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Liquefaction and impurity separation of oxygen-bearing coal-bed methane

Qiuying LI, Yonglin JU, Li WANG,

《能源前沿（英文）》 2010年 第4卷 第3期   页码 319-325 doi: 10.1007/s11708-010-0115-9

摘要： Coal-bed methane (CBM) is a type of clean energy. However, most oxygen-bearing CBM have not yet to be utilized due to limited techniques, and when utilized, the discharged gas leads to resource wastage and environment pollution. In this paper, a liquefaction process is proposed and designed for the specified oxygen-bearing CBM obtained from the Daqing Qingshen gas field. The distillation column is employed to separate the oxygen and nitrogen components present in the CBM. HYSYS software is adopted to simulate the process, and the results reveal that the energy consumption of the whole liquefaction process is low. Moreover, oxygen and nitrogen are nearly removed completely, achieving a high-purity liquefied natural gas product with a high methane recovery rate. The applicability and safety of the liquefaction process are also analyzed. The simulation results can offer references for the separation of the oxygen component from CBM.

关键词： coal bed methane     oxygen-bearing     liquefaction     distillation    

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The catalytic effect of both oxygen-bearing functional group and ash in carbonaceous catalyst on CH 4

Weidong ZHANG, Yongfa ZHANG,

《化学科学与工程前沿（英文）》 2010年 第4卷 第2期   页码 147-152 doi: 10.1007/s11705-009-0242-1

摘要： A kind of new catalyst—carbonaceous catalyst—for CH-CO reformation has been developed in our laboratory. The effect of both oxygen-bearing functional group such as phenolic hydroxyl, carbonyl, carboxyl, and lactonic, and ash such as FeO, NaCO, and KCO in the carbonaceous catalyst on the CH-CO reforming has been investigated with a fixed-bed reactor. It has been found that the carbonaceous catalyst is an efficient catalyst on CO-CH reforming. With the decrease of oxygen-bearing functional group, the catalytic activity of carbonaceous catalyst decreases quickly. The oxygen-bearing functional groups play a significant role in the carbonaceous-catalyzed CO-CH reforming; the ash components in carbonaceous catalyst also have an important influence on the CO-CH reforming. FeO, NaCO, and KCO in the ash can catalyze the CO-CH reforming reaction; CaO has little effect on CO-CH reforming reaction. CaO can catalyze the gasification between carbonaceous catalyst and CO; AlO and MgO inhibit the CO-CH reforming.

关键词： oxygen-bearing functional     carboxyl     phenolic hydroxyl     CH-CO reformation     CO-CH reforming    

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Heterometallic cluster-based organic frameworks as highly active electrocatalysts for oxygen reductionand oxygen evolution reaction: a density functional theory study

《化学科学与工程前沿（英文）》 2023年 第17卷 第5期   页码 570-580 doi: 10.1007/s11705-022-2247-y

摘要： Recently, metal–organic frameworks are one of the potential catalytic materials for electrocatalytic applications. The oxygen reduction reaction and oxygen evolution reaction catalytic activities of heterometallic cluster-based organic frameworks are investigated using density functional theory. Firstly, the catalytic activities of heterometallic clusters are investigated. Among all heterometallic clusters, Fe2Mn–Mn has a minimum overpotential of 0.35 V for oxygen reduction reaction, and Fe2Co–Co possesses the smallest overpotential of 0.32 V for oxygen evolution reaction, respectively 100 and 50 mV lower than those of Pt(111) and RuO2(110) catalysts. The analysis of the potential gap of Fe2M clusters indicates that Fe2Mn, Fe2Co, and Fe2Ni clusters possess good bifunctional catalytic activity. Additionally, the catalytic activity of Fe2Mn and Fe2Co connected through 3,3′,5,5′-azobenzenetetracarboxylate linker to form Fe2M–PCN–Fe2M is explored. Compared with Fe2Mn–PCN–Fe2Mn, Fe2Co–PCN–Fe2Co, and isolated Fe2M clusters, the mixed-metal Fe2Co–PCN–Fe2Mn possesses excellent bifunctional catalytic activity, and the values of potential gap on the Mn and Co sites of Fe2Co–PCN–Fe2Mn are 0.69 and 0.70 V, respectively. Furthermore, the analysis of the electron structure indicates that constructing a mixed-metal cluster can efficiently enhance the electronic properties of the catalyst. In conclusion, the mixed-metal cluster strategy provides a new approach to further design and synthesize high-efficiency bifunctional electrocatalysts.

