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Nonpolar cross-stacked super-aligned carbon nanotube membrane for efficient wastewater treatment

《环境科学与工程前沿（英文）》 2023年 第17卷 第3期 doi: 10.1007/s11783-023-1630-3

摘要：

● A novel nonpolar super-aligned carbon nanotube (SACNT) membrane was prepared.

关键词： Membrane fouling     Wastewater     Membrane separation     Antifouling     Aligned carbon nanotube    

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Velocity gradient elasticity for nonlinear vibration of carbon nanotube resonators

Hamid M. SEDIGHI, Hassen M. OUAKAD

《结构与土木工程前沿（英文）》 2020年 第14卷 第6期   页码 1520-1530 doi: 10.1007/s11709-020-0672-x

摘要： In this study, for the first time, we investigate the nonlocality superimposed to the size effects on the nonlinear dynamics of an electrically actuated single-walled carbon-nanotube-based resonator. We undertake two models to capture the nanostructure nonlocal size effects: the strain and the velocity gradient theories. We use a reduced-order model based on the differential quadrature method (DQM) to discretize the governing nonlinear equation of motion and acquire a discretized-parameter nonlinear model of the system. The structural nonlinear behavior of the system assuming both strain and velocity gradient theories is investigated using the discretized model. The results suggest that nonlocal and size effects should not be neglected because they improve the prediction of corresponding dynamic amplitudes and, most importantly, the critical resonant frequencies of such nanoresonators. Neglecting these effects may impose a considerable source of error, which can be amended using more accurate modeling techniques.

关键词： velocity gradient elasticity theory     nanotube resonators     differential-quadrature method     nonlinear vibration    

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Large-scale synthesis of isolated Mn2O3 nanotube/fiber with ferric nitrate as catalyst

ZHANG Aifei, LIU Jiping, L? Guangshu

《化学科学与工程前沿（英文）》 2007年 第1卷 第1期   页码 55-58 doi: 10.1007/s11705-007-0011-y

摘要： Isolated MnO nanotubes and nanofibers were prepared very easily at a large scale with the liquid-phase catalysis method. The MnO nanotubes had dimensions of 30 50 nm (exterior diameter) and 0.2 1.0 ?m (length), approximately. The O nanofibers had dimensions of 10 30 nm (diameter) and 0.4 2.0 ?m (length), approximately. Nano-O with different microstructures including nanotubes, nanofibers and nanoparticles could be selectively synthesized by controlling the contents and proportions of potassium permanganate and ferric nitrate. Ferric nitrate was an ideal catalyst for the preparation of O nanotube/fiber. When cobalt nitrate or nickel nitrate was used as catalyst, only amorphous nano-O was synthesized. X-ray diffraction (XRD) result shows that the O nanotube has a crystalline structure different from o-O, t-O, h-O and ?-O.

关键词： different     nickel     exterior diameter     nanotube     XRD    

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The role of ions in plasma catalytic carbon nanotube growth: A review

Erik C. Neyts

《化学科学与工程前沿（英文）》 2015年 第9卷 第2期   页码 154-162 doi: 10.1007/s11705-015-1515-5

摘要： While it is well-known that the plasma-enhanced catalytic chemical vapor deposition (PECVD) of carbon nanotubes (CNTs) offers a number of advantages over thermal CVD, the influence of the various individual contributing factors is not well understood. Especially the role of ions is unclear, since ions in plasmas are generally associated with sputtering rather than with growing a material. Even so, various studies have demonstrated the beneficial effects of ion bombardment during the growth of CNTs. This review looks at the role of the ions in plasma-enhanced CNT growth as deduced from both experimental and simulation studies. Specific attention is paid to the beneficial effects of ion bombardment. Based on the available literature, it can be concluded that ions can be either beneficial or detrimental for carbon nanotube growth, depending on the exact conditions and the control over the growth process.

关键词： plasma-enhanced chemical vapor deposition (PECVD)     carbon nanotube (CNT)     ion bombardment     defect healing    

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Nonlinear dynamic analysis of functionally graded carbon nanotube-reinforced composite plates using MISQ20

《结构与土木工程前沿（英文）》 2023年 第17卷 第7期   页码 1072-1085 doi: 10.1007/s11709-023-0951-4

摘要： The main objective of this study is to further extend the mixed integration smoothed quadrilateral element with 20 unknowns of displacement (MISQ20) to investigate the nonlinear dynamic responses of functionally graded carbon nanotube-reinforced composite (FG-CNTRC) plates with four types of carbon nanotube distributions. The smooth finite element method is used to enhance the accuracy of the Q4 element and avoid shear locking without using any shear correction factors. This method yields accurate results even if the element exhibits a concave quadrilateral shape and reduces the error when the element meshing is rough. Additionally, the element stiffness matrix is established by integrating the boundary of the smoothing domains. The motion equation of the FG-CNTRC plates is solved by adapting the Newmark method combined with the Newton–Raphson algorithm. Subsequently, the calculation program is coded in the MATLAB software and verified by comparing it with other published solutions. Finally, the effects of the input parameters on the nonlinear vibration of the plates are investigated.

