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δN-stable isotope analysis of NH: An overview on analytical measurements, source sampling and its sourceapportionment

《环境科学与工程前沿（英文）》 2021年第15卷第6期 doi: 10.1007/s11783-021-1414-6

摘要：

• Challenges in sampling of NH₃ sources for d¹⁵N analysis are highlighted.

关键词： Aerosol ammonium Atmospheric gaseous ammonia Isotope fingerprinting Isotope-based source apportionment Ammonia gas-to-particle conversion

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Development of source profiles and their application in source apportionment of PM

Ningning Zhang, Mazhan Zhuang, Jie Tian, Pengshan Tian, Jieru Zhang, Qiyuan Wang, Yaqing Zhou, Rujin Huang, Chongshu Zhu, Xuemin Zhang, Junji Cao

《环境科学与工程前沿（英文）》 2016年第10卷第5期 doi: 10.1007/s11783-016-0879-1

摘要： Seasonal and spatial distribution of PM and its component were shown. Local source profiles of major PM sources were developed. Source apportionment was conducted using CMB model. Inorganic secondary components is the biggest contribution at Xiamen. Ambient PM samples were collected at four sites in Xiamen, including Gulangyu (GLY), Hongwen (HW), Huli (HL) and Jimei (JM) during January, April, July and October 2013. Local source samples were obtained from coal burning power plants, industries, motor vehicles, biomass burning, fugitive dust, and sea salt for the source apportionment studies. The highest value of PM mass concentration and species related to human activities (SO , NO , Pb, Ni, V, Cu, Cd, organic carbon (OC) and elemental carbon (EC)) were found in the ambient samples from HL, and the highest and lowest loadings of PM and its components occurred in winter and summer, respectively. The reconstructed mass balance indicated that ambient PM consisted of 24% OM (organic matter), 23% sulfate, 14% nitrate, 9% ammonium, 9% geological material, 6% sea salt, 5% EC and 10% others. For the source profiles, the dominant components were OC for coal burning, motor vehicle, biomass burning and sea salt; SO for industry; and crustal elements for fugitive dust. Source contributions were calculated using a chemical mass balance (CMB) model based on ambient PM concentrations and the source profiles. GLY was characterized by high contributions from secondary sulfate and cooking, while HL and JM were most strongly affected by motor vehicle emissions, and biomass burning and fugitive dust, respectively. The CMB results indicated that PM from Xiamen is composed of 27.4% secondary inorganic components, 20.8% motor vehicle emissions, 11.7% fugitive dust, 9.9% sea salt, 9.3% coal burning, 5.0% biomass burning, 3.1% industry and 6.8% others.

关键词： PM_2.5 Source profile Source apportionment CMB Xiamen

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Source apportionment of PM

Wei WEN,Shuiyuan CHENG,Lei LIU,Gang WANG,Xiaoqi WANG

《环境科学与工程前沿（英文）》 2016年第10卷第5期 doi: 10.1007/s11783-016-0839-9

摘要： The new hybrid approaches for the source apportionment of PM were proposed. The hybrid approach can be used for source apportionment of secondary species. The metallurgy industry was the biggest contribution source to PM of Tangshan. In winter, the contribution from the coal-fired boilers was the largest one. The objective of this paper is to propose a hybrid approach for the source apportionment of primary and secondary species of PM in the city of Tangshan. The receptor-based PMF (Positive Matrix Factorization) is integrated with the emission inventory (EI) to form the first hybrid method for the source apportionment of the primary species. The hybrid CAMx-PSAT-CP (Comprehensive Air Quality Model with Extensions – Particulate Source Apportionment Technology – Chemical Profile) approach is then proposed and used for the source apportionment of the secondary species. The PM sources identified for Tangshan included the soil dust, the metallurgical industry, power plants, coal-fired boilers, vehicles, cement production, and other sources. It is indicated that the PM pollution is a regional issue. Among all the identified sources, the metallurgy industry was the biggest contribution source to PM , followed by coal-fired boilers, vehicles and soil dust. The other-source category plays a crucial role for PM , particularly for the formation of secondary species and aerosols, and these other sources include non-specified sources such as agricultural activities, biomass combustion, residential emissions, etc. The source apportionment results could help the local authorities make sound policies and regulations to better protect the citizens from the local and regional PM pollution. The study also highlights the strength of utilizing the proposed hybrid approaches in the identification of PM sources. The techniques used in this study show considerable promise for further application to other regions as well as to identify other source categories of PM .

