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Carbon Footprint Drivers in China’s Municipal Wastewater Treatment Plants and Mitigation Opportunities

Shen Qu,Yuchen Hu,Renke Wei,Ke Yu,Zhouyi Liu,Qi Zhou,Chenchen Wang,Lujing Zhang,

《工程（英文）》 doi: 10.1016/j.eng.2024.01.021

摘要： Reducing greenhouse gas (GHG) emissions to address climate change is a global consensus, and municipal wastewater treatment plants (MWWTPs) should lead the way in low-carbon sustainable development. However, achieving effluent discharge standards often requires considerable energy and chemical consumption during operation, resulting in significant carbon footprints. In this study, GHG emissions are systematically accounted for, and the driving factors of carbon footprint growth in China’s MWWTPs are explored. In 2020, a total of 41.9 million tons (Mt) of carbon dioxide equivalent (CO2-eq) were released by the sector, with nearly two-thirds being indirect emissions resulting from energy and material usage. The intensity of electricity, carbon source, and phosphorus removing agent consumption increasingly influence carbon footprint growth over time. Through statistical inference, benchmarks for electricity and chemical consumption intensity are established across all MWWTPs under various operational conditions, and the potential for mitigation through more efficient energy and material utilization is calculated. The results suggest that many MWWTPs offer significant opportunities for emission reduction. Consequently, empirical decarbonization measures, including intelligent device control, optimization of aeration equipment, energy recovery initiatives, and other enhancements to improve operational and carbon efficiency, are recommended.

关键词： Municipal wastewater treatment plants (MWWTPs)     Carbon footprint     Driving Factors     Mitigation opportunities    

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Microplastics in municipal wastewater treatment plants: a case study of Denizli/Turkey

《环境科学与工程前沿（英文）》 2023年 第17卷 第8期 doi: 10.1007/s11783-023-1699-8

摘要：

● High amounts of microplastics are released to receiving media from WWTPs.

关键词： Microplastics     Wastewater treatment plant     Removal efficiency     Daily discharge    

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Current status of municipal wastewater treatment plants in North-east China: implications for reforming

《环境科学与工程前沿（英文）》 2023年 第17卷 第6期 doi: 10.1007/s11783-023-1673-5

摘要：

● The performance and costs of 20 municipal WWTPs were analyzed.

关键词： Low temperature     Municipal WWTPs     Cold region     Electricity consumption     Nitrogen removal    

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Occurrence and migration of microplastics and plasticizers in different wastewater and sludge treatmentunits in municipal wastewater treatment plant

《环境科学与工程前沿（英文）》 2022年 第16卷 第11期 doi: 10.1007/s11783-022-1577-9

摘要：

● Reduce the quantifying MPs time by using Nile red staining.

关键词： Microplastics     Municipal wastewater treatment plant     Phthalate esters     Thermal hydrolysis    

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Pollution of NPEOs in four municipal sewage treatment plants in the north of China

HOU Shaogang, SUN Hongwen

《环境科学与工程前沿（英文）》 2007年 第1卷 第2期   页码 196-201 doi: 10.1007/s11783-007-0034-0

摘要： The concentration and distribution of nonylphenol polyethoxylates (NPEOs represents the mixture, and NPEO represents the monomer) and its metabolites in the influent and effluent of four municipal sewage treatment plants (STPs) in the north of China were measured. Moreover, the concentration and distribution of the above chemicals in the sludge of two STPs were also determined, and the transfer and fate of NPEOs in the sewage treatment process were discussed primarily by analyzing the distribution of the products in the effluent and the sludge. The results showed that NPEOs and its metabolites existed in all the samples of the influent, effluent, and sludge. NPEOs were degraded in the sewage treatment process with the removal efficiency in the range of 23.38% 77.11%, or an average of 52.86%. However, the large analogs of NPEO were only degraded to small ones, whose degradation rate was rather slow, and consequently the degradation was not complete. Hence, the concentrations of some small metabolites, such as nonylphenol (NP), nonylphenol monoethoxylate (NP1EO), and nonylphenol diethoxylate (NP2EO) were elevated in the effluent. These small metabolites are more toxic than the large NPnEO analogs, and some of them were reported to exhibit environmental endocrine disrupting activity. From this point of view, the process of sewage treatment does not reduce but elevate the risk of NPEOs, which becomes the main source of these small NPEO in the environment. The sludge exhibited good adsorption ability for NPEOs, especially for the small analogs, which led to the high level of NPEOs in the sludge. Hence, reasonable disposal of the surplus sludge to avoid re-pollution is very important.
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Photosensitivity sources of dissolved organic matter from wastewater treatment plants and their mediation

《环境科学与工程前沿（英文）》 2023年 第17卷 第6期 doi: 10.1007/s11783-023-1669-1

摘要：

● EE2 photodegradation behavior in the presence of four WWTPs’ DOM was explored.