关键词： carbon nanotube     MISQ20     FG-CNTRC plate     nonlinear vibration     nonlinear dynamic analysis     SFEM    

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Polypyrrole@NiCo hybrid nanotube arrays as high performance electrocatalyst for hydrogen evolution reaction

Shenghua Ye, Gaoren Li

《化学科学与工程前沿（英文）》 2018年 第12卷 第3期   页码 473-480 doi: 10.1007/s11705-018-1724-9

摘要：

The polypyrrole(PPy)@NiCo hybrid nanotube arrays have been successfully fabricated as a high performance electrocatalyst for hydrogen evolution reaction (HER) in alkaline solution. The strong electronic interactions between PPy and NiCo alloy are confirmed by X-ray photoelectron spectroscopy and Raman spectra. Because these interations can remarkably reduce the apparent activation energy (Ea) for HER and enhance the turnover frequency of catalysts, the electrocatalytic performance of PPy@NiCo hybrid nanotube arrays are significantly improved. The electrochemical tests show that the PPy@NiCo hybrid catalysts exhibit a low overpotential of ~186 mV at 10.0 mA·cm−2 and a small tafel slope of 88.6 mV·deg−1 for HER in the alkaline solution. The PPy@NiCo hybrid nanotubes also exhibit high catalytic activity and high stability for HER.

关键词： NiCo alloy     polypyrrole     hybrid nanotube     electrocatalyst     hydrogen evolution reaction    

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A deep feed-forward neural network for damage detection in functionally graded carbon nanotube-reinforced

《结构与土木工程前沿（英文）》 2021年 第15卷 第6期   页码 1453-1479 doi: 10.1007/s11709-021-0767-z

摘要： This paper proposes a new Deep Feed-forward Neural Network (DFNN) approach for damage detection in functionally graded carbon nanotube-reinforced composite (FG-CNTRC) plates. In the proposed approach, the DFNN model is developed based on a data set containing 20 000 samples of damage scenarios, obtained via finite element (FE) simulation, of the FG-CNTRC plates. The elemental modal kinetic energy (MKE) values, calculated from natural frequencies and translational nodal displacements of the structures, are utilized as input of the DFNN model while the damage locations and corresponding severities are considered as output. The state-of-the art Exponential Linear Units (ELU) activation function and the Adamax algorithm are employed to train the DFNN model. Additionally, in order to enhance the performance of the DFNN model, the mini-batch and early-stopping techniques are applied to the training process. A trial-and-error procedure is implemented to determine suitable parameters of the network such as the number of hidden layers and the number of neurons in each layer. The accuracy and capability of the proposed DFNN model are illustrated through two distinct configurations of the CNT-fibers constituting the FG-CNTRC plates including uniform distribution (UD) and functionally graded-V distribution (FG-VD). Furthermore, the performance and stability of the DFNN model with the consideration of noise effects on the input data are also investigated. Obtained results indicate that the proposed DFNN model is able to give sufficiently accurate damage detection outcomes for the FG-CNTRC plates for both cases of noise-free and noise-influenced data.

关键词： damage detection     deep feed-forward neural networks     functionally graded carbon nanotube-reinforced composite plates     modal kinetic energy    

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Temperature difference-powered carbon nanotube bearings

Quanwen HOU, Bingyang CAO, Zengyuan GUO

《能源前沿（英文）》 2011年 第5卷 第1期   页码 49-52 doi: 10.1007/s11708-010-0111-0

摘要： Molecular dynamics simulations are conducted to study the motion of carbon nanotube-based nanobearings powered by temperature difference. When a temperature difference exists between stator nanotubes, the rotor nanotubes acquire a higher temperature, which arises from the interaction between phonon currents and nanotubes. The thermal driving force increases with the increase in temperature difference between the stators, an increase that is nearly proportional to the temperature difference. Confined by the minimum energy track, the (5, 5)@(10, 10) nanotube bearings only translate along the axis direction but without successive rotation.

关键词： temperature difference-induced motion     carbon nanotubes     nanobearing     molecular dynamics simulation    

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Electrocatalytic reduction of nitrate using Pd-Cu modified carbon nanotube membranes

《环境科学与工程前沿（英文）》 2023年 第17卷 第4期 doi: 10.1007/s11783-023-1640-1

摘要：

● Pd-Cu modified CNT membranes were prepared successfully by electrodeposition method.

