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Online single particle analysis of chemical composition and mixing state of crop straw burning particles

Juntao HUO,Xiaohui LU,Xinning WANG,Hong CHEN,Xingnan YE,Song Gao,Deborah S. Gross,Jianmin CHEN,Xin YANG

《环境科学与工程前沿（英文）》 2016年 第10卷 第2期   页码 244-252 doi: 10.1007/s11783-015-0768-z

摘要： Fresh straw burning (SB) particles were generated in the laboratory by the combustion of rice straw and corn straw. The chemical composition and mixing state of the fresh SB particles were investigated by an Aerosol Time-of-Flight Mass Spectrometer (ATOFMS). Based on the mass spectral patterns, the SB particles were clustered into four major types: Salt, Organic Carbon (OC), Elemental Carbon (EC), and internally mixed particles of EC and OC (EC-OC). In addition, particles containing ash, polycyclic aromatic hydrocarbons, heavy metals or nicotine were also observed. Physical and chemical changes of the SB particles immediately after the emission were analyzed with highly time-resolved data. During the aging processes, the average particle size increased steadily. Freshly emitted organic compounds were gradually oxidized to more oxygenated compounds in the OC-containing particles. Meanwhile, an important displacement reaction (2KCl+ → K SO + 2Cl ) was observed. The marker ions for SB particles were optimized and applied to identify the SB particles in the ambient atmosphere. The fluctuation of the number fraction of ambient SB particles sorted by ATOFMS agrees well with that of water soluble K measured by an online ion chromatography, demonstrating that the optimized marker ions could be good tracers for SB particles in field measurements.

关键词： crop straw burning particles     mixing state     aging process     ATOFMS     ion markers    

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Performance and mechanism for cadmium and lead adsorption from water and soil by corn straw biochar

Tong Chi,Jiane Zuo,Fenglin Liu

《环境科学与工程前沿（英文）》 2017年 第11卷 第2期 doi: 10.1007/s11783-017-0921-y

摘要： Corn straw biochar prepared under 400 °C was the best Cd and Pb adsorption capacity Maximum adsorption capacity of Cd and Pb were 43.48 and 22.73 mg·g , respectively The dominant mechanism of Cd and Pb adsorption was precipitation Biochar could reduce the bioavailability of heavy metals when mixed with soil Cadmium (Cd) and lead (Pb) in water and soil could be adsorbed by biochar produced from corn straw. Biochar pyrolyzed under 400°C for 2 h could reach the ideal removal efficiencies (99.24% and 98.62% for Cd and Pb, respectively) from water with the biochar dosage of 20 g·L and initial concentration of 20 mg·L . The pH value of 4–7 was the optimal range for adsorption reaction. The adsorption mechanism was discussed on the basis of a range of characterizations, including X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), Fourier transform infrared spectroscopy (FTIR) and Raman analysis; it was concluded as surface complexation with active sorption sites (-OH, -COO-), coordination with π electrons (C= C, C= O) and precipitation with inorganic anions (OH , CO , SO ) for both Cd and Pb. The sorption isotherms fit Langmuir model rather than Freundlich model, and the saturated sorption capacities for Cd and Pb were 38.91 mg·g and 28.99 mg·g , respectively. When mixed with soil, biochar could effectively increase alkalinity and reduce bioavailability of heavy metals. Thus, biochar derived from corn straw would be a green material for both removal of heavy metals and amelioration of soil.

