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期刊论文 8

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Evaluating the impact of sulfamethoxazole on hydrogen production during dark anaerobic sludge fermentation

《环境科学与工程前沿(英文)》 2023年 第17卷 第1期 doi: 10.1007/s11783-023-1607-2

摘要:

● SMX promotes hydrogen production from dark anaerobic sludge fermentation.

关键词: Sulfamethoxazole     Hydrogen production     Dark anaerobic fermentation     Waste activated sludge    

Mechanisms for simultaneous ozonation of sulfamethoxazole and natural organic matters in secondary effluent

《环境科学与工程前沿(英文)》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1368-0

摘要:

• SMX was mainly degraded by hydrolysis, isoxazole oxidation and double-bond addition.

关键词: Sulfamethoxazole     Ozonation     Natural organic matters     Secondary effluent     Degradation mechanism    

Removal of sulfamethoxazole and trimethoprim from reclaimed water and the biodegradation mechanism

Qinqin Liu, Miao Li, Xiang Liu, Quan Zhang, Rui Liu, Zhenglu Wang, Xueting Shi, Jin Quan, Xuhui Shen, Fawang Zhang

《环境科学与工程前沿(英文)》 2018年 第12卷 第6期 doi: 10.1007/s11783-018-1048-5

摘要:

The artificial composite soil treatment system could efficiently remove SMX and TMP by biodegradation mechanism.

Bacillus subtilis from column reactors degraded SMX and TMP efficiently.

Bacillus subtilis biodegrades TMP to NH4+, and then converts NH4+ to NO3.

关键词: Trimethoprim     Sulfamethoxazole     Biodegradation     Aerobic nitrification    

Feasibility assessment of up-flow anaerobic sludge blanket treatment of sulfamethoxazole pharmaceutical

Yi Chen, Shilong He, Mengmeng Zhou, Tingting Pan, Yujia Xu, Yingxin Gao, Hengkang Wang

《环境科学与工程前沿(英文)》 2018年 第12卷 第5期 doi: 10.1007/s11783-018-1069-0

摘要:

The UASB system successfully treated sulfamethoxazole pharmaceutical wastewater.

High concentration sulfate of this wastewater was the main refractory factor.

UASB recovery performance after a few days of inflow arrest was studied.

The optimal UASB operating conditions for practical application were determined.

关键词: Up-flow anaerobic sludge blanket (UASB)     Methane production     Sulfate reduction     Sulfamethoxazole pharmaceutical wastewater     Electron flow     Recovery    

Theoretical insights into influence of additives on sulfamethoxazole crystal growth kinetics and mechanisms

《化学科学与工程前沿(英文)》 2023年 第17卷 第10期   页码 1503-1515 doi: 10.1007/s11705-022-2294-4

摘要: In this work, the influence of the initial chemical potential gradient, stirring speed, and polymer type on sulfamethoxazole (SMX) crystal growth kinetics was systematically investigated through density functional theory (DFT) calculations, experimental measurements and the two-step chemical potential gradient model. To investigate the influence of different conditions on the thermodynamic driving force of SMX crystal growth, SMX solubilities in different polymer solutions were studied. Four model polymers effectively improved SMX solubility. It was further found that polyvinylpyrrolidone (PVP) and hydroxypropyl methyl cellulose (HPMC) played a crucial role in inhibiting SMX crystal growth. However, polyethylene glycol (PEG) promoted SMX crystal growth. The effect of the polymer on the crystal growth mechanisms of SMX was further analyzed by the two-step chemical potential gradient model. In the system containing PEG 6000, crystal growth is dominated by the surface reaction. However, in the system containing PEG 20000, crystal growth is dominated by both the surface reaction and diffusion. In addition, DFT calculations results showed that HPMC and PVP could form strong and stable binding energies with SMX, indicating that PVP and HPMC had the potential ability to inhibit SMX crystal growth.

关键词: insoluble drugs     polymer     inhibition crystallization     crystal growth kinetics     DFT calculations    

Mesophilic and thermophilic anaerobic digestion of swine manure with sulfamethoxazole and norfloxacin

《环境科学与工程前沿(英文)》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1342-x

摘要:

• SMX addition had negative effect on acetoclastic methanogens in mesophilic AD.