关键词： Pd-Cu modified CNT membrane     Nitrate reduction     Flow-through     Electrodeposition     Electrocatalytic reduction    

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Erratum to: Polypyrrole@NiCo hybrid nanotube arrays as high performance electrocatalyst for hydrogen

Shenghua Ye, Gaoren Li

《化学科学与工程前沿（英文）》 2019年 第13卷 第4期   页码 845-845 doi: 10.1007/s11705-019-1879-z

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Insights into the electron transfer mechanisms of permanganate activation by carbon nanotube membrane

《环境科学与工程前沿（英文）》 2023年 第17卷 第9期 doi: 10.1007/s11783-023-1706-0

摘要：

● A CNT filter enabled effective KMnO4 activation via facilitated electron transfer.

关键词： KMnO4     Carbon nanotubes     Non-radical pathway     Electron transfer     Water treatment    

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Strengthening mechanisms in carbon nanotube reinforced bioglass composites

Jing ZHANG, Chengchang JIA, Zhizhong JIA, Jillian LADEGARD, Yanhong GU, Junhui NIE

《化学科学与工程前沿（英文）》 2012年 第6卷 第2期   页码 126-131 doi: 10.1007/s11705-012-1279-0

摘要： Carbon nanotube reinforced bioglass composites have been successfully synthesized by two comparative sintering techniques, i.e., spark plasma sintering (SPS) and conventional compaction and sinteirng. The composites show improved mechanical properties, with SPS technique substantially better than conventional compact and sintering approach. Using SPS, compared with the 45S5Bioglass matrix, the maximum flexural strength and fracture toughness increased by 159% and 105%, respectively. Enhanced strength and toughness are attributed to the interfacial bonding and bridging effects between the carbon nanotubes and bioglass powders during crack propagations.

关键词： 45S5Bioglass     multi-wall carbon nanotubes     biocomposite     mechanical properties     sintering    

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Interlayer-confined two-dimensional manganese oxide-carbon nanotube catalytic ozonation membrane for

《化学科学与工程前沿（英文）》 2022年 第16卷 第5期   页码 731-744 doi: 10.1007/s11705-021-2110-6

摘要： Catalytic ozonation technology has attracted copious attention in water purification owing to its favorable oxidative degradation of pollutants and mitigation of membrane fouling capacity. However, its extensive industrial application has been restricted by the low ozone utilization and limited mass transfer of the short-lived radical species. Interlayer space-confined catalysis has been theoretically proven to be a viable strategy for achieving high catalytic efficiency. Here, a two-dimensional MnO2-incorporated ceramic membrane with tunable interspacing, which was obtained via the intercalation of a carbon nanotube, was designed as a catalytic ozonation membrane reactor for degrading methylene blue. Benefiting from the abundant catalytic active sites on the surface of two-dimensional MnO2 as well as the ultralow mass transfer resistance of fluids due to the nanolayer confinement, an excellent mineralization effect, i.e., 1.2 mg O3(aq) mg–1 TOC removal (a total organic carbon removal rate of 71.5%), was achieved within a hydraulic retention time of 0.045 s of pollutant degradation. Further, the effects of hydraulic retention time and interlayer spacing on methylene blue removal were investigated. Moreover, the mechanism of the catalytic ozonation employing catalytic ozonation membrane was proposed based on the contribution of the Mn(III/IV) redox pair to electron transfer to generate the reactive oxygen species. This innovative two-dimensional confinement catalytic ozonation membrane could act as a nanoreactor and separator to efficiently oxidize organic pollutants and enhance the control of membrane fouling during water purification.

关键词： catalytic membrane reactor     catalytic ozonation     nanoconfinement     two-dimensional manganese oxide    

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Cross-stacked super-aligned carbon nanotube/activated carbon composite electrodes for efficient water