关键词： Corn straw     Biochar     Heavy metals     Sorption isotherm     Bioavailability    

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Direct ethanol production from rice straw by coculture with two high-performing fungi

Maki TAKANO, Kazuhiro HOSHINO

《化学科学与工程前沿（英文）》 2012年 第6卷 第2期   页码 139-145 doi: 10.1007/s11705-012-1281-6

摘要： To develop efficient and economical direct ethanol production from fine rice straw crashed mechanically, two high-performing fungi, which can secret hyperactive cellulases and/or ferment effectively various sugars, were selected from some strains belong to preserved in our laboratory. The simultaneous saccharification and fermentation (SSF) by coculture with these fungi was investigated. The screening of high-performing fungi resulted in the selection of NBRC 4572 as an ethanol-producing fungus and NBRC 5398 as a cellulase-secreting fungus. The strain 4572 produced ethanol aerobically from glucose and xylose in high yields of 0.420 g/g at 36 h and 0.478 g/g at 60 h, respectively, but secreted fairly low cellulases. On the other hand, the strain 5398 also produced ethanol from glucose in yield of 0.340 g/g though it had a little growth in xylose culture. However, it secreted hyperactive cellulases that are essential for hydrolysis of rice straw in culture and the maximum activities of endo-β-glucanase and β-glucosidase were 2.11 U/L and 1.47 U/L, respectively. In SSF of rice straw by coculture with two fungi selected, the ethanol production reached 1.28 g/L after 96 h when the inoculation ratio of the strain 5398 to the strain 4572 was 9.

关键词： Mucor circinelloides     ethanol production     cellulase secretion     SSF     coculture     rice straw    

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Fabrication of cellulose aerogel from wheat straw with strong absorptive capacity

Jian LI,Caichao WAN,Yun LU,Qingfeng SUN

《农业科学与工程前沿（英文）》 2014年 第1卷 第1期   页码 46-52 doi: 10.15302/J-FASE-2014004

摘要： An effectively mild solvent solution containing NaOH/PEG was employed to dissolve the cellulose extracted from the wheat straw. With further combined regeneration process and freeze-drying, the cellulose aerogel was successfully obtained. Scanning electron microscope, X-ray diffraction technique, Fourier transform infrared spectroscopy, and Brunauer-Emmett-Teller were used to characterize this cellulose aerogel of low density (about 40 mg·cm ) and three-dimensional network with large specific surface area (about 101 m ·g ). Additionally, with a hydrophobic modification by trimethylchlorosilane, the cellulose aerogel showed a strong absorptive capacity for oil and dye solutions.

关键词： cellulose aerogel     absorptive capacity     waste wheat straw     freeze-drying    

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Isolation of highly purity cellulose from wheat straw using a modified aqueous biphasic system

Lifeng YAN, Yi ZHAO, Qing GU, Wan LI

《化学科学与工程前沿（英文）》 2012年 第6卷 第3期   页码 282-291 doi: 10.1007/s11705-012-0901-5

摘要： Cellulose samples with molecular weights ranging from 8.39 × 10 to 11.00 × 10 g/mol were obtained from wheat straw. The dewaxed wheat straw was pretreated with aqueous hydrochloric acid followed by delignification using an environmentally benign poly(ethyleneglycol)/salt aqueous biphasic system. The yield of cellulose was in the range of 48.9%–55.5% and the cellulose contained 1.2%–3.2% hemicelluloses, and 0.97%–3.47% lignin. All the isolated cellulose samples could be directly dissolved in a 6 wt-% NaOH/4 wt-% urea aqueous solution through a precooling-thawing process to form a homogenous solution. The separation process was investigated and the obtained cellulose and its solution were characterized by Fourier transform infrared spectroscopy, scanning electron microscopy and energy dispersive X-ray apparatus, and X-ray diffraction. The results revealed that aqueous soluble cellulose can be directly prepared from wheat straw by this method and this study opens a novel pathway to prepare cellulosic materials from agricultural waste.