关键词: Pig manure     Antibiotics     Anaerobic digestion     Resistance genes     Microbial community    

The removal of trimethoprim and sulfamethoxazole by a high infiltration rate artificial composite soil

Qinqin Liu,Miao Li,Fawang Zhang,Hechun Yu,Quan Zhang,Xiang Liu

《环境科学与工程前沿(英文)》 2017年 第11卷 第2期 doi: 10.1007/s11783-017-0920-z

摘要: Artificial composite soil treatment system with the high infiltration rate (1.394 m·d ) had a good removal efficiency of TMP (80%–90%) and SMX (60%–70%). The removal mechanism of TMP and SMX was mainly sorption and was related with hydrogeochemical process. Sulfamethoxzole (SMX) and trimethoprim (TMP), two combined-using sulfonamide antibiotics, have gained increasing attention in the surface water, groundwater and the drinking water because of the ecological risk. The removal of TMP and SMX by artificial composite soil treatment system (ACST) with different infiltration rates was systematically investigated using K , Na , Ca , Mg hydrogeochemical indexes. Batch experiments showed that the sorption onto the low-cost and commercially available clay ceramsites was effective for the removal of SMX and TMP from water. The column with more silty clay at high infiltration rate (1.394 m·d ) had removal rates of 80% to 90% for TMP and 60% to 70% for SMX. High SMX and TMP removal rates had a higher effluent concentration of K , Ca and Mg and had a lower effluent Na concentration. Removal was strongly related to sorption. The results showed that the removal of SMX and TMP was related to hydrogeochemical processes. In this study, ACST is determined to be applicable to the drinking water plants.

关键词: Trimethoprim     Sulfamethoxazole     Artificial composite soil treatment     Hydrogeochemical processes     Ion exchange    

Removal of trimethoprim and sulfamethoxazole in artificial composite soil treatment systems and diversity

Qinqin Liu, Miao Li, Rui Liu, Quan Zhang, Di Wu, Danni Zhu, Xuhui Shen, Chuanping Feng, Fawang Zhang, Xiang Liu

《环境科学与工程前沿(英文)》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1112-9

摘要:

• Novel ACST allowed biodegradation to effectively remove adsorbed SMX and TMP.

• Ammonia and nitrite were efficiently removed in ACSTs and water quality was improved.

关键词: Trimethoprim     Sulfamethoxazole     Reclaimed water     Biodegradation     Aerobic nitrification     Microbial community    

标题 作者 时间 类型 操作

Evaluating the impact of sulfamethoxazole on hydrogen production during dark anaerobic sludge fermentation

期刊论文

Mechanisms for simultaneous ozonation of sulfamethoxazole and natural organic matters in secondary effluent

期刊论文

Removal of sulfamethoxazole and trimethoprim from reclaimed water and the biodegradation mechanism

Qinqin Liu, Miao Li, Xiang Liu, Quan Zhang, Rui Liu, Zhenglu Wang, Xueting Shi, Jin Quan, Xuhui Shen, Fawang Zhang

期刊论文

Feasibility assessment of up-flow anaerobic sludge blanket treatment of sulfamethoxazole pharmaceutical

Yi Chen, Shilong He, Mengmeng Zhou, Tingting Pan, Yujia Xu, Yingxin Gao, Hengkang Wang

期刊论文

Theoretical insights into influence of additives on sulfamethoxazole crystal growth kinetics and mechanisms

期刊论文

Mesophilic and thermophilic anaerobic digestion of swine manure with sulfamethoxazole and norfloxacin

期刊论文

The removal of trimethoprim and sulfamethoxazole by a high infiltration rate artificial composite soil

Qinqin Liu,Miao Li,Fawang Zhang,Hechun Yu,Quan Zhang,Xiang Liu

期刊论文

Removal of trimethoprim and sulfamethoxazole in artificial composite soil treatment systems and diversity

Qinqin Liu, Miao Li, Rui Liu, Quan Zhang, Di Wu, Danni Zhu, Xuhui Shen, Chuanping Feng, Fawang Zhang, Xiang Liu

期刊论文