关键词： Secondary species Emission inventory PM_2.5 Source apportionment

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Source apportionment of ambient PM

Bo HAN, Xiaohui BI, Yonghua XUE, Jianhui WU, Tan ZHU, Baogui ZHANG, Jianqing DING, Yuanxin DU

《环境科学与工程前沿（英文）》 2011年第5卷第4期页码 552-563 doi: 10.1007/s11783-010-0263-5

摘要： A total of 168 PM samples were collected during the year of 2005 at eight sites in the city of Wuxi in China. Fifteen chemical elements, three water-soluble ions, total carbon and organic carbon were analyzed. Six source categories were identified and their contributions to ambient PM in Wuxi were estimated using a nested chemical mass balance method that reduces the effects of colinearity on the chemical mass balance model. In addition, the concentrations of secondary aerosols, such as secondary organic carbon, sulfate and nitrate, were quantified. The spatially averaged PM was high in the spring and winter (123 μg·m and low in the summer–fall (90 μg·m ). According to the result of source apportionment, resuspended dust was the largest contributor to ambient PM , accounting for more than 50% of the PM mass. Coal combustion (14.6%) and vehicle exhaust (9.4%) were also significant source categories of ambient PM . Construction and cement dust, sulfates, secondary organic carbon, and nitrates made contributions ranging between 4.1% and 4.9%. Other source categories such as steel manufacturing dust and soil dust made low contributions to ambient PM .

关键词： source apportionment inhalable particulate matter nested chemical mass balance method

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Local and regional contributions to PM in the Beijing 2022 Winter Olympics infrastructure areas during haze episodes

《环境科学与工程前沿（英文）》 2021年第15卷第6期 doi: 10.1007/s11783-021-1434-2

摘要：

• Regional transportation contributed more than local emissions during haze episodes.

关键词： 2022 Winter Olympics PM_2.5 Source apportionment

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A method for quantifying bias in modeled concentrations and source impacts for secondary particulate

Cesunica E. Ivey, Heather A. Holmes, Yongtao Hu, James A. Mulholland, Armistead G. Russell

《环境科学与工程前沿（英文）》 2016年第10卷第5期 doi: 10.1007/s11783-016-0866-6

摘要： A method for quantifying source impacts for secondary PM species is derived. The method provides estimates of bias in modeled concentrations. Adjusted concentrations match corresponding observations at monitored locations. Sources impacts on secondary species are estimated over the US for 20 sources. Community Multi-Scale Air Quality (CMAQ) estimates of sulfates, nitrates, ammonium, and organic carbon are highly influenced by uncertainties in modeled secondary formation processes, such as chemical mechanisms, volatilization, and condensation rates. These compounds constitute the majority of PM mass, and reducing bias in estimated concentrations has benefits for policy measures and epidemiological studies. In this work, a method for adjusting source impacts on secondary species is developed that provides estimates of source contributions and reduces bias in modeled concentrations compared to observations. The bias correction adjusts concentrations and source impacts based on the difference between modeled concentrations and observations while taking into account uncertainties at the location of interest; and it is applied both spatially and temporally. We apply the method over the US for 2006. The mean bias for initial CMAQ concentrations compared to observations is −0.28 (OC), 0.11 (NO ), 0.05 (NH ), and −0.08 (SO ). The normalized mean bias in modeled concentrations compared to observations was effectively zero for OC, NO , NH , and SO after applying the secondary bias correction. 10-fold cross-validation was conducted to determine the performance of the spatial application of the bias correction. Cross-validation performance was favorable; correlation coefficients were greater than 0.69 for all species when comparing observations and concentrations based on kriged correction factors. The methods presented here address model uncertainties by improving simulated concentrations and source impacts of secondary particulate matter through data assimilation. Secondary-adjusted concentrations and source impacts from 20 emissions sources are generated for 2006 over continental US.

关键词： Particulate matter Source apportionment Secondary particulate matter Chemical transport modeling Receptor modeling

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Fault tolerant control strategy for modular PWM current source inverter

《能源前沿（英文）》 doi: 10.1007/s11708-022-0852-6

摘要： In this paper, a fault-tolerant control method for an input-series output-parallel modular grid-tied pulse-width modulation (PWM) current source inverter is proposed to address the most commonly seen single symmetrical gate-commutated thyristor (SGCT) open-circuit fault problems. This method actively offsets the neutral point of the current space vector to ensure a sinusoidal output of the grid current, and it can achieve the upper limit power of the inverter under the condition of a single SGCT open-circuit fault. In addition, an active damping control method based on grid harmonic current feedback is proposed after analyzing the influence of the transformer ferromagnetic resonance caused by the neutral point offset on the power quality of the grid current. It has been demonstrated that the proposed method effectively suppresses the resonance caused by the transformer and the modified modulation, improving the grid current’s power quality.

关键词： current source converter (CSC) fault-tolerant control space vector modulation active damping resonance suppression power quality

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The source and transport of bioaerosols in the air: A review

《环境科学与工程前沿（英文）》 2021年第15卷第3期 doi: 10.1007/s11783-020-1336-8

摘要：

• Emission of microbe from local environments is a main source of bioaerosols.

