s (CNNs) have been developed quickly in many real-world fields. However, CNN’s performance depends heavily on its hyperparameters, while finding suitable hyperparameters for CNNs working in application fields is challenging for three reasons: (1) the problem of encoding for different types of hyperparameters in CNNs, (2) expensive computational costs in evaluating candidate hyperparameter configuration, and (3) the problem of ensuring convergence rates and model performance during hyperparameter search. To overcome these problems and challenges, a hybrid-model optimization algorithm is proposed in this paper to search suitable hyperparameter configurations automatically based on the and (GPPSO) algorithm. First, a new encoding method is designed to efficiently deal with the CNN hyperparameter problem. Second, a hybrid-surrogate-assisted model is proposed to reduce the high cost of evaluating candidate hyperparameter configurations. Third, a novel activation function is suggested to improve the model performance and ensure the convergence rate. Intensive experiments are performed on imageclassification benchmark datasets to demonstrate the superior performance of GPPSO over state-of-the-art methods. Moreover, a case study on metal fracture diagnosis is carried out to evaluate the GPPSO algorithm performance in practical applications. Experimental results demonstrate the effectiveness and efficiency of GPPSO, achieving accuracy of 95.26% and 76.36% only through 0.04 and 1.70 GPU days on the CIFAR-10 and CIFAR-100 datasets, respectively.