关键词： bimetallic metal–organic frameworks     bifunctional electrocatalyst     density functional theory     oxygen reduction reaction     oxygen evolution reaction    

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Iterative HOEO fusion strategy: a promising tool for enhancing bearing fault feature

《机械工程前沿（英文）》 2023年 第18卷 第1期 doi: 10.1007/s11465-022-0725-z

摘要： As parameter independent yet simple techniques, the energy operator (EO) and its variants have received considerable attention in the field of bearing fault feature detection. However, the performances of these improved EO techniques are subjected to the limited number of EOs, and they cannot reflect the non-linearity of the machinery dynamic systems and affect the noise reduction. As a result, the fault-related transients strengthened by these improved EO techniques are still subject to contamination of strong noises. To address these issues, this paper presents a novel EO fusion strategy for enhancing the bearing fault feature nonlinearly and effectively. Specifically, the proposed strategy is conducted through the following three steps. First, a multi-dimensional information matrix (MDIM) is constructed by performing the higher order energy operator (HOEO) on the analysis signal iteratively. MDIM is regarded as the fusion source of the proposed strategy with the properties of improving the signal-to-interference ratio and suppressing the noise in the low-frequency region. Second, an enhanced manifold learning algorithm is performed on the normalized MDIM to extract the intrinsic manifolds correlated with the fault-related impulses. Third, the intrinsic manifolds are weighted to recover the fault-related transients. Simulation studies and experimental verifications confirm that the proposed strategy is more effective for enhancing the bearing fault feature than the existing methods, including HOEOs, the weighting HOEO fusion, the fast Kurtogram, and the empirical mode decomposition.

关键词： higher order energy operator     fault diagnosis     manifold learning     rolling element bearing     information fusion    

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New analysis model for rotor-bearing systems based on plate theory

Zhinan ZHANG, Mingdong ZHOU, Weimin DING, Huifang MA

《机械工程前沿（英文）》 2019年 第14卷 第4期   页码 461-473 doi: 10.1007/s11465-019-0525-2

摘要： The purpose of this work is to develop a new analysis model for angular-contact, ball-bearing systems on the basis of plate theory instead of commonly known approaches that utilize spring elements. Axial and radial stiffness on an annular plate are developed based on plate, Timoshenko beam, and plasticity theories. The model is developed using theoretical and inductive methods and validated through a numerical simulation with the finite element method. The new analysis model is suitable for static and modal analyses of rotor-bearing systems. Numerical examples are presented to reveal the effectiveness and applicability of the proposed approach.

关键词： rotor-bearing system     rolling element bearing     plate theory     finite element analysis    

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API-based assessment on urban air environment bearing capability in China

Jinnan WANG,Jing ZHANG,Hongqiang JIANG,Yaling LU

《环境科学与工程前沿（英文）》 2015年 第9卷 第6期   页码 1049-1055 doi: 10.1007/s11783-014-0662-0

摘要： Given the complexity and time-consuming of the conventional environmental capacity based assessment on air environment carrying capacity; a new method for assessing urban air environment carrying capacity based on air pollution index (API) is presented. By using this new method, the air environmental bearing capability of 333 cities at the prefecture level and above is assessed. The results show that of the 333 cities 9.6% is of high bearing capability, 34.5% relatively high bearing capability, 52.6% medium bearing capability, 2.7% low capability, and 0.6% is of weak bearing capability; in terms of regional distribution, the western region is of relatively high air environment bearing capability, followed by north-eastern and eastern regions, and the ambient air quality in the middle region is quite poor; among the 12 urban agglomerations in key regions, Pearl River delta, west side of Taiwan Strait and Chengdu-Chongqing agglomerations are of relatively high carrying capacity while other agglomerations are of medium bearing capability. The assessment results imply that the existing air quality standard (GB3095-1996) is quite unsound.