关键词： cellulose     straw     separation     aqueous solution    

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Integrated benefits of power generation by straw biomass —A case study on the Sheyang Straw Power Plants

Xiaoshun LI , Futian QU , Dongmei JIANG , Peixin ZHU ,

《环境科学与工程前沿（英文）》 2009年 第3卷 第3期   页码 348-353 doi: 10.1007/s11783-009-0026-3

摘要： Power generation using straw biomass has quantifiable benefits from an economic, ecological, and sociological perspective in China. The methods used to construct the assessment models of these integrated benefits were the revenue capitalization approach and the discounted-cash-flow approach. The results indicated that a straw power plant with the capacity of 2.50×10 W and burning 1.23×10 tons of cotton straw could annually supply 1.40×10 kWh of power. However, it would not be until six years later that these results could be measured. Over the long term, the gross benefits could reach up to 4.63×10 Yuan. Therefore, the total benefits are expected to be 1.18 × 10 Yuan if all available straw resources are used to generate power. The policy implication showed that the long-term integrated benefits of power generation by straw biomass outweighed the short-term benefits. This is the main incentive to use straw biomass for power generation in the future.

关键词： straw biomass resources     power generation     renewable energy     Sheyang county    

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煤净化燃烧及伴生物产品化

朱雪芳

《中国工程科学》 1999年 第1卷 第1期   页码 53-57

摘要：

煤净化燃烧及伴生物产品化新工艺，是在电厂燃煤中加特制的掺烧剂共同粉磨产生亲合颗粒，喷入锅炉内进行亲合煅烧。保证供热发电的同时实现降低残炭、提高粉煤灰活性、固结脱硫、降低Nox、CO2，并将全部固态伴生物在具有速烧速冷的燃煤锅炉内直接生成优质水泥熟料；实现基本消除燃烧的全部污染（气体和固体污染），且不产生二次污染，从而达到清洁生产的目的。

关键词： 净化燃烧     伴生物产品化     速烧速冷     固结脱硫     亲合颗料     亲合煅烧    

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Effect of mulching with maize straw on water infiltration and soil loss at different initial soil moistures

Yifu ZHANG,Hongwen LI,Jin HE,Qingjie WANG,Ying CHEN,Wanzhi CHEN,Shaochun MA

《农业科学与工程前沿（英文）》 2016年 第3卷 第2期   页码 161-170 doi: 10.15302/J-FASE-2016104

摘要： Mulching and soil water content (SWC) have a significant impact on soil erosion, and this study investigated the effect of straw mulching on water infiltration and soil loss under different initial SWC treatments in a rainfall simulation experiment conducted in northern China. Increasing initial SWC can decrease soil infiltration and increase soil loss. During an 80 mm rainfall event (80 mm·h for 60 min), 8%, 12% and 16% initial SWC treatments decreased cumulative infiltration by 8.7%, 42.5% and 58.1%, and increased total sediment yield by 44, 146 and 315 g, respectively, compared to 4% initial SWC. However, in all the straw mulching treatments, there was no significant difference in stable infiltration rate between the different initial SWC treatments. For all initial SWC treatments, straw mulching of 30% or more significantly enhanced water infiltration by over 31% and reduced soil loss by over 49%, compared to the unmulched treatment. Taking into consideration the performance of no-till planters, a maize straw mulching rate of 30% to 60% (1400–3100 kg·hm ) is recommended for the conservation of water and soil in northern China.

关键词： infiltration     initial soil water content     rainfall simulation     soil loss     straw mulching    

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Formation of secondary inorganic aerosol in a frigid urban atmosphere

《环境科学与工程前沿（英文）》 2022年 第16卷 第2期 doi: 10.1007/s11783-021-1452-0

摘要：

•Harbin showed relatively high threshold RH (80%) for apparent increase of SOR.

关键词： Haze     Sulfate     Nitrate     Heterogeneous chemistry     Biomass burning     Northeast China    

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METAGENOMICS COMBINED WITH HIGH-THROUGHPUT SEQUENCING REVEALS THE METHANOGENIC POTENTIAL OF FRESH CORN STRAW

《农业科学与工程前沿（英文）》 2023年 第10卷 第3期   页码 403-423 doi: 10.15302/J-FASE-2022471

摘要：

● Methane production from fresh straw was 7.50% higher than dry straw.