关键词： Bioaerosols Diffusion Source identification Biogeography

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Performance analysis of an air-source heat pump using an immersed water condenser

Jie JI, Huide FU, Hanfeng HE, Gang PEI,

《能源前沿（英文）》 2010年第4卷第2期页码 234-245 doi: 10.1007/s11708-009-0056-3

摘要： A distributed model of an air-source heat pump (ASHP) system and its experimental setup using an immersed water condenser were presented. Dynamic performance of the ASHP was then evaluated by both simulation and experiment. The results indicated that the system coefficient of performance (COP) decreased as the condenser temperature increased, ranging from 4.41 to 2.32 with the average COP equaling 3.29 during the experiment. Comparisons between simulation results and experimental measurements demonstrated that the model was able to yield satisfactory predictions. Furthermore, temperature profiles of the refrigerant in the evaporator and condenser were also given. This paper provides the theoretical and experimental background for ASHP system optimization and a valuable reference for a solar air-source heat pump water heater when the solar irradiation energy is insufficient on cloudy or rainy days.

关键词： air-source heat pump distributed model immersed water condenser

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CO capture and sequestration source-sink match optimization in Jing-Jin-Ji region of China

Zhong ZHENG , Dan GAO , Linwei MA , Zheng LI , Weidou NI ,

《能源前沿（英文）》 2009年第3卷第3期页码 359-368 doi: 10.1007/s11708-009-0053-6

摘要： Carbon dioxide capture and sequestration (CCS) is considered to be an important option for climate change mitigation. A key problem for the implementation of CCS technology is the source-sink match design and optimization when considering both economic and environmental requirement. This paper presents a generic-optimization-based model for the strategic planning and design of future CCS source-sink matching. The features and capabilities of the model are illustrated through a detailed case study for the Jing-Jin-Ji (Beijing, Tianjin and Hebei Province) region in China. It shows how the model helps make a compromise in arriving at a strategic decision for CCS source-sink matching by providing the tradeoff frontiers between economic and environmental performance, and the features of match solutions with the best economic performance or with the best environmental performance.

关键词： CO₂ capture and sequestration China source-sink match tradeoff frontiers multi-objective optimization

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Identification and ranking of the risky organic contaminants in the source water of the Danjiangkou reservoir

Qingwei BU, Donghong WANG, Zijian WANG, Junnong GU

《环境科学与工程前沿（英文）》 2014年第8卷第1期页码 42-53 doi: 10.1007/s11783-013-0499-y

摘要： The Danjiangkou reservoir was selected to provide the source water for the middle routes of the South to North Water Transfer Project, which has provoked many environmental concerns. To date, investigations of water contamination of the source water of the Danjiangkou reservoir with organic micro-pollutants have been limited. This study was conducted to identify and rank organic contaminants that pose risks in the Danjiangkou reservoir. To this end, the Chemical Hazard Evaluation and Management Strategies (CHEMS-1) approach was adapted to integrate the deconvolution technology of qualitative identifying contaminants for site-specific environmental matrices. The samples were screened for the presence of 1093 contaminants using deconvolution technologies and the hazard values of the identified contaminants were calculated using the adapted CHEMS-1 approach according to their hazardous properties and occurrence in source water. The results showed that 46 contaminants from 1093 targets were present in Danjiangkou water, 23 of which appeared at frequencies higher than 50%, and 15 of which were identified as priorities. Over half (53%) of the high-ranked contaminants were polycyclic aromatic hydrocarbons (PAHs), with chrysene ranked highest on the list. Health risk assessment of the top-ranked PAHs was conducted and revealed that cancer risks of PAHs detected in the source water of Danjiangkou to different populations ranged from 10 to 10 , indicating a low cancer risk to consumers. The results of this study indicated that the adapted CHEMS-1 approach was feasible for site-specific screening of organic contaminants to identify and rank potential priority pollutants.

关键词： identification and ranking source water deconvolution risk assessment Danjiangkou South to North Water Transfer Project

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Acid Orange 7 degradation using methane as the sole carbon source and electron donor

《环境科学与工程前沿（英文）》 2022年第16卷第3期 doi: 10.1007/s11783-021-1468-5

摘要：

• AO7 degradation was coupled with anaerobic methane oxidation.