关键词： air pollution index (API)     air environment bearing capability     key city     assessment method    

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Interface engineering for enhancing electrocatalytic oxygen evolution reaction of CoS/CeO heterostructures

《化学科学与工程前沿（英文）》 2022年 第16卷 第3期   页码 376-383 doi: 10.1007/s11705-021-2062-x

摘要： To realize renewable energy conversion, it is important to develop low-cost and high-efficiency electrocatalyst for oxygen evolution reaction. In this communication, a novel bijunction CoS/CeO2 electrocatalyst grown on carbon cloth is prepared by the interface engineering. The interface engineering of CoS and CeO2 facilitates a rapid charge transfer from CeO2 to CoS. Such an electrocatalyst exhibits outstanding electrocatalytic activity with a low overpotential of 311 mV at 10 mA∙cm−2 and low Tafel slope of 76.2 mV∙dec–1, and is superior to that of CoS (372 mV) and CeO2 (530 mV) counterparts. And it has long-term durability under alkaline media.

关键词： interface engineering     CoS/CeO2     electrodeposition     electrocatalyst     oxygen evolution reaction    

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The convexity about ultimate bearing hypersurfaces of structures

Chengxi GUO,Tingting GUO

《结构与土木工程前沿（英文）》 2016年 第10卷 第4期   页码 456-461 doi: 10.1007/s11709-016-0334-1

摘要： The relationship between the convexity on the ultimate bearing surface of a structure and the second-order effects of loads is discussed. All of generalized non-overload forces acted on a structure forms a convex set when ignoring the second-order effects (coupling effects between the generalized forces). It is true also when the Hessian matrix composed of the second-order partial derivatives on the hypersurface about the ultimate bearing of the structure is negative definite. The outward convexity is kept when the surface is expressed by certain dimensionless parameters. A series of properties based on the convexity are pointed out. Some applications in the analysis of bearing capacity of structures were illustrated with examples. The study shows that an evaluation about the bearing capacity state of a complex structure can be made on the basis of several points on the surface of the ultimate bearing of the structure.

关键词： service     limit load     ultimate bearing surface     convexity     generalized force     generalized displacement     frame structure    

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Foundations bearing capacity subjected to seepage by the kinematic approach of the limit analysis

Mehdi VEISKARAMI, Ghasem HABIBAGAHI

《结构与土木工程前沿（英文）》 2013年 第7卷 第4期   页码 446-455 doi: 10.1007/s11709-013-0227-5

摘要： An estimate of the ultimate load on foundations on soil layers subject to groundwater flow has been presented. The kinematic approach of the limit analysis was employed to find the upper-bound limit of the bearing capacity. Both smooth and rough base strip foundations were considered associated with different collapse patterns. Presence of the groundwater flow leads to a non-symmetric collapse pattern, i.e., a weak side and a strong side in two-sided collapse patterns, depending on the direction of the flow. It was found that the bearing capacity has a decreasing trend with increase in the groundwater flow gradient and hence, a reduction factor has been introduced to the third term in the bearing capacity equation as a function of the flow gradient.

关键词： foundation     bearing capacity     limit analysis     numerical computation     plasticity     seepage    

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Undrained seismic bearing capacity of strip footing adjacent to a heterogeneous excavation

《结构与土木工程前沿（英文）》 2023年 第17卷 第4期   页码 566-583 doi: 10.1007/s11709-023-0905-x

摘要： The analysis of the bearing capacity of strip footings sited near an excavation is critical in geotechnics. In this study, the effects of the geometrical features of the excavation and the soil strength properties on the seismic bearing capacity of a strip footing resting on an excavation were evaluated using the lower and upper bounds of the finite element limit analysis method. The effects of the setback distance ratio (L/B), excavation height ratio (H/B), soil strength heterogeneity (kB/cu), and horizontal earthquake coefficient (kh) were analyzed. Design charts and tables were produced to clarify the relationship between the undrained seismic bearing capacity and the selected parameters.