关键词： fresh corn straw     high solid anaerobic digestion     metagenomics     microbial communities     thermophilic    

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Effects of cotton straw amendment on soil fertility and microbial communities

Wuren HUANG, Zhihui BAI, Daniel HOEFEL, Qing HU, Xin LV, Guoqiang ZHUANG, Shengjun XU, Hongyan QI, Hongxun ZHANG

《环境科学与工程前沿（英文）》 2012年 第6卷 第3期   页码 336-349 doi: 10.1007/s11783-011-0337-z

摘要： Maintaining soil fertility, while controlling pollution from excessive chemical fertilizer application is important for keeping soil productivity of sustainable agriculture. Variety of straws have been used and proven to be good soil amendments for increasing soil organic matter (OM) and a range of additional soil nutrients. However, little is known about the utilization of cotton straw for soil amendment. To better understand the mechanism behind cotton straw soil amendments, investigations were performed upon cucumber seedlings, where changes to soil nutrients and microbial communities were investigated. The results revealed that the cotton straw application promoted the cucumber seedling growth by significantly increasing the soil OM, available nitrogen, available phosphorus, and available potassium. The concentration of cotton straw was positively correlated to both the number of the culturable microorganisms and also the total microbial biomass within soil. Furthermore, assessment of cotton straw application using Biolog metabolic profiling and phospholipid fatty acid analysis revealed that such application increased the microbial community metabolic activity, and markedly changed the structure of microbial community. 16S rRNA gene clone library construction and phylogenetic analysis of soil bacteria revealed - Proteobacteria sequences dominated the cotton straw amendment soil, comprising 27.8% of the total number of analyzed sequences, while they were less represented in control soil (13.4%). On the contrary, the Sphingobacteria (7.8%) and Verrucomicrobia (2.4%) in the cotton straw amendment soil decreased after application when compared to the control soil 15.2% and 15.2%.

关键词： cotton straw     soil amendments     microbial diversity     Biolog     phospholipid fatty acid     16S rRNA gene clone library    

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Calculation of collision frequency function for aerosol particles in free molecule regime in presence

Xiaowei LUO, Yannick BENICHOU, Suyuan YU

《能源前沿（英文）》 2013年 第7卷 第4期   页码 506-510 doi: 10.1007/s11708-013-0275-5

摘要： The collision frequency function for aerosol particles has already been calculated for the free molecule regime and for the continuum range. The present work, taking into account the influence of internal force fields such as magnetic force, electric force and molecular forces, created by particles themselves, recalculated the collision frequency in the case of particles much smaller than the mean free path of the gas (free molecule regime). Attractive forces increase naturally the collision frequency, while repulsive forces decrease it. The calculation was performed for all types of central forces deriving from a potential, including Coulomb forces and Van der Waals forces.

关键词： aerosol particles     collision frequency function     coagulation    

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Polymer-nanoinorganic particles composite membranes: a brief overview

Zhen-liang XU, Li-yun YU, Ling-feng HAN

《化学科学与工程前沿（英文）》 2009年 第3卷 第3期   页码 318-329 doi: 10.1007/s11705-009-0199-0

摘要： Polymer-nanoinorganic particles composite membranes present an interesting approach for improving the physical and chemical, as well as separation properties of polymer membranes, because they possess characteristics of both organic and inorganic membranes such as good permeability, selectivity, mechanical strength, thermal stability and so on. The preparations and structures of polymer-nanoinorganic particles composite membranes and their unique properties are reviewed.

关键词： polymer     nanoinorganic particles     composite membranes    

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Transparent exopolymer particles (TEPs)-associated protobiofilm: A neglected contributor to biofouling

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1361-7

摘要：

• Bacteria could easily and quickly attached onto TEP to form protobiofilms.