关键词： Photosensitivity sources     17α-ethinylestradiol     Photodegradation     Dissolved organic matter     Wastewater treatment plants    

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Nitrogen removal efficiencies and microbial communities in full-scale IFAS and MBBR municipal wastewatertreatment plants at high COD:N ratio

Supaporn Phanwilai, Naluporn Kangwannarakul, Pongsak (Lek) Noophan, Tamao Kasahara, Akihiko Terada, Junko Munakata-Marr, Linda Ann Figueroa

《环境科学与工程前沿（英文）》 2020年 第14卷 第6期 doi: 10.1007/s11783-020-1374-2

摘要： Abstract • Two IFAS and two MBBR full-scale systems (high COD:N ratio 8:1) were characterized. • High specific surface area carriers grew and retained slow-growing nitrifiers. • High TN removal is related to high SRT and low DO concentration in anoxic tanks. The relative locations of AOB, NOB, and DNB were examined for three different kinds of carriers in two types of hybrid biofilm process configurations: integrated fixed-film activated sludge (IFAS) and moving bed biofilm reactor (MBBR) processes. IFAS water resource recovery facilities (WRRFs) used AnodkalnessTM K1 carriers (KC) at Broomfield, Colorado, USA and polypropylene resin carriers (RC) at Fukuoka, Japan, while MBBR WRRFs used KC carriers at South Adams County, Colorado, USA and sponge carriers (SC) at Saga, Japan. Influent COD to N ratios ranged from 8:1 to 15:1. The COD and BOD removal efficiencies were high (96%–98%); NH4+-N and TN removal efficiencies were more varied at 72%–98% and 64%–77%, respectively. The extent of TN removal was higher at high SRT, high COD:N ratio and low DO concentration in the anoxic tank. In IFAS, RC with high specific surface area (SSA) maintained higher AOB population than KC. Sponge carriers with high SSA maintained higher overall bacteria population than KC in MBBR systems. However, the DNB were not more abundant in high SSA carriers. The diversity of AOB, NOB, and DNB was fairly similar in different carriers. Nitrosomonas sp. dominated over Nitrosospira sp. while denitrifying bacteria included Rhodobacter sp., Sulfuritalea sp., Rubrivivax sp., Paracoccus sp., and Pseudomonas sp. The results from this work suggest that high SRT, high COD:N ratio, low DO concentration in anoxic tanks, and carriers with greater surface area may be recommended for high COD, BOD and TN removal in WRRFs with IFAS and MBBR systems.

关键词： IFAS     MBBR     AnodkalnessTM K1 carrier     Polypropylene resin carrier     Sponge carrier    

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Development and application of some renovated technologies for municipal wastewater treatment in China

QIAN Yi, WEN Xianghua, HUANG Xia

《环境科学与工程前沿（英文）》 2007年 第1卷 第1期   页码 1-12 doi: 10.1007/s11783-007-0001-9

摘要： China has been experiencing fast economic development in recent decades at the cost of serious environmental deterioration. Wastewater discharge, especially municipal wastewater discharge, and non-point pollution sources are becoming the major water pollution source and research focus. Great efforts have been made on water pollution control and a number of renovated technologies and processes for municipal wastewater treatment and reclamation as well as non-point pollution control have been developed and applied in China. This paper discusses the development and application of the appropriate technologies, including natural treatment systems, anaerobic biological treatment, biofilm reactors and wastewater reclamation technologies, for water pollution control in the country.

关键词： reclamation     Wastewater discharge     renovated     biological treatment     application    

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Energy neutrality potential of wastewater treatment plants: A novel evaluation framework integrating

《环境科学与工程前沿（英文）》 2022年 第16卷 第9期 doi: 10.1007/s11783-022-1549-0

摘要：

• Framework of indicators was established based on energy efficiency and recovery.

关键词： Wastewater treatment plants     Energy neutrality potential     Energy efficiency     Energy recovery     Evaluation framework    

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Tracking in urban wastewater treatment plants in a cold region: Occurrence, species and infectivity

《环境科学与工程前沿（英文）》 2022年 第16卷 第9期 doi: 10.1007/s11783-022-1533-8

摘要：

• Cryptosporidium in WWTPs in a cold region was investigated in different seasons.

关键词： WWTPs     Cryptosporidium     Occurrence     Species     Infectivity     Low temperature    

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Impacts of advanced treatment processes on elimination of antibiotic resistance genes in a municipalwastewater treatment plant

Lian Yang, Qinxue Wen, Zhiqiang Chen, Ran Duan, Pan Yang

《环境科学与工程前沿（英文）》 2019年 第13卷 第3期 doi: 10.1007/s11783-019-1116-5

摘要：

The distributions of ARGs were monitored in a WWTP in Harbin during six months.