关键词： excavation     finite element limit analysis     heterogeneous soil     strip footing     undrained bearing capacity    

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High-entropy catalysts for electrochemical water-electrolysis of hydrogen evolution and oxygen evolution

《能源前沿（英文）》 doi: 10.1007/s11708-023-0892-6

摘要： High entropy materials (HEMs) have developed rapidly in the field of electrocatalytic water-electrolysis for oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) due to their unique properties. In particular, HEM catalysts are composed of many elements. Therefore, they have rich active sites and enhanced entropy stability relative to single atoms. In this paper, the preparation strategies and applications of HEM catalysts in electrochemical water-electrolysis are reviewed to explore the stabilization of HEMs and their catalytic mechanisms as well as their application in support green hydrogen production. First, the concept and four characteristics of HEMs are introduced based on entropy and composition. Then, synthetic strategies of HEM catalysts are systematically reviewed in terms of the categories of bottom-up and top-down. The application of HEMs as catalysts for electrochemical water-electrolysis in recent years is emphatically discussed, and the mechanisms of improving the performance of electrocatalysis is expounded by combining theoretical calculation technology and ex-situ/in situ characterization experiments. Finally, the application prospect of HEMs is proposed to conquer the challenges in HEM catalyst fabrications and applications.

关键词： high-entropy     electrocatalysis     synthetic methods     water-electrolysis     hydrogen and oxygen evolutions    

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Influence of the Mechanical Seals on the Dynamic Performance of Rotor–Bearing Systems

XU Hua, ZHU Jun

《机械工程前沿（英文）》 2006年 第1卷 第1期   页码 96-100 doi: 10.1007/s11465-005-0008-5

摘要：

In this paper, to consider the effects of mechanical seals, a lumped-mass model and the transfer matrix method are used to establish the equations for the dynamics performance of rotor bearing system. The general inverted iteration method is also used to solve the eigenvalue problem of these equations. To check the response of the rotor bearing system under unbalance motivation, the Gauss method is used to calculate the dynamic response of the constrained vibration. The results, based on the dynamic properties calculation of a typical mechanical spiral seal, such as stiffness coefficients and damping coefficients, exert the influence of the mechanical seal on the rotor bearing system of the high-speed machinery. Meanwhile, some structure parameters that may affect the dynamic performance and forced vibration under unbalance motivation of the rotor bearing system considering mechanical seals are analyzed in the paper. The analysis results show that the mechanical seal more or less has effects on the rotor bearing system. The mechanical seal has much more effects on the flexible rotor bearing system than on the rigid one. For instance, in a certain case, if the effects of the mechanical seal were taken into account, the system s critical speed may increase by 70 80%.

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A review of Pt-based electrocatalysts for oxygen reduction reaction

Changlin ZHANG, Xiaochen SHEN, Yanbo PAN, Zhenmeng PENG

《能源前沿（英文）》 2017年 第11卷 第3期   页码 268-285 doi: 10.1007/s11708-017-0466-6

摘要： Development of active and durable electrocatalyst for oxygen reduction reaction (ORR) remains one challenge for the polymer electrolyte membrane fuel cell (PEMFC) technology. Pt-based nanomaterials show the greatest promise as electrocatalyst for this reaction among all current catalytic structures. This review focuses on Pt-based ORR catalyst material development and covers the past achievements, current research status and perspectives in this research field. In particular, several important categories of Pt-based catalytic structures and the research advances are summarized. Key factors affecting the catalyst activity and durability are discussed. An outlook of future research direction of ORR catalyst research is provided.

