基于车载测试的轻型汽油车实际道路黑碳排放特征研究
郑轩 , 何立强 , 何晓旖 , 张少君 , 曹翊寰 , 郝吉明 , 吴烨
工程(英文) ›› 2022, Vol. 16 ›› Issue (9) : 73 -81.
基于车载测试的轻型汽油车实际道路黑碳排放特征研究
Real-Time Black Carbon Emissions from Light-Duty Passenger Vehicles Using a Portable Emissions Measurement System
黑碳(BC)是影响气候的第二大人为因素,但BC的辐射效应与其燃烧来源息息相关。BC的人为排放源主要是道路机动车。然而,目前轻型汽油车(LDPV)的BC排放估算存在很大的不确定性,尤其缺乏使用车载测试(PEMS)方法获得的估算结果。本研究开发了一款新型轻型车PEMS平台,并对10 辆在用车进行了实际道路BC排放测试。结果表明,缸内直喷(GDI)车辆BC排放因子(EF)的范围为1.10~1.56 mg∙ km−1,是进气道喷射(PFI)车辆EFs(0.10~0.17 mg∙km−1)的11 倍。冷启动阶段BC排放贡献显著,可占排放总量的2%~33%。与此同时,相对BC EFs 和平均车速存在强相关性(R2 = 0.70),这表明缓解交通拥堵可以有效减少BC排放。此外,BC与颗粒物数浓度(PN)排放呈线性相关(R2 = 0.90)。与PFI 车辆相比,所有速度区间内GDI车辆的PN与BC瞬时排放速率的比值对车辆比功率-速度(VSP-v)的增加并不敏感。
Black carbon (BC) is considered the second largest anthropogenic climate forcer, but the radiative effects of BC are highly correlated with its combustion sources. On-road vehicles are an important source of anthropogenic BC. However, there are major uncertainties in the estimates of the BC emissions from on-road light-duty passenger vehicles (LDPVs), and results obtained with the portable emissions measurement system (PEMS) method are particularly lacking. We developed a PEMS platform and evaluated the on-road BC emissions from ten in-use LDPVs. We demonstrated that the BC emission factors (EFs) of gasoline direction injection (GDI) engine vehicles range from 1.10 to 1.56 mg·km−1, which are higher than the EFs of port fuel injection (PFI) engine vehicles (0.10–0.17 mg·km−1) by a factor of 11. The BC emissions during the cold-start phase contributed 2%–33% to the total emissions. A strong correlation (R2 = 0.70) was observed between the relative BC EFs and average vehicle speed, indicating that traffic congestion alleviation could effectively mitigate BC emissions. Moreover, BC and particle number (PN) emissions were linearly correlated (R2 = 0.90), and compared to PFI engine vehicles, the instantaneous PN-to-BC emission rates of GDI engine vehicles were less sensitive to vehicle-specific power-to-velocity (VSPV) increase in all speed ranges.
Black carbon / Light-duty gasoline vehicles / Portable emissions measurement system / Real-time emissions
| Vehicle number | Manufacturer | Model year a | Main application | Emission standard | Curb weight (kg) | Fuel injection system | After-treatment device | Engine size (L) | Mileage traveled (km) | Ambient temperature (℃) |
|---|---|---|---|---|---|---|---|---|---|---|
| #1 | Ford | 2012 | Private cars | China 4 | 1340 | PFI | TWC | 1.8 | 130957 | 2 |
| #2 | TOYOTA | 2012 | Private cars | China 4 | 1300 | PFI | TWC | 1.6 | 58747 | 33 |
| #3 | Buick | 2015 | Private cars | China 4 | 1430 | PFI | TWC | 1.4 | 91334 | 21 |
| #4 | Buick | 2015 | Private cars | China 4 | 1595 | PFI | TWC | 2.4 | 118347 | 3 |
| #5 | Volkswagen | 2016 | Private cars | China 5 | 1265 | PFI | TWC | 1.6 | 104611 | 22 |
| #6 | Buick | 2017 | Privatecars | China 5 | 1225 | PFI | TWC | 1.5 | 57949 | 24 |
| #7 | Volkswagen | 2014 | Private cars | China 4 | 1600 | GDI | TWC | 1.8 | 28976 | 22 |
| #8 | Dongfeng | 2016 | Private cars | China 5 | 1305 | GDI | TWC | 1.2 | 72495 | 33 |
| #9 | Honda | 2018 | Private cars | China 5 | 1205 | GDI | TWC | 1.5 | 11367 | 27 |
| #10 | Chevrolet | 2018 | Private cars | China 5 | 1520 | GDI | TWC | 1.5 | 50912 | 3 |
| Study | Testing method and instruments | Model years | Distance specific emission factors (mg·km-1) | Fuel consumption specific emission factors (mg·km-1) | ||
|---|---|---|---|---|---|---|
| PFI | GDI | PFI | GDI | |||
| This study | PEMS | 2012‒2015 | 0.10‒0.17 | 1.10‒1.56 | 0.73‒3.61 | 15.61‒24.85 |
| Ref. | PEMS | 2017‒2018 | — | 0.11‒1.00 | — | — |
| Ref. | On-board tailpipe | 2006‒2012 | — | — | 0.57 ± 1.19 | — |
| Ref. | Dynamometer | 1993‒2014 | 0.05‒0.33 | 6.5‒7.6 | 1.70‒8.90 | — |
| Ref. | Dynamometer | 1998‒2011 | 0.06‒2.20 | 1.09 | — | 36.00 |
| Ref. | Dynamometer | 2010‒2012 | 0.11‒2.04 | 1.33‒4.42 | — | — |
| Ref. | Dynamometer | 2012‒2015 | 0.24‒0.67 | 1.62‒4.08 | — | — |
| Ref. | Roadside | 2010 fleet at Toronto | — | — | 71.2‒151.8 (not specified) | |
| Ref. | Roadside | 2016 fleet at Londrina | — | — | 25.7 ± 12.4 (not specified) | |
| Ref. | Plume Chasing | 2011 fleet at Slovenia | — | — | 280 (150‒460, not specified) | |
| Ref. | Plume Chasing | 2007 fleet at Los Angeles | — | — | 60 (not specified) | |
| Ref. | Plume Chasing | 2007 fleet at Beijing | — | — | 300 (not specified) | |
| Ref. | Tunnel | 2006 fleet at California | — | — | 26 ± 4 (LDVs, mostly powered by gasoline) | |
| Ref. | Tunnel | 2004 fleet at California | — | — | 30.4 (LDVs, mostly powered by gasoline) | |
| Ref. | Tunnel | 1997 fleet at California | — | — | 35 ± 3 (not specified) | |
| Ref. | Tunnel | 1996 fleet at California | — | — | 30 ± 2 (not specified) | |
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