CASS had the best removal efficacy of ARGs compared to other processes in the WWTP.

UV disinfection could effectively control the HGT.

AGAC significantly remove ARGs and organics due to its high absorption capacity.

Combination of ozone and AGAC significantly improve removal of ARGs and organics.

关键词： Antibiotic resistance genes (ARGs)     Wastewater treatment plant (WWTP)     Ultraviolet (UV)     Ozonation     Granular activated carbon (GAC)    

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Removal of odors and VOCs in municipal solid waste comprehensive treatment plants using a novel three-stage

《环境科学与工程前沿（英文）》 2021年 第15卷 第3期 doi: 10.1007/s11783-021-1421-7

摘要：

A novel three-stage integrated biofilter (TSIBF) composed of acidophilic bacteria reaction segment (ABRS), fungal reaction segment (FRS) and heterotrophic bacteria reaction segment (HBRS) was constructed for the treatment of odors and volatile organic compounds (VOCs)from municipal solid waste (MSW) comprehensive treatment plants. The performance, counts of predominant microorganisms, and bioaerosol emissions of a full-scale TSIBF system were studied. High and stable removal efficiencies of hydrogen sulfide, ammonia and VOCs could be achieved with the TSIBF system, and the emissions of culturable heterotrophic bacteria, fungi and acidophilic sulfur bacteria were relatively low.

关键词： Biofiltration     Multi-stage biofilter     Volatile organic compounds     Waste gas treatment     Bioaerosol emissions    

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chemometric analysis on the fluorescent dissolved organic matter in a full-scale sequencing batch reactor for municipalwastewater treatment

Chen Qian, Wei Chen, Wei-Hua Li, Han-Qing Yu

《环境科学与工程前沿（英文）》 2017年 第11卷 第4期 doi: 10.1007/s11783-017-0962-2

摘要： Rapid monitoring of water quality is crucial to the operation of municipal wastewater treatment plants (WWTPs). Fluorescence excitation-emission matrix (EEM) in combination with parallel factor analysis (PARAFAC) has been used as a powerful tool for the characterization of dissolved organic matter (DOM) in WWTPs. However, a recent work has revealed the drawback of PARAFAC analysis, i.e., overestimating the component number. A novel method, parallel factor framework-clustering analysis (PFFCA), has been developed in our earlier work to resolve this drawback of PARAFAC. In the present work, both PARAFAC and PFFCA were used to analyze the EEMs of water samples from a full-scale WWTP from a practical application point of view. The component number and goodness-of-fit from these two methods were compared and the relationship between the relative score change of component and the actual concentration was investigated to evaluate the estimation error introduced by both methods. PFFCA score and actual concentration exhibited a higher correlation coefficient ( = 0.870) compared with PARAFAC ( <0.771), indicating that PFFCA provided a more accurate relative change estimation than PARAFAC. The results suggest that use of PARAFAC may cause confusion in selecting the component number, while EEM-PFFCA is a more reliable alternative approach for monitoring water quality in WWTPs.

关键词： Wastewater treatment plants (WWTPs)     Excitation-emission matrix (EEM)     Parallel factor (PARAFAC)     Parallel factor framework-clustering analysis (PFFCA)    

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Composition, dispersion, and health risks of bioaerosols in wastewater treatment plants: A review

Yunping Han, Lin Li, Ying Wang, Jiawei Ma, Pengyu Li, Chao Han, Junxin Liu

《环境科学与工程前沿（英文）》 2021年 第15卷 第3期 doi: 10.1007/s11783-020-1330-1

摘要： Abstract • Bioaerosols are produced in the process of wastewater biological treatment. • The concentration of bioaerosol indoor is higher than outdoor. • Bioaerosols contain large amounts of potentially pathogenic biomass and chemicals. • Inhalation is the main route of exposure of bioaerosol. • Both the workers and the surrounding residents will be affected by the bioaerosol. Bioaerosols are defined as airborne particles (0.05–100 mm in size) of biological origin. They are considered potentially harmful to human health as they can contain pathogens such as bacteria, fungi, and viruses. This review summarizes the most recent research on the health risks of bioaerosols emitted from wastewater treatment plants (WWTPs) in order to improve the control of such bioaerosols. The concentration and size distribution of WWTP bioaerosols; their major emission sources, composition, and health risks; and considerations for future research are discussed. The major themes and findings in the literature are as follows: the major emission sources of WWTP bioaerosols include screen rooms, sludge-dewatering rooms, and aeration tanks; the bioaerosol concentrations in screen and sludge-dewatering rooms are higher than those outdoors. WWTP bioaerosols contain a variety of potentially pathogenic bacteria, fungi, antibiotic resistance genes, viruses, endotoxins, and toxic metal(loid)s. These potentially pathogenic substances spread with the bioaerosols, thereby posing health risks to workers and residents in and around the WWTP. Inhalation has been identified as the main exposure route, and children are at a higher risk of this than adults. Future studies should identify emerging contaminants, establish health risk assessments, and develop prevention and control systems.