关键词： oxygen reduction reaction (ORR)     electrocatalysis     platinum catalyst     activity     durability    

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Ultimate bearing capacity of strip footing resting on clay soil mixed with tire-derived aggregates

《结构与土木工程前沿（英文）》 2021年 第15卷 第4期   页码 1016-1024 doi: 10.1007/s11709-021-0751-7

摘要： This study investigated the use of recycled tire-derived aggregate (TDA) mixed with kaolin as a method of increasing the ultimate bearing capacity ( UBC) of a strip footing. Thirteen 1g physical modeling tests were prepared in a rigid box of 0.6 m × 0.9 m in plan and 0.6 m in height. During sample preparation, 0%, 20%, 40%, or 60% (by weight) of powdery, shredded, small-sized granular (G 1–4 mm) or large-sized granular (G 5–8 mm) TDA was mixed with the kaolin. A strip footing was then placed on the stabilized kaolin and was caused to fail under stress-controlled conditions to determine the UBC. A rigorous 3D finite element analysis was developed in Optum G-3 to determine the UBC values based on the experimental test results. The experimental results showed that, except for the 20% powdery TDA, the TDA showed an increase in the UBC of the strip footing. When kaolin mixed with 20% G (5–8 mm), the UBC showed a threefold increase over that for the unreinforced case. The test with 20% G (1–4 mm) recorded the highest subgrade modulus. It was observed that the UBC calculated using finite element modeling overestimated the experimental UBC by an average of 9%.

关键词： kaolin     physical modeling tests     stabilization     numerical modeling    

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Temperature control of transfer roller’s bearing based on finite element analysis

Peng ZHANG, Yourong LI, Han XIAO

《机械工程前沿（英文）》 2009年 第4卷 第2期   页码 215-218 doi: 10.1007/s11465-009-0026-9

摘要： After a heat preservation cover is installed on the main rolling line, the heat dissipation environment of the transfer roller working on the heat preservation cover is changed. To ensure the normal production, a reasonable working jet capacity of the roller neck is derived. First, a globe model of the transfer roller is built for finite element analysis. Second, the sub-model of the fixed end bearing is built and the boundary condition of the sub-model is supplied by the results of the globe model. The analysis result of the sub-model shows that the temperature of the transfer roller bearing exceeds 85°C a rolling periodicity later. With finite element analysis, the heat flux is obtained and the minimum working jet capacity is derived.

关键词： transfer roller bearing     finite element analysis     sub-model     temperature control    

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标题 作者 时间 类型 操作

Liquefaction and impurity separation of oxygen-bearing coal-bed methane

Qiuying LI, Yonglin JU, Li WANG,

期刊论文

The catalytic effect of both oxygen-bearing functional group and ash in carbonaceous catalyst on CH 4

Weidong ZHANG, Yongfa ZHANG,

期刊论文

Heterometallic cluster-based organic frameworks as highly active electrocatalysts for oxygen reductionand oxygen evolution reaction: a density functional theory study

期刊论文

Iterative HOEO fusion strategy: a promising tool for enhancing bearing fault feature

期刊论文

New analysis model for rotor-bearing systems based on plate theory

Zhinan ZHANG, Mingdong ZHOU, Weimin DING, Huifang MA

期刊论文

API-based assessment on urban air environment bearing capability in China

Jinnan WANG,Jing ZHANG,Hongqiang JIANG,Yaling LU

期刊论文

Interface engineering for enhancing electrocatalytic oxygen evolution reaction of CoS/CeO heterostructures

期刊论文

The convexity about ultimate bearing hypersurfaces of structures

Chengxi GUO,Tingting GUO

期刊论文

Foundations bearing capacity subjected to seepage by the kinematic approach of the limit analysis

Mehdi VEISKARAMI, Ghasem HABIBAGAHI

期刊论文

Undrained seismic bearing capacity of strip footing adjacent to a heterogeneous excavation

期刊论文

High-entropy catalysts for electrochemical water-electrolysis of hydrogen evolution and oxygen evolution

期刊论文

Influence of the Mechanical Seals on the Dynamic Performance of Rotor–Bearing Systems

XU Hua, ZHU Jun

期刊论文

A review of Pt-based electrocatalysts for oxygen reduction reaction

Changlin ZHANG, Xiaochen SHEN, Yanbo PAN, Zhenmeng PENG

期刊论文

Ultimate bearing capacity of strip footing resting on clay soil mixed with tire-derived aggregates

期刊论文

Temperature control of transfer roller’s bearing based on finite element analysis

Peng ZHANG, Yourong LI, Han XIAO

期刊论文