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Localized high-concentration electrolytes for lithium metal batteries: progress and prospect

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10,   Pages 1354-1371 doi: 10.1007/s11705-022-2286-4

Abstract: With the increasing development of digital devices and electric vehicles, high energy-density rechargeable batteries are strongly required. As one of the most promising anode materials with an ultrahigh specific capacity and extremely low electrode potential, lithium metal is greatly considered an ideal candidate for next-generation battery systems. Nevertheless, limited Coulombic efficiency and potential safety risks severely hinder the practical applications of lithium metal batteries due to the inevitable growth of lithium dendrites and poor interface stability. Tremendous efforts have been explored to address these challenges, mainly focusing on the design of novel electrolytes. Here, we provide an overview of the recent developments of localized high-concentration electrolytes in lithium metal batteries. Firstly, the solvation structures and physicochemical properties of localized high-concentration electrolytes are analyzed. Then, the developments of localized high-concentration electrolytes to suppress the formation of dendritic lithium, broaden the voltage window of electrolytes, enhance safety, and render low-temperature operation for robust lithium metal batteries are discussed. Lastly, the remaining challenges and further possible research directions for localized high-concentration electrolytes are outlined, which can promisingly render the practical applications of lithium metal batteries.

Keywords: high-concentration electrolyte     localized high-concentration electrolyte     lithium metal battery     solidelectrolyte interphase     dendrite    

Boosting the direct conversion of NHHCO electrolyte to syngas on Ag/Zn zeolitic imidazolate framework

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 9,   Pages 1196-1207 doi: 10.1007/s11705-022-2289-1

Abstract: which were used for the first time for boosting the direct conversion of NH4HCO3 electrolyteIts activity is comparable to that of the CO2-saturated NH4HCO3 electrolyte

Keywords: Ag catalyst     zeolitic imidazolate framework     CO2 electroreduction     ammonium bicarbonate electrolyte    

A review on the development of electrolytes for lithium-based batteries for low temperature applications

Frontiers in Energy 2023, Volume 17, Issue 1,   Pages 43-71 doi: 10.1007/s11708-022-0853-5

Abstract: cosolvents, additives, and salts have been researched to fine tune the conductivity, solvation, and solid-electrolyteWith these objectives in mind, tailoring of the electrolyte with higher-capacity materials such as lithiumThis review paper highlights the progression of electrolyte research for low temperature performance

Keywords: electrolyte     lithium-ion     low temperature     aerospace     solid-electrolyte interface    

Recent advances toward high voltage, EC-free electrolytes for graphite-based Li-ion battery

Tong Zhang, Elie Paillard

Frontiers of Chemical Science and Engineering 2018, Volume 12, Issue 3,   Pages 577-591 doi: 10.1007/s11705-018-1758-z

Abstract: graphite anode operation–also required for high energy density batteries–by stabilizing the electrode/electrolyteThis review covers electrolyte compositions, with the widespread use of additives, the change in mainconcentration, but also reports on graphite protection strategies, by coatings or artificial solid electrolyte

Keywords: lithium-ion     electrolyte     solid electrolyte interphase     additives     high voltage     graphite    

Effect of electrolyte concentration on the tribological performance of MAO coatings on aluminum alloys

Chao Wang, Jun Chen, Jihua He, Jing Jiang, Qinyong Zhang

Frontiers of Chemical Science and Engineering 2020, Volume 14, Issue 6,   Pages 1065-1071 doi: 10.1007/s11705-019-1909-x

Abstract: In order to investigate the effect of the electrolyte concentration on the properties of MAO coatings

Keywords: aluminum alloy     micro-arc oxidation     coating     electrolyte concentration     tribological performance    

Review of characterization and modeling of polymer electrolyte fuel cell catalyst layer: The blessing

Jun HUANG, Zhe LI, Jianbo ZHANG

Frontiers in Energy 2017, Volume 11, Issue 3,   Pages 334-364 doi: 10.1007/s11708-017-0490-6

Abstract: Ionomer impregnation represents a milestone in the evolution of polymer electrolyte fuel cell (PEFC)

Keywords: polymer electrolyte fuel cell     ultra-thin catalyst layer     electrostatic interactions     characterization and    

Characterization and comparison of organic functional groups effects on electrolyte performance for vanadium