关键词： Transparent exopolymer particles (TEPs)     TEP-protobiofilm     Bacteria attachment     Biofouling of membrane    

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Dynamic characteristics of molten droplets and hot particles falling in liquid pool

Liangxing LI, Weimin MA, Huixiong LI, Tingkuan CHEN,

《能源前沿（英文）》 2010年 第4卷 第2期   页码 246-251 doi: 10.1007/s11708-009-0077-y

摘要： The dynamic characteristics of molten droplets and hot particles at the very beginning of their fall into coolant pools are presented. The falling course of a single droplet or a single hot particle was recorded by a high-speed camera and a curve of velocity . time was obtained. Emphasis was placed on the effects of the droplet’s size and temperature, the coolant’s temperature and properties, and the droplet’s physical properties on the moving behavior. The results for the all cases showed that the velocity of a falling droplet/particle decreased rapidly but rebounded shortly, at the beginning of droplet/particle falling in the coolant. Following such a V-shaped evolution in velocity, the droplet/particle slows down gradually to a comparatively steady velocity. An increase in either coolant temperature or droplet temperature results in a larger velocity variation in the “J-region”, but a smaller deceleration when it moves out of the “J-region”. The elevated volatility of a coolant leads to a steeper deceleration in the “J-region” and beyond. The bigger size of a particle leads to a greater velocity variation in the “J-region” and terminal velocity. A high melting point and thermal conductivity as well as lower heat capacity contribute to dramatic variation in the “J-region” and low terminal velocity.

关键词： dynamic characteristics     molten droplets     high-temperature particles     fuel and coolant interactions    

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标题 作者 时间 类型 操作

Online single particle analysis of chemical composition and mixing state of crop straw burning particles

Juntao HUO,Xiaohui LU,Xinning WANG,Hong CHEN,Xingnan YE,Song Gao,Deborah S. Gross,Jianmin CHEN,Xin YANG

期刊论文

Performance and mechanism for cadmium and lead adsorption from water and soil by corn straw biochar

Tong Chi,Jiane Zuo,Fenglin Liu

期刊论文

Direct ethanol production from rice straw by coculture with two high-performing fungi

Maki TAKANO, Kazuhiro HOSHINO

期刊论文

Fabrication of cellulose aerogel from wheat straw with strong absorptive capacity

Jian LI,Caichao WAN,Yun LU,Qingfeng SUN

期刊论文

Isolation of highly purity cellulose from wheat straw using a modified aqueous biphasic system

Lifeng YAN, Yi ZHAO, Qing GU, Wan LI

期刊论文

Integrated benefits of power generation by straw biomass —A case study on the Sheyang Straw Power Plants

Xiaoshun LI , Futian QU , Dongmei JIANG , Peixin ZHU ,

期刊论文

煤净化燃烧及伴生物产品化

朱雪芳

期刊论文

Effect of mulching with maize straw on water infiltration and soil loss at different initial soil moistures

Yifu ZHANG,Hongwen LI,Jin HE,Qingjie WANG,Ying CHEN,Wanzhi CHEN,Shaochun MA

期刊论文

Formation of secondary inorganic aerosol in a frigid urban atmosphere

期刊论文

METAGENOMICS COMBINED WITH HIGH-THROUGHPUT SEQUENCING REVEALS THE METHANOGENIC POTENTIAL OF FRESH CORN STRAW

期刊论文

Effects of cotton straw amendment on soil fertility and microbial communities

Wuren HUANG, Zhihui BAI, Daniel HOEFEL, Qing HU, Xin LV, Guoqiang ZHUANG, Shengjun XU, Hongyan QI, Hongxun ZHANG

期刊论文

Calculation of collision frequency function for aerosol particles in free molecule regime in presence

Xiaowei LUO, Yannick BENICHOU, Suyuan YU

期刊论文

Polymer-nanoinorganic particles composite membranes: a brief overview

Zhen-liang XU, Li-yun YU, Ling-feng HAN

期刊论文

Transparent exopolymer particles (TEPs)-associated protobiofilm: A neglected contributor to biofouling

期刊论文

Dynamic characteristics of molten droplets and hot particles falling in liquid pool

Liangxing LI, Weimin MA, Huixiong LI, Tingkuan CHEN,

期刊论文