMoO4 catalyst displayed a photocatalytic nitrogen fixation rate of 443.7 μmol·L‒1·g‒1·h‒1, which is 3.2 times higher than that of pure CdMoO4. In addition, the composite also exhibited excellent performance in tetracycline degradation, with hole and superoxide species identified as the primary reactive species. These findings offer practical insights into designing and synthesizing efficient photocatalysts for photocatalytic nitrogen fixation and antibiotics removal.

关键词： photocatalytic N2 fixation     Pt/CdMoO4     tetracycline degradation     Schottky barrier    

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Restoration of hyper-eutrophic water with a modularized and air adjustable constructed submerged plant

Jinzhong LI, Xueju LI, Shujuan SUN, Xuegong LIU, Suiliang HUANG

《环境科学与工程前沿（英文）》 2011年 第5卷 第4期   页码 573-584 doi: 10.1007/s11783-011-0363-x

摘要： A modularized and air adjustable constructed submerged plant bed (CSPB) which can be used to restore the eutrophic water is introduced in this paper. This plant bed helps hydrophyte grow under poor conditions such as frequently changed water depth, impaired water transparency, algae bloom and substantial duckweed in summer, which are not naturally suitable for growing hydrophyte. This pilot study in Waihuan River of Tianjin, China, revealed that reduction of Chemical Oxygen Demand (COD), Total Nitrogen (TN) and Total Phosphorus (TP) by the use of CSPB could be reached 30%–35%, 35%–40%, 30%–40% respectively in the growing season (from March to October) and 5%–10%, 5%–15%, 7%–20% respectively in the winter (from November to February) when the detention time was 6 d. The relationships between the concentration of COD, TN, TP and the detention time fit the first-order kinetic equation well and the coefficients of determination ( ) were all above 0.9. The attenuation coefficients k of the kinetic equation were a function of the water temperature. When the water temperature was quite low or quite high, was not significantly changed with increasing or decreasing water temperature. While when the temperature was in a moderate range, an increase or decrease of water temperature would lead to a rapid increase or decrease in .

关键词： modularized and air adjustable constructed submerged plant bed     water purification     eco-restoration techniques     aquatic plants     eutrophication    

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Interlayer-confined two-dimensional manganese oxide-carbon nanotube catalytic ozonation membrane for efficient waterpurification

《化学科学与工程前沿（英文）》 2022年 第16卷 第5期   页码 731-744 doi: 10.1007/s11705-021-2110-6

摘要： Catalytic ozonation technology has attracted copious attention in water purification owing to its favorable oxidative degradation of pollutants and mitigation of membrane fouling capacity. However, its extensive industrial application has been restricted by the low ozone utilization and limited mass transfer of the short-lived radical species. Interlayer space-confined catalysis has been theoretically proven to be a viable strategy for achieving high catalytic efficiency. Here, a two-dimensional MnO2-incorporated ceramic membrane with tunable interspacing, which was obtained via the intercalation of a carbon nanotube, was designed as a catalytic ozonation membrane reactor for degrading methylene blue. Benefiting from the abundant catalytic active sites on the surface of two-dimensional MnO2 as well as the ultralow mass transfer resistance of fluids due to the nanolayer confinement, an excellent mineralization effect, i.e., 1.2 mg O3(aq) mg–1 TOC removal (a total organic carbon removal rate of 71.5%), was achieved within a hydraulic retention time of 0.045 s of pollutant degradation. Further, the effects of hydraulic retention time and interlayer spacing on methylene blue removal were investigated. Moreover, the mechanism of the catalytic ozonation employing catalytic ozonation membrane was proposed based on the contribution of the Mn(III/IV) redox pair to electron transfer to generate the reactive oxygen species. This innovative two-dimensional confinement catalytic ozonation membrane could act as a nanoreactor and separator to efficiently oxidize organic pollutants and enhance the control of membrane fouling during water purification.

关键词： catalytic membrane reactor     catalytic ozonation     nanoconfinement     two-dimensional manganese oxide    

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Functional magnetic nanoparticles for facile viable but nonculturable bacteria separation and purification

Chunming Wang, Huirong Lin, Chengsong Ye

《环境科学与工程前沿（英文）》 2016年 第10卷 第6期 doi: 10.1007/s11783-016-0874-6

摘要： The functional surface-modified MNPs were capable of capture with high efficiency. After induced to VBNC state by chlorination, cells could be separated by MNPs with an additional incubation process. This study provides a facile and economic method for VBNC cell enrichment and purification. GRAPHIC ABSTRACT Viable But Nonculturable (VBNC) Bacteria, which represent a unique population of microorganisms in drinking water systems, have become a potential threat to human health. Current studies on VBNC cells usually fail to obtain pure VBNC state bacteria, which may lead to inaccurate results. We therefore introduce a novel method of VBNC cell separation and purification in this paper. PAH-coated magnetic nanoparticles (MNPs) were synthesized and found to be capable of capturing and releasing bacterial cells with high efficiency. With the aid of an additional incubation step, VBNC cells were easily isolated and purified from normal bacteria using functional MNPs. Our method represents a new technique that can be utilized in studies of VBNCs.

关键词： Drinking water biosafety     VBNC     Nanoparticles     Magnetic separation and purification    

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标题 作者 时间 类型 操作

Bioinspired and biomimetic membranes for water purification and chemical separation: A review

期刊论文

A hybrid fuel cell for water purification and simultaneously electricity generation

期刊论文

Hybrid energy harvesting systems for self-powered sustainable water purification by harnessing ambient

期刊论文

and nitrogen co-doped porous carbon derived from sodium alginate enhanced capacitive deionization for waterpurification

期刊论文

Jellyfish-inspired alginate composite hydrogel filter prepared by macro-micro double bionic strategy for efficient waterpurification

期刊论文

Selection and characterization of eight freshwater green algae strains for synchronous water purification

Jingjing ZHAN,Qiao ZHANG,Momei QIN,Yu HONG

期刊论文

The energy-free purification of trace thallium(I)-contaminated potable water using a high-selective filter

期刊论文

New approaches to water purification for resource-constrained settings: Production of activated biochar

Mohit Nahata, Chang Y. Seo, Pradeep Krishnakumar, Johannes Schwank

期刊论文

饮用水安全问题及净水技术发展

李圭白

期刊论文

Cross-stacked super-aligned carbon nanotube/activated carbon composite electrodes for efficient waterpurification via capacitive deionization enhanced ultrafiltration

Min Li, Shuai Liang, Yang Wu, Meiyue Yang, Xia Huang

期刊论文

Reductant-assisted polydopamine-modified membranes for efficient water purification

Feng Sun, Jinren Lu, Yuhong Wang, Jie Xiong, Congjie Gao, Jia Xu

期刊论文

micron polyhedron with Pt nanoparticle and their enhanced photocatalytic performance in N fixation and waterpurification

期刊论文

Restoration of hyper-eutrophic water with a modularized and air adjustable constructed submerged plant

Jinzhong LI, Xueju LI, Shujuan SUN, Xuegong LIU, Suiliang HUANG

期刊论文

Interlayer-confined two-dimensional manganese oxide-carbon nanotube catalytic ozonation membrane for efficient waterpurification

期刊论文

Functional magnetic nanoparticles for facile viable but nonculturable bacteria separation and purification

Chunming Wang, Huirong Lin, Chengsong Ye

期刊论文