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 9,   Pages 1221-1230 doi: 10.1007/s11705-023-2298-8

Abstract: sulfonic acid, sulfonic acid, amino methane sulfonic acid, and taurine are used to overcome the low electrolyteWhen compared to the pristine electrolyte (0.22 Ah, 5.0 Wh·L–1, 85.0%), the results show thatThe acetic acid electrolyte is more conducive to the low-temperature stability of the V(II) electrolytesub>H group, specifically the coaction of the –NH2 and –SO3H groups, improves electrolyte

Keywords: vanadium redox flow battery     functional groups     organic additives     energy density     stability    

The composite electrolyte materials for low-temperature solid oxide fuel cell

Xie Fucheng,Wang Cheng,Mao Zongqiang

Strategic Study of CAE 2013, Volume 15, Issue 2,   Pages 72-76

Abstract: Functional composite electrolytes are regarded as the promising electrolyte materials, and the ionThe recent progress in composite electrolyte, the characteristics, type and conductive mechanismof composite electrolyte were introduced in the paper.

Keywords: low-temperature SOFC     composite electrolyte     conductive mechanism    

Chemical composition and formation mechanisms in the cathode-electrolyte interface layer of lithium manganese

Sahithya REDDIVARI, Christian LASTOSKIE, Ruofei WU, Junliang ZHANG

Frontiers in Energy 2017, Volume 11, Issue 3,   Pages 365-373 doi: 10.1007/s11708-017-0500-8

Abstract: Although a thin layer of electrolyte decomposition products is known to form at the cathode surface,The ReaxFFMD simulations reveal that the cathode-electrolyte interface layer is composed of oxidationproducts of electrolyte solvent molecules including aldehydes, esters, alcohols, polycarbonates, andThe oxidation reaction pathways for the electrolyte solvent molecules involve the formation of surfaceAn overall cathode-electrolyte interface reaction scheme is proposed based on the molecular simulation

Keywords: lithium manganese oxide batteries     reactive force field (ReaxFF)     cathode-electrolyte interface layer     molecular    

The method for the conductivity measurement of electrolyte and electrode materials in solid oxide fuel

He Beibei,Pan Xin,Xia Changrong

Strategic Study of CAE 2013, Volume 15, Issue 2,   Pages 57-65

Abstract: Some commonly used measurements for electrolyte and electrode materials, such as total conductivity

Keywords: conduction mechanism     electrolyte     electrode     conductivity     solid oxide fuel cell    

synthesis of double-shell truncated octahedral Pt-Ni alloys for oxygen reduction reaction of polymer electrolyte

Xiashuang LUO, Yangge GUO, Hongru ZHOU, Huan REN, Shuiyun SHEN, Guanghua WEI, Junliang ZHANG

Frontiers in Energy 2020, Volume 14, Issue 4,   Pages 767-777 doi: 10.1007/s11708-020-0667-2

Abstract: offer an exceptional electrocatalytic activity toward the oxygen reduction reaction (ORR) of polymer electrolytepower density of the dealloyed truncated octahedral Pt Ni core-shell alloy catalyst based membrane electrolyte

Keywords: dealloyed Pt-Ni alloys     truncated octahedron     double-shell     thermal annealing     oxygen reduction reaction (ORR)    

Electrolyte material progress of low-temperature SOFC

Han Da,Wu Tianzhi,Xin Xianshuang,Wang Shaorong,Zhan Zhongliang

Strategic Study of CAE 2013, Volume 15, Issue 2,   Pages 66-71

Abstract: The principal approach to achieve reduction in operating temperature is to reduce the electrolyte thicknessand adopt alternative electrolyte materials that exhibit much higher ionic conductivities than the state-of-the-artyttria-stabilized zirconia electrolyte at comparable temperatures.Here, electrolyte materials for low-temperature SOFC, including lanthanum gallate-based, 

Keywords: low-temperature SOFC     new electrolyte     ion conductivity    

Comparative analysis of ceramic-carbonate nanocomposite fuel cells using composite GDC/NLC electrolyte

Muhammad I. Asghar, Sakari Lepikko, Janne Patakangas, Janne Halme, Peter D. Lund

Frontiers of Chemical Science and Engineering 2018, Volume 12, Issue 1,   Pages 162-173 doi: 10.1007/s11705-017-1642-2