关键词： Wastewater treatment plant     Bioaerosols     Pathogen     Dispersion     Risk assessment    

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Performance and mechanistic study on electrocoagulation process for municipal wastewater treatment based

Zhenlian Qi, Shijie You, Ranbin Liu, C. Joon Chuah

《环境科学与工程前沿（英文）》 2020年 第14卷 第3期 doi: 10.1007/s11783-020-1215-3

摘要： EC modified with BPEs enhances pollutant removal and reduce energy consumption. Increasing BPE number cannot increase flocculants yield exponentially. Simulations help to predict the distribution of electrochemical reactions on BPEs. The design of electrodes is crucial to electrocoagulation process (EC), specifically, with respect to pollutant removal and energy consumption. During EC, the mechanisms for interaction between different electrode arrangement and electrode reactions remain unclear. This work presents an integrated EC process based on horizontal bipolar electrodes (BPEs). In the electrochemical cell, the graphite plates are used as driving cathode while either Fe or Al plates serves as driving anode and BPEs. The BPEs are placed horizontally between the driving electrodes. For municipal wastewater treatment, the pollutant removal efficiency and energy consumption in different configurations of two-dimension electrocoagulation (2D-EC) system with horizontal BPEs were investigated. The removal efficiency of turbidity, total phosphorus and total organic carbon increased significantly with the number of BPEs. Noted that the energy consumption for TP removal decreased by 75.2% with Fe driving anode and 81.5% with Al driving anode than those of 2D-EC, respectively. In addition, the physical field simulation suggested the distributions of potential and current in electrolyte and that of induced charge density on BPE surface. This work provides a visual theoretical guidance to predict the distribution of reactions on BPEs for enhanced pollutant removal and energy saving based on electrocoagulation process for municipal wastewater treatment.

关键词： Electrocoagulation     Bipolar electrodes     Municipal wastewater     Simulations    

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标题 作者 时间 类型 操作

Carbon Footprint Drivers in China’s Municipal Wastewater Treatment Plants and Mitigation Opportunities

Shen Qu,Yuchen Hu,Renke Wei,Ke Yu,Zhouyi Liu,Qi Zhou,Chenchen Wang,Lujing Zhang,

期刊论文

Microplastics in municipal wastewater treatment plants: a case study of Denizli/Turkey

期刊论文

Current status of municipal wastewater treatment plants in North-east China: implications for reforming

期刊论文

Occurrence and migration of microplastics and plasticizers in different wastewater and sludge treatmentunits in municipal wastewater treatment plant

期刊论文

Pollution of NPEOs in four municipal sewage treatment plants in the north of China

HOU Shaogang, SUN Hongwen

期刊论文

Photosensitivity sources of dissolved organic matter from wastewater treatment plants and their mediation

期刊论文

Nitrogen removal efficiencies and microbial communities in full-scale IFAS and MBBR municipal wastewatertreatment plants at high COD:N ratio

Supaporn Phanwilai, Naluporn Kangwannarakul, Pongsak (Lek) Noophan, Tamao Kasahara, Akihiko Terada, Junko Munakata-Marr, Linda Ann Figueroa

期刊论文

Development and application of some renovated technologies for municipal wastewater treatment in China

QIAN Yi, WEN Xianghua, HUANG Xia

期刊论文

Energy neutrality potential of wastewater treatment plants: A novel evaluation framework integrating

期刊论文

Tracking in urban wastewater treatment plants in a cold region: Occurrence, species and infectivity

期刊论文

Impacts of advanced treatment processes on elimination of antibiotic resistance genes in a municipalwastewater treatment plant

Lian Yang, Qinxue Wen, Zhiqiang Chen, Ran Duan, Pan Yang

期刊论文

Removal of odors and VOCs in municipal solid waste comprehensive treatment plants using a novel three-stage

期刊论文

chemometric analysis on the fluorescent dissolved organic matter in a full-scale sequencing batch reactor for municipalwastewater treatment

Chen Qian, Wei Chen, Wei-Hua Li, Han-Qing Yu

期刊论文

Composition, dispersion, and health risks of bioaerosols in wastewater treatment plants: A review

Yunping Han, Lin Li, Ying Wang, Jiawei Ma, Pengyu Li, Chao Han, Junxin Liu

期刊论文

Performance and mechanistic study on electrocoagulation process for municipal wastewater treatment based

Zhenlian Qi, Shijie You, Ranbin Liu, C. Joon Chuah

期刊论文