Min Li, Shuai Liang, Yang Wu, Meiyue Yang, Xia Huang

《环境科学与工程前沿（英文）》 2020年 第14卷 第6期 doi: 10.1007/s11783-020-1286-1

摘要： Abstract • A high-performance electrode was prepared with super-aligned carbon nanotubes. • SACNT/AC electrode achieved a ~100% increase in desalination capacity and rate. • SACNT/AC electrode achieved a ~26% increase in charge efficiency. • CUF process with SACNT/AC achieved an up to 2.43-fold fouling reduction. • SACNT/AC imparts overall improved water purification efficiency. The practical application of the capacitive deionization (CDI) enhanced ultrafiltration (CUF) technology is hampered due to low performance of electrodes. The current study demonstrated a novel super-aligned carbon nanotube (SACNT)/activated carbon (AC) composite electrode, which was prepared through coating AC on a cross-stacked SACNT film. The desalination capability and water purification performance of the prepared electrode were systematically investigated at different applied voltages (0.8–1.2 V) with a CDI system and a CUF system, respectively. In the CDI tests, as compared with the control AC electrode, the SACNT/AC electrode achieved an approximately 100% increase in both maximum salt adsorption capacity and average salt adsorption rate under all the applied voltage conditions, demonstrating a superior desalination capability. Meanwhile, a conspicuous increase by an average of ~26% in charge efficiency was also achieved at all the voltages. In the CUF tests, as compared with the control run at 0 V, the treatment runs at 0.8, 1.0, and 1.2 V achieved a 2.40-fold, 2.08-fold, and 2.43-fold reduction in membrane fouling (calculated according to the final transmembrane pressure (TMP) data at the end of every purification stage), respectively. The average TMP increasing rates at 0.8, 1.0, and 1.2 V were also roughly two times smaller than that at 0 V, indicating a dramatical reduction of membrane fouling. The SACNT/AC electrode also maintained its superior desalination capability in the CUF process, resulting in an overall improved water purification efficiency.

关键词： Carbon nanotube     Super aligned     Conductive membrane     Capacitive deionization     Ultrafiltration     Desalination    

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Application and structure of carbon nanotube and graphene-based flexible electrode materials and assembly

《能源前沿（英文）》 doi: 10.1007/s11708-024-0911-2

摘要： In recent years, the rapid development of portable/wearable electronics has created an urgent need for the development of flexible energy storage devices. Flexible lithium-ion batteries (FLIBs) have emerged as the most attractive and versatile flexible electronic storage devices available. Carbon nanotubes (CNTs) are hollow-structured tubular nanomaterials with high electrical conductivity, large specific surface area, and excellent mechanical properties. Graphene (G) is to some extent comparable to CNTs, because both have unlimited value in flexible electrodes. Herein, a systematic summary of the application of CNT and G in FLIBs electrodes is presented, including different functional applications and services at different temperatures. Furthermore, the effects of electrode structures, including powder, wire-shaped, and film-shaped structures, on electrochemical properties is highlighted. The assembly structures of the FLIBs consisting of CNT and G-based flexible electrodes to realize different functions, including bendability, stretchability, foldability, self-healing, and self-detecting, are systematically reviewed. The current challenges and development prospects of flexible CNT and G-based flexible electrodes and corresponding FLIBs are discussed.

关键词： flexible lithium-ion batteries (FLIBs)     carbon nanotubes (CNTs)     graphene (G)     electrode structure     function    

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标题 作者 时间 类型 操作

Nonpolar cross-stacked super-aligned carbon nanotube membrane for efficient wastewater treatment

期刊论文

Velocity gradient elasticity for nonlinear vibration of carbon nanotube resonators

Hamid M. SEDIGHI, Hassen M. OUAKAD

期刊论文

Large-scale synthesis of isolated Mn2O3 nanotube/fiber with ferric nitrate as catalyst

ZHANG Aifei, LIU Jiping, L? Guangshu

期刊论文

The role of ions in plasma catalytic carbon nanotube growth: A review

Erik C. Neyts

期刊论文

Nonlinear dynamic analysis of functionally graded carbon nanotube-reinforced composite plates using MISQ20

期刊论文

Polypyrrole@NiCo hybrid nanotube arrays as high performance electrocatalyst for hydrogen evolution reaction

Shenghua Ye, Gaoren Li

期刊论文

A deep feed-forward neural network for damage detection in functionally graded carbon nanotube-reinforced

期刊论文

Temperature difference-powered carbon nanotube bearings

Quanwen HOU, Bingyang CAO, Zengyuan GUO

期刊论文

Electrocatalytic reduction of nitrate using Pd-Cu modified carbon nanotube membranes

期刊论文

Erratum to: Polypyrrole@NiCo hybrid nanotube arrays as high performance electrocatalyst for hydrogen

Shenghua Ye, Gaoren Li

期刊论文

Insights into the electron transfer mechanisms of permanganate activation by carbon nanotube membrane

期刊论文

Strengthening mechanisms in carbon nanotube reinforced bioglass composites

Jing ZHANG, Chengchang JIA, Zhizhong JIA, Jillian LADEGARD, Yanhong GU, Junhui NIE

期刊论文

Interlayer-confined two-dimensional manganese oxide-carbon nanotube catalytic ozonation membrane for

期刊论文

Cross-stacked super-aligned carbon nanotube/activated carbon composite electrodes for efficient water

Min Li, Shuai Liang, Yang Wu, Meiyue Yang, Xia Huang

期刊论文

Application and structure of carbon nanotube and graphene-based flexible electrode materials and assembly

期刊论文