Abstract: La Sr Co Fe O (LSCF), was performed for a ceramic-carbonate nanocomposite fuel cell using composite electrolyteFinally, a fuel cell was fabricated using GDC/NLC nanocomposite electrolyte and its composite with NiO

Keywords: electrode     fuel cell     low-temperature     nanocomposite     perovskite    

Fabrication and performance of PEN SOFCs with proton-conducting electrolyte

ZHONG Li, LUO Jingli, Karl Chuang

Frontiers of Chemical Science and Engineering 2007, Volume 1, Issue 1,   Pages 40-44 doi: 10.1007/s11705-007-0008-6

Abstract: A positive-electrolyte-negative (PEN) assembly solid oxide fuel cell (SOFC) with a thin electrolyte filmand cathode catalysts were pressed simultaneously and formed with the fabrication of nano-composite electrolyteThis design offered some advantageous configurations that diminished ohmic resistance between electrolyteimproved the performance of SOFC due to the reduction of membrane thickness and good contact between electrolytecm and 130 mW " cm for the PEN configuration with a Mo-Ni-S-based composite anode, nano-composite electrolyte

Keywords: proton-conducting     positive-electrolyte-negative     temperature operation     Mo-Ni-S-based composite     advantageous    

Modeling the methyldiethanolamine-piperazine scrubbing system for CO

Stefania Moioli,Laura A. Pellegrini

Frontiers of Chemical Science and Engineering 2016, Volume 10, Issue 1,   Pages 162-175 doi: 10.1007/s11705-016-1555-5

Abstract: In this work a thermodynamic analysis with the Electrolyte-NRTL model has been performed for systems

Keywords: vapor-liquid equilibrium     methyldietanolamine     piperazine     regression     Electrolyte-NRTL    

Title Author Date Type Operation

Localized high-concentration electrolytes for lithium metal batteries: progress and prospect

Journal Article

Boosting the direct conversion of NHHCO electrolyte to syngas on Ag/Zn zeolitic imidazolate framework

Journal Article

A review on the development of electrolytes for lithium-based batteries for low temperature applications

Journal Article

Recent advances toward high voltage, EC-free electrolytes for graphite-based Li-ion battery

Tong Zhang, Elie Paillard

Journal Article

Effect of electrolyte concentration on the tribological performance of MAO coatings on aluminum alloys

Chao Wang, Jun Chen, Jihua He, Jing Jiang, Qinyong Zhang

Journal Article

Review of characterization and modeling of polymer electrolyte fuel cell catalyst layer: The blessing

Jun HUANG, Zhe LI, Jianbo ZHANG

Journal Article

Characterization and comparison of organic functional groups effects on electrolyte performance for vanadium

Journal Article

The composite electrolyte materials for low-temperature solid oxide fuel cell

Xie Fucheng,Wang Cheng,Mao Zongqiang

Journal Article

Chemical composition and formation mechanisms in the cathode-electrolyte interface layer of lithium manganese

Sahithya REDDIVARI, Christian LASTOSKIE, Ruofei WU, Junliang ZHANG

Journal Article

The method for the conductivity measurement of electrolyte and electrode materials in solid oxide fuel

He Beibei,Pan Xin,Xia Changrong

Journal Article

synthesis of double-shell truncated octahedral Pt-Ni alloys for oxygen reduction reaction of polymer electrolyte

Xiashuang LUO, Yangge GUO, Hongru ZHOU, Huan REN, Shuiyun SHEN, Guanghua WEI, Junliang ZHANG

Journal Article

Electrolyte material progress of low-temperature SOFC

Han Da,Wu Tianzhi,Xin Xianshuang,Wang Shaorong,Zhan Zhongliang

Journal Article

Comparative analysis of ceramic-carbonate nanocomposite fuel cells using composite GDC/NLC electrolyte

Muhammad I. Asghar, Sakari Lepikko, Janne Patakangas, Janne Halme, Peter D. Lund

Journal Article

Fabrication and performance of PEN SOFCs with proton-conducting electrolyte

ZHONG Li, LUO Jingli, Karl Chuang

Journal Article

Modeling the methyldiethanolamine-piperazine scrubbing system for CO

Stefania Moioli,Laura A. Pellegrini

Journal Article