关键词： Azo dyes AO7 degradation Anaerobic methane oxidation Microbial community ANME-2d

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Optimization model analysis of centralized groundwater source heat pump system in heating season

Shilei LU,Yunfang QI,Zhe CAI,Yiran LI

《能源前沿（英文）》 2015年第9卷第3期页码 343-361 doi: 10.1007/s11708-015-0372-8

摘要： The ground-water heat-pump system (GWHP) provides a high efficient way for heating and cooling while consuming a little electrical energy. Due to the lack of scientific guidance for operating control strategy, the coefficient of performance (COP) of the system and units are still very low. In this paper, the running strategy of GWHP was studied. First, the groundwater thermal transfer calculation under slow heat transfixion and transient heat transfixion was established by calculating the heat transfer simulation software Flow Heat and using correction factor. Next, heating parameters were calculated based on the building heat load and the terminal equipment characteristic equation. Then, the energy consumption calculation model for units and pumps were established, based on which the optimization method and constraints were established. Finally, a field test on a GWHP system in Beijing was conducted and the model was applied. The new system operation optimization idea for taking every part of the GWHP into account that put forward in this paper has an important guiding significance to the actual operation of underground water source heat pump.

关键词： optimization model groundwater source heat pump system theoretical analysis example verification heating season

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THAI experimental research on hydrogen risk and source term related safety systems

《能源前沿（英文）》 2021年第15卷第4期页码 887-915 doi: 10.1007/s11708-021-0789-1

摘要： In the defense-in-depth concept employed for the safety of nuclear installations, maintaining integrity of containment as the last barrier is of high importance to limit the release of radioactivity to the environment in case of a severe accident. The active and passive safety systems implemented in containments of light water reactors (LWRs) are designed to limit the consequences of such accidents. Assessing the performance and reliability of such systems under accident conditions is critical to the safety of nuclear installations.

关键词： severe accident containment safety mitigation H₂ risk source term

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Toward separation at source: Evolution of Municipal Solid Waste management in China

Jianguo Liu, Shuyao Yu, Yixuan Shang

《环境科学与工程前沿（英文）》 2020年第14卷第2期 doi: 10.1007/s11783-020-1232-2

摘要： Municipal Solid Waste (MSW) management in China has been transitioning from a mixed collection and treatment system to a separated collection and treatment system. The continuous rise of MSW treatment capacity and the optimization of technology structure provided basic facility support for China to promote MSW separation at source. China preferred a four-type separation system. Regulated recycling should be enhanced to improve the efficiency and sustainability of recycling industry. As food waste is the main composition of MSW in China, 20%–30% of the food waste diversion and land application could maximize the comprehensive environmental performance. Incineration is to be the pillar technology in MSW separated treatment system in China.

关键词： Municipal Solid Waste Separation at source Recycling Biological treatment Incineration

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标题作者时间类型操作

δN-stable isotope analysis of NH: An overview on analytical measurements, source sampling and its sourceapportionment

期刊论文

Development of source profiles and their application in source apportionment of PM

Ningning Zhang, Mazhan Zhuang, Jie Tian, Pengshan Tian, Jieru Zhang, Qiyuan Wang, Yaqing Zhou, Rujin Huang, Chongshu Zhu, Xuemin Zhang, Junji Cao

期刊论文

Source apportionment of PM

Wei WEN,Shuiyuan CHENG,Lei LIU,Gang WANG,Xiaoqi WANG

期刊论文

Source apportionment of ambient PM

Bo HAN, Xiaohui BI, Yonghua XUE, Jianhui WU, Tan ZHU, Baogui ZHANG, Jianqing DING, Yuanxin DU

期刊论文

Local and regional contributions to PM in the Beijing 2022 Winter Olympics infrastructure areas during haze episodes

期刊论文

A method for quantifying bias in modeled concentrations and source impacts for secondary particulate

Cesunica E. Ivey, Heather A. Holmes, Yongtao Hu, James A. Mulholland, Armistead G. Russell

期刊论文

Fault tolerant control strategy for modular PWM current source inverter

期刊论文

The source and transport of bioaerosols in the air: A review

期刊论文

Performance analysis of an air-source heat pump using an immersed water condenser

Jie JI, Huide FU, Hanfeng HE, Gang PEI,

期刊论文

CO capture and sequestration source-sink match optimization in Jing-Jin-Ji region of China

Zhong ZHENG , Dan GAO , Linwei MA , Zheng LI , Weidou NI ,

期刊论文

Identification and ranking of the risky organic contaminants in the source water of the Danjiangkou reservoir

Qingwei BU, Donghong WANG, Zijian WANG, Junnong GU

期刊论文

Acid Orange 7 degradation using methane as the sole carbon source and electron donor

期刊论文

Optimization model analysis of centralized groundwater source heat pump system in heating season

Shilei LU,Yunfang QI,Zhe CAI,Yiran LI

期刊论文

THAI experimental research on hydrogen risk and source term related safety systems

期刊论文

Toward separation at source: Evolution of Municipal Solid Waste management in China

Jianguo Liu, Shuyao Yu, Yixuan Shang

